ICRP Publication 142: Radiological Protection from Naturally Occurring Radioactive Material (NORM) in Industrial Processes.

The purpose of this publication is to provide guidance on radiological protection in industries involving naturally occurring radioactive material (NORM). These industries may give rise to multiple hazards and the radiological hazard is not necessarily dominant. The industries are diverse and may involve exposure of people and the environment where protective actions need to be considered. In some cases, there is a potential for significant routine exposure of workers and members of the public if suitable control measures are not considered. Releases of large volumes of NORM may also result in detrimental effects on the environment from radiological and non-radiological constituents. However, NORM industries present no real prospect of a radiological emergency leading to tissue reactions or immediate danger for life. Radiological protection in industries involving NORM can be appropriately addressed on the basis of the principles of justification of the actions taken and optimisation of protection using reference levels. An integrated and graded approach is recommended for the protection of workers, the public, and the environment, where consideration of non-radiological hazards is integrated with radiological hazards, and the approach to protection is optimised (graded) so that the use of various radiological protection programme elements is consistent with the hazards while not imposing unnecessary burdens. For workers, the approach starts with characterisation of the exposure situation, and integration, as necessary, of specific radiological protective actions to complement the protection strategy already in place or planned to manage other workplace hazards. According to the characteristics of the exposure situation and the magnitude of the hazards, a relevant reference level should be selected and appropriate collective or individual protective actions taken. Exposure to radon is also treated using a graded approach, based first on application of typical radon prevention and mitigation techniques, as described in Publication 126. A similar approach should be implemented for public exposure through the control of discharges, wastes, and residues after characterisation of the situation. If the protection of non-human species is warranted, it should be dealt with after an assessment of radiological exposure appropriate for the circumstances, taking into account all hazards and impacts. This should include identification of exposed organisms in the environment, and use relevant derived consideration reference levels to inform decisions on options for control of exposure.

An evaluation of radiation exposures in a tropical phosphogypsum disposal environment.

Environmental radiological aspects of phosphatic fertiliser production with particular reference to disposal of phosphogypsum at two sites in India are examined. Concentration of uranium and its decay products in the rock phosphate and products are presented. External gamma exposure and inhalation of radon and progeny are found to be the major routes of exposure to public in phosphogypsum disposal environment. An estimate of the committed effective dose to a representative person gives an average additional dose of 0.6 mSv annually in the study sites.

Occupational radiation exposure due to norm in a rare-earth compounds production facility.

In India, rare-earth compounds are produced from the beach sand mineral monazite. Caustic digestion of the mineral followed by selective acid extraction is the method used to separate composite rare-earth fraction. The composite rare-earth chloride contains low levels of natural radionuclides and is the starting material for individual rare-earth compounds which have wide applications. Activity concentrations in composite rare-earth compounds such as chlorides, fluorides, carbonates and oxides of Ce, Nd, Pr, Sm, Gd, etc. are presented in this paper. The external gamma exposure rates and airborne activity due to thorium and thoron progeny in the occupational environment are studied. The activity levels in liquid effluent are presented. The potential individual occupational dose is estimated to be 1.9 mSv per annum.

Thorium in ilmenite and its radiological implications in the production of titanium dioxide.

This study gives the results of measurements of (232)Th and (228)Ra in the titanium mineral ilmenite and its derived products and an assessment of related radiological issues in mineral separation and titanium dioxide production plants in India. The concentrations of (232)Th and (228)Ra in ilmenite, synthetic rutile and TiO2 are presented along with percent distribution of the radionuclides in different stages of process. External gamma exposure rates and airborne thorium levels in plants processing such minerals are studied. The study estimated a potential external gamma exposure of 1 mSv and an inhalation dose of 0.7 mSv annually to the occupational worker due to the presence of naturally occurring radioactive material in these industries. The concentrations of the nuclides in liquid effluent and solid wastes are analysed, and disequilibria with respect to (228)Ra are observed.

Natural radionuclides in zircon and related radiological impacts in mineral separation plants.

The activity concentration of uranium and thorium present in zircon obtained from mineral sand industries are presented. External gamma radiation levels and inhalation of airborne dust are found to be the significant routes of radiation exposure to occupational workers. The annual average dose attributed to zircon processing is estimated to be 2.3 mSv in the plants under study. This paper presents the results of external gamma measurements, estimation of airborne radioactivity in zircon process locations and radon and thoron in the occupational environment of two mineral separation plants in India. Analyses of the solid wastes and liquid effluent generated and resultant environmental impacts are indicated.

Measurement of 40k as an indicator of body potassium: implication for diabetes and other disease conditions.

Potassium (K) content in 408 male workers of a rare earths processing plant was estimated using a shadow shield whole body counter. The average K content in the non-vegetarian and vegetarian group was found to be 1.5 g kg(-1) and 2.1 g kg(-1) respectively. The absorbed dose due to 40K is determined as 0.18 +/- 0.02 mGy. While the K content was found to be proportional to body build index, it is inversely proportional to slenderness. Body K was maximum in the middle aged group (35-45 y) and a minimum in younger and older persons. The correlation of potassium content with some disease patterns was also studied. Diabetes mellitus patients were observed to have low K content of 0.9 +/- 0.2 g kg(-1) and those who suffer from cardiovascular disorders were found to have high K content 2.7 +/- 0.3 g kg(-1). The studies showed that the depletion of body K content takes place a few years prior to the clinical detection of diabetes and it builds up a few years before the clinical detection of cardiovascular disorders. It is stressed that the medical information is preliminary as the number of subjects studied was not very large. Wider and in depth study by various groups can hopefully strengthen the observation.

Dissolution characteristics of 226Ra from phosphogypsum.

The paper presents the results of the dissolution characteristics of 226Ra from phosphogypsum, a by-product from phosphate fertilizer industries. Leachability of 226Ra in distilled water and rainwater have been examined under different leaching conditions such as contact time, solid:liquid ratio and simulating natural conditions. The concentration of 226Ra activity in the leachates ranged from 0.07 to 0.53 Bq l(-1). Study indicated that leaching of radium may be slow in field conditions near the phosphogypsum stock piles.

Natural radionuclides in the aquatic environment of a phosphogypsum disposal area.

Rock phosphate ore processing and disposal of phosphogypsum contribute to enhanced levels of natural radionuclides in the environment. Studies on the distribution of U-series nuclides were carried out in the Chitrapuzha River, near Cochin, in the southern part of India. The concentrations of radionuclides, especially 226Ra, in the river waters showed enhancement by an order of magnitude relative to the levels in nearby water bodies. The concentrations were influenced by seasonal changes in the river flows during monsoon and summer periods. Ingestion doses via fish and milk have an upper estimate of 18 microSv for the critical population.