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1.
J Environ Radioact ; 275: 107428, 2024 May.
Artigo em Inglês | MEDLINE | ID: mdl-38547560

RESUMO

In order to investigate the impact of environmental conditions on the distribution and migration of 90Sr in the Longji terrace environment, the activity concentrations of 90Sr and 137Cs were determined. The activity concentration ranges of 90Sr and 137Cs in surface soil were 0.15-1.04 Bq/kg and 2.16-6.94 Bq/kg, respectively. These results showed that there was a similar trend between the activity concentration of 90Sr and 137Cs in the surface soil along the runoff path and their activity concentration were influenced by the slope of the terraced terrain. On the other hand, the activity ranges of 90Sr and 137Cs in soil cores were 0.01-2.74 Bq/kg and 0.43-7.19 Bq/kg, respectively. These results indicate that the migration mechanism of 90Sr is different from that of 137Cs. As compared with 137Cs, 90Sr is significantly influenced by the moisture content. In addition, high span of 137Cs/90Sr activity ratios were found in this study, which were attributed to the characteristics of cultivated land and frequent artificial disturbances that intensified the migration of 90Sr.


Assuntos
Radioisótopos de Césio , Monitoramento de Radiação , Poluentes Radioativos do Solo , Radioisótopos de Estrôncio , Radioisótopos de Césio/análise , Radioisótopos de Estrôncio/análise , Poluentes Radioativos do Solo/análise
2.
Mar Pollut Bull ; 199: 115972, 2024 Feb.
Artigo em Inglês | MEDLINE | ID: mdl-38154170

RESUMO

To investigate the spatial distribution and source of plutonium isotopes in the Beibu Gulf, surface sediments were collected and analyzed using sector field inductively coupled plasma mass spectrometry (SF-ICP-MS). The activities of 239+240Pu in surface sediments ranged from 0.012 to 0.451 mBq/g (mean: 0.171 ± 0.138 mBq/g, n = 36), indicating a decreasing trend in a counterclockwise direction from the southern bay mouth. The counterclockwise decreasing trend in the south of the bay mouth is similar to the current in the Beibu Gulf. The 240Pu/239Pu atom ratios in surface sediments ranged from 0.156 to 0.283 (mean: 0.236 ± 0.031, n = 36), slightly higher than that of the global fallout value of 0.18. This suggests that the Pu in the Beibu Gulf was a combination of global fallout and Pacific Proving Ground (PPG). The average contribution of the plutonium (Pu) derived from the PPG in the sediment was estimated to be 52 % ± 24 %.


Assuntos
Plutônio , Monitoramento de Radiação , Cinza Radioativa , Poluentes Radioativos da Água , Sedimentos Geológicos/química , Plutônio/análise , Poluentes Radioativos da Água/análise , China , Cinza Radioativa/análise
3.
J Environ Radioact ; 261: 107145, 2023 May.
Artigo em Inglês | MEDLINE | ID: mdl-36870165

RESUMO

Radionuclides in environmental ecosystems have ecotoxicity and health impact on human and environment, so radioactive contamination has always been one of the global concerns. This study mainly focused on the radioactivity of mosses collected from the Leye Tiankeng Group in Guangxi. The activities of 239+240Pu measured by SF-ICP-MS and 137Cs measured by HPGe in moss and soil samples are as follows: 0-2.29 Bq/kg in mosses and 1.5-11.9 Bq/kg in soils for 137Cs, and 0.025-0.25Bq/kg in mosses and 0.07-0.51Bq/kg in soils for 239+240Pu. The range of 240Pu/239Pu atom ratios (0.201 in mosses and 0.184 in soils) and 239+240Pu/137Cs activity ratios (0.128 in mosses and 0.044 in soils) indicated that the 137Cs and 239+240Pu in study area were mainly contributed by global fallout. 137Cs and 239+240Pu showed similar distribution in soils. However, their behaviors in mosses were quite different due to the differences in the growth environment of mosses. The transfer factors of 137Cs and 239+240Pu from soil to moss varied in different growth stages and specific environments. A weak positive correlation among 137Cs, 239+240Pu in mosses and soil-derived radionuclides suggested that resettlement was predominant here. The negative correlation between 7Be, 210Pb and soil-derived radionuclides indicated that 7Be and 210Pb came from atmospheric components, while the weak correlation between them suggested that their specific sources were different. The Cu and Ni were moderately enriched in mosses here due to the use of agricultural fertilizers, At the same time, Zn was at a high level in the Lilang area, where transportation was more developed.


Assuntos
Briófitas , Plutônio , Monitoramento de Radiação , Radioatividade , Poluentes Radioativos do Solo , Humanos , Poluentes Radioativos do Solo/análise , Plutônio/análise , Ecossistema , Chumbo , China , Radioisótopos de Césio/análise , Solo
4.
Mar Pollut Bull ; 176: 113476, 2022 Mar.
Artigo em Inglês | MEDLINE | ID: mdl-35240458

RESUMO

Historical 90Sr activity in seawater was established in the China seas from 1963 to 2018. Based on the exponential decrease in 90Sr activity in seawater, the effective half-life (EHL) of 90Sr was quantified to be 11.5 ± 1.6 a, 16.5 ± 2.4 a, 27.2 ± 6.2 a, and 26.7 ± 4.3 a in the Bohai Sea, Yellow Sea, East China Sea, and South China Sea, respectively. We found contrasting patterns in the EHL of 90Sr and 137Cs in the marginal seas and open oceans that were closely related to the subtly different pathways of 90Sr and 137Cs in marine environment. Additionally, we demonstrated that Fukushima-derived 90Sr (<0.01 Bq/m3) would be difficult to identify in the China seas. Our study not only provided the key parameter of the EHL in marine models for predicting the 90Sr activity in the China seas in the post-Fukushima era but also enhanced our understanding of 90Sr behavior and its fate in marine environments.


Assuntos
Acidente Nuclear de Fukushima , Monitoramento de Radiação , Poluentes Radioativos da Água , China , Oceanos e Mares , Água do Mar , Radioisótopos de Estrôncio , Poluentes Radioativos da Água/análise
5.
Appl Radiat Isot ; 176: 109873, 2021 Oct.
Artigo em Inglês | MEDLINE | ID: mdl-34315033

RESUMO

Plutonium isotopes in the coral were determined with chemical separation method using AG 1-X8 and AG-MP-1M anion exchange resins and sector field inductively coupled plasma mass spectrometry (SF-ICP-MS) in order to elucidate the activity concentration and source of Pu around Weizhou land in Beibu Gulf, China. Furthermore, the activity concentrations of other radionuclides (238U, 226Ra, 232Th, 137Cs, 40K and 210Pb) were measured by a HPGe spectrometer. The activity concentration of 240+239Pu in the coral is determined to be in the range of 8.95-27.84 mBq/kg. The 240Pu/239Pu atom ratios in the samples range from 0.173 to 0.225, indicating that the main source of plutonium in this area is global fallout while the contribution of PPG is about 30%. Further, the activity concentrations of 238U, 232Th, 40K and 226Ra are determined to be in the range of 18.72-64.63, 1.37-20.8, 29.78-72.52 and 3.48-61.97 Bq/kg, respectively.


Assuntos
Antozoários/química , Plutônio/análise , Radioisótopos/análise , Poluentes Radioativos do Solo/análise , Poluentes Radioativos da Água/análise , Animais , China , Cinza Radioativa/análise
6.
PLoS One ; 15(9): e0239144, 2020.
Artigo em Inglês | MEDLINE | ID: mdl-32946477

RESUMO

In genome-wide association studies (GWAS), a wide variety of analysis tools have been designed, leading to various formats of GWAS data. How to convert a dataset in non-PLINK format into PLINK format to use its powerful analysis performance, or to convert a dataset in PLINK format into the format of other analysis tools, is a problem that needs to be faced and solved. To address this issue, we developed a tool called coPLINK, a complementary tool to PLINK, to cooperate with PLINK to implement the conversions of GWAS data formats and to provide some additional functions, such as data files comparison. The tool can implement mutual conversions not only between an existing data format and PLINK PED/BED, but also between a user-defined data format and PLINK PED. The usage and performance of the tool are similar to PLINK. The characteristics of the conversions of existing data formats and user-defined formats make it be a good assistant to PLINK or other tools and, have good potential for GWAS studies or other works.


Assuntos
Biologia Computacional/métodos , Estudo de Associação Genômica Ampla/estatística & dados numéricos , Técnicas de Genotipagem/métodos , Software , Estudos de Casos e Controles , Doença da Artéria Coronariana/genética , Interpretação Estatística de Dados , Conjuntos de Dados como Assunto , Estudos de Viabilidade , Técnicas de Genotipagem/estatística & dados numéricos , Humanos , Polimorfismo de Nucleotídeo Único
7.
PLoS One ; 14(7): e0219551, 2019.
Artigo em Inglês | MEDLINE | ID: mdl-31314810

RESUMO

The hypothesis of data probability density distributions has many effects on the design of a new statistical method. Based on the analysis of a group of real gene expression profiles, this study reveal that the primary density distributions of the real profiles are normal/log-normal and t distributions, accounting for 80% and 19% respectively. According to these distributions, we generated a series of simulation data to make a more comprehensive assessment for a novel statistical method, maximal information coefficient (MIC). The results show that MIC is not only in the top tier in the overall performance of identifying differentially expressed genes, but also exhibits a better adaptability and an excellent noise immunity in comparison with the existing methods.


Assuntos
Biologia Computacional/métodos , Perfilação da Expressão Gênica , Algoritmos , Animais , Área Sob a Curva , Bactérias , Simulação por Computador , Humanos , Modelos Lineares , Modelos Estatísticos , Plantas , Probabilidade , Reprodutibilidade dos Testes
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