Evidence for Quantum Stripe Ordering in a Triangular Optical Lattice.

Understanding strongly correlated quantum materials, such as high-T_{c} superconductors, iron-based superconductors, and twisted bilayer graphene systems, remains as one of the outstanding challenges in condensed matter physics. Quantum simulation with ultracold atoms in particular optical lattices, which provide orbital degrees of freedom, is a powerful tool to contribute new insights to this endeavor. Here, we report the experimental realization of an unconventional Bose-Einstein condensate of ^{87}Rb atoms populating degenerate p orbitals in a triangular optical lattice, exhibiting remarkably long coherence times. Using time-of-flight spectroscopy, we observe that this state spontaneously breaks the rotational symmetry and its momentum spectrum agrees with the theoretically predicted coexistence of exotic stripe and loop-current orders. Like certain strongly correlated electronic systems with intertwined orders, such as high-T_{c} cuprate superconductors, twisted bilayer graphene, and the recently discovered chiral density-wave state in kagome superconductors AV_{3}Sb_{5} (A=K, Rb, Cs), the newly demonstrated quantum state, in spite of its markedly different energy scale and the bosonic quantum statistics, exhibits multiple symmetry breakings at ultralow temperatures. These findings hold the potential to enhance our comprehension of the fundamental physics governing these intricate quantum materials.

Condensate Formation in a Dark State of a Driven Atom-Cavity System.

We demonstrate the formation of a condensate in a dark state of momentum states, in a pumped and shaken cavity-BEC system. The system consists of an ultracold quantum gas in a high-finesse cavity, which is pumped transversely by a phase-modulated laser. This phase-modulated pumping couples the atomic ground state to a superposition of excited momentum states, which decouples from the cavity field. We demonstrate how to achieve condensation in this state, supported by time-of-flight and photon emission measurements. With this, we show that the dark state concept provides a general approach to efficiently prepare complex many-body states in an open quantum system.

Experimental realization of a high precision tunable hexagonal optical lattice.

Hexagonal optical lattices offer a tunable platform to study exotic orbital physics in solid state materials. Here, we present a versatile high-precision scheme to implement a hexagonal optical lattice potential, which is engineered by overlapping two independent triangular optical sublattices generated by laser beams with slightly different wavelengths around 1064 nm. This enables us to precisely control the detailed structure of the hexagonal lattice by adjusting the relative position and the relative lattice depth of the two triangular optical sublattices. Taking advantage of the sensitive dependence of the second Bloch band on small lattice deformations, we propose a strategy to optimize the optical lattice geometry with an extremely high precision. This method can also be extended to other lattice configurations involving more than two sublattices. Our work provides the experimental requirements in the search for novel orbital physics of ultracold atoms, for example, in the flat p-band of the hexagonal optical lattice.

Observation of a continuous time crystal.

Time crystals are classified as discrete or continuous depending on whether they spontaneously break discrete or continuous time translation symmetry. Although discrete time crystals have been extensively studied in periodically driven systems, the experimental realization of a continuous time crystal is still pending. We report the observation of a limit cycle phase in a continuously pumped dissipative atom-cavity system that is characterized by emergent oscillations in the intracavity photon number. The phase of the oscillation was found to be random for different realizations, and hence, this dynamical many-body state breaks continuous time translation symmetry spontaneously. Furthermore, the observed limit cycles are robust against temporal perturbations and therefore demonstrate the realization of a continuous time crystal.

Observation of a Dissipative Time Crystal.

We present the first experimental realization of a time crystal stabilized by dissipation. The central signature in our implementation in a driven open atom-cavity system is a period doubled switching between distinct checkerboard density wave patterns, induced by the interplay between controlled cavity dissipation, cavity-mediated interactions, and external driving. We demonstrate the robustness of this dynamical phase against system parameter changes and temporal perturbations of the driving.

Evidence for an atomic chiral superfluid with topological excitations.

Topological superfluidity is an important concept in electronic materials as well as ultracold atomic gases1. However, although progress has been made by hybridizing superconductors with topological substrates, the search for a material-natural or artificial-that intrinsically exhibits topological superfluidity has been ongoing since the discovery of the superfluid 3He-A phase2. Here we report evidence for a globally chiral atomic superfluid, induced by interaction-driven time-reversal symmetry breaking in the second Bloch band of an optical lattice with hexagonal boron nitride geometry. This realizes a long-lived Bose-Einstein condensate of 87Rb atoms beyond present limits to orbitally featureless scenarios in the lowest Bloch band. Time-of-flight and band mapping measurements reveal that the local phases and orbital rotations of atoms are spontaneously ordered into a vortex array, showing evidence of the emergence of global angular momentum across the entire lattice. A phenomenological effective model is used to capture the dynamics of Bogoliubov quasi-particle excitations above the ground state, which are shown to exhibit a topological band structure. The observed bosonic phase is expected to exhibit phenomena that are conceptually distinct from, but related to, the quantum anomalous Hall effect3-7 in electronic condensed matter.

Realization of a Periodically Driven Open Three-Level Dicke Model.

A periodically driven open three-level Dicke model is realized by resonantly shaking the pump field in an atom-cavity system. As an unambiguous signature, we demonstrate the emergence of a dynamical phase, in which the atoms periodically localize between the antinodes of the pump lattice, associated with an oscillating net momentum along the pump axis. We observe this dynamical phase through the periodic switching of the relative phase between the pump and cavity fields at a small fraction of the driving frequency, suggesting that it exhibits a time crystalline character.

Pulse Delay Time Statistics in a Superradiant Laser with Calcium Atoms.

Cold samples of calcium atoms are prepared in the metastable ^{3}P_{1} state inside an optical cavity resonant with the narrow band (375 Hz) ^{1}S_{0}→^{3}P_{1} intercombination line at 657 nm. We observe a superradiant emission of hyperbolic secant shaped pulses into the cavity with an intensity proportional to the square of the atom number, a duration much shorter than the natural lifetime of the ^{3}P_{1} state, and a delay time fluctuating from shot to shot in excellent agreement with theoretical predictions. Our incoherent pumping scheme to produce inversion on the ^{1}S_{0}→^{3}P_{1} transition should be extendable to allow for continuous wave laser operation.

Light-Induced Coherence in an Atom-Cavity System.

We demonstrate a light-induced formation of coherence in a cold atomic gas system that utilizes the suppression of a competing density wave (DW) order. The condensed atoms are placed in an optical cavity and pumped by an external optical standing wave, which induces a long-range interaction mediated by photon scattering and a resulting DW order above a critical pump strength. We show that the light-induced temporal modulation of the pump wave can suppress this DW order and restore coherence. This establishes a foundational principle of dynamical control of competing orders analogous to a hypothesized mechanism for light-induced superconductivity in high-T_{c} cuprates.

Dynamical Control of Order in a Cavity-BEC System.

We demonstrate dynamical control of the superradiant transition of cavity-BEC system via periodic driving of the pump laser. We show that the dominant density wave order of the superradiant state can be suppressed, and that the subdominant competing order of Bose-Einstein condensation emerges in the steady state. Furthermore, we show that additional, nonequilibrium density wave orders, which do not exist in equilibrium, can be stabilized dynamically. Finally, for strong driving, chaotic dynamics emerge.

Rotation-Symmetry-Enforced Coupling of Spin and Angular Momentum for p-Orbital Bosons.

Intrinsic spin angular-momentum coupling of an electron has a relativistic quantum origin with the coupling arising from charged orbits, which does not carry over to charge-neutral atoms. Here, we propose a mechanism of spontaneous generation of spin angular-momentum coupling with spinor atomic bosons loaded into p-orbital bands of a two-dimensional optical lattice. This spin angular-momentum coupling originates from many-body correlations and spontaneous symmetry breaking in a superfluid, with the key ingredients attributed to spin-channel quantum fluctuations and an approximate rotation symmetry. The resultant spin angular-momentum intertwined superfluid has Dirac excitations. In the presence of a chemical potential difference for adjacent sites, it provides a bosonic analogue of a symmetry-protected-topological insulator. Through a dynamical mean-field calculation, this novel superfluid is found to be a generic low-temperature phase, and it gives way to Mott localization only at strong interactions and even-integer fillings. We show the temperature to reach this order is accessible with present experiments.

π-Flux Dirac Bosons and Topological Edge Excitations in a Bosonic Chiral p-Wave Superfluid.

We study the topological properties of elementary excitations in a staggered p_{x}±ip_{y} Bose-Einstein condensate realized in recent orbital optical lattice experiments. The condensate wave function may be viewed as a configuration space variant of the famous p_{x}+ip_{y} momentum space order parameter of strontium ruthenate superconductors. We show that its elementary excitation spectrum possesses Dirac bosons with π Berry flux. Remarkably, if we induce a population imbalance between the p_{x}+ip_{y} and p_{x}-ip_{y} condensate components, a gap opens up in the excitation spectrum resulting in a nonzero Chern invariant and topologically protected edge excitation modes. We give a detailed description of how our proposal can be implemented with standard experimental technology.

Dynamical phase transition in the open Dicke model.

The Dicke model with a weak dissipation channel is realized by coupling a Bose-Einstein condensate to an optical cavity with ultranarrow bandwidth. We explore the dynamical critical properties of the Hepp-Lieb-Dicke phase transition by performing quenches across the phase boundary. We observe hysteresis in the transition between a homogeneous phase and a self-organized collective phase with an enclosed loop area showing power-law scaling with respect to the quench time, which suggests an interpretation within a general framework introduced by Kibble and Zurek. The observed hysteretic dynamics is well reproduced by numerically solving the mean-field equation derived from a generalized Dicke Hamiltonian. Our work promotes the understanding of nonequilibrium physics in open many-body systems with infinite range interactions.

Proposed formation and dynamical signature of a chiral Bose liquid in an optical lattice.

Recent experiments on p-orbital atomic bosons have suggested the emergence of a spectacular ultracold superfluid with staggered orbital currents in optical lattices. This raises fundamental questions concerning the effects of thermal fluctuations as well as possible ways of directly observing such chiral order. Here we show via Monte Carlo simulations that thermal fluctuations destroy this superfluid in an unexpected two-step process, unveiling an intermediate normal phase with spontaneously broken time-reversal symmetry, dubbed a 'chiral Bose liquid'. For integer fillings (n≥2) in the chiral Mott regime, thermal fluctuations are captured by an effective orbital Ising model, and Onsager's powerful exact solution is adopted to determine the transition from this intermediate liquid to the para-orbital normal phase at high temperature. A lattice quench is designed to convert the staggered angular momentum, previously thought by experts difficult to directly probe, into coherent orbital oscillations, providing a time-resolved dynamical signature of chiral order.

Cavity cooling below the recoil limit.

Conventional laser cooling relies on repeated electronic excitations by near-resonant light, which constrains its area of application to a selected number of atomic species prepared at moderate particle densities. Optical cavities with sufficiently large Purcell factors allow for laser cooling schemes, avoiding these limitations. Here, we report on an atom-cavity system, combining a Purcell factor above 40 with a cavity bandwidth below the recoil frequency associated with the kinetic energy transfer in a single photon scattering event. This lets us access a yet-unexplored regime of atom-cavity interactions, in which the atomic motion can be manipulated by targeted dissipation with sub-recoil resolution. We demonstrate cavity-induced heating of a Bose-Einstein condensate and subsequent cooling at particle densities and temperatures incompatible with conventional laser cooling.

Topologically induced avoided band crossing in an optical checkerboard lattice.

We report on the condensation of bosons in the 4th band of an optical checkerboard lattice providing a topologically induced avoided band crossing involving the 2nd, 3rd, and 4th Bloch bands. When the condensate is slowly tuned through the avoided crossing, accelerated band relaxation arises and the zero momentum approximately C4-invariant condensate wave function acquires finite momentum order and reduced C2 symmetry. For faster tuning Landau-Zener oscillations between different superfluid orders arise, which are used to characterize the avoided crossing.

Unconventional superfluid order in the F band of a bipartite optical square lattice.

We report on the first observation of bosons condensed into the energy minima of an F band of a bipartite square optical lattice. Momentum spectra indicate that a truly complex-valued staggered angular momentum superfluid order is established. The corresponding wave function is composed of alternating local F2x3-3x ± iF2y3-3y orbits and local S orbits residing in the deep and shallow wells of the lattice, which are arranged as the black and white areas of a checkerboard. A pattern of staggered vortical currents arises, which breaks time-reversal symmetry and the translational symmetry of the lattice potential. We have measured the populations of higher order Bragg peaks in the momentum spectra for varying relative depths of the shallow and deep lattice wells and find remarkable agreement with band calculations.

Staggered-vortex superfluid of ultracold bosons in an optical lattice.

We show that the dynamics of cold bosonic atoms in a two-dimensional square optical lattice produced by a bichromatic light-shift potential is described by a Bose-Hubbard model with an additional effective staggered magnetic field. In addition to the known uniform superfluid and Mott insulating phases, the zero-temperature phase diagram exhibits a novel kind of finite-momentum superfluid phase, characterized by a quantized staggered rotational flux. An extension for fermionic atoms leads to an anisotropic Dirac spectrum, which is relevant to graphene and high-T(c) superconductors.

Observation of multichannel collisions of cold metastable calcium atoms.

Recent theoretical work indicates that collisions between metastable alkaline-earth atoms (AEAs) in the presence of external magnetic fields should be largely determined by partial waves with large angular momenta even at very low temperatures. Unusually large inelastic collision cross sections were predicted and doubts have been raised regarding the feasibility of evaporative cooling of metastable AEAs in magnetic traps. Here we present experimental data for 40Ca[4s4p]3 P2 clearly confirming the asserted multichannel character of the collision mechanism. While elastic cross sections are found to be similar to the predicted values, inelastic cross sections exceed the calculations by an order of magnitude. Our results substantiate the expectation of inefficient evaporative cooling.

Normal mode splitting and mechanical effects of an optical lattice in a ring cavity.

A novel regime of atom-cavity physics is explored, arising when large atom samples dispersively interact with high-finesse optical cavities. A stable far-detuned optical lattice of several million rubidium atoms is formed inside an optical ring resonator by coupling equal amounts of laser light to each propagation direction of a longitudinal cavity mode. An adjacent longitudinal mode, detuned by about 3 GHz, is used to perform probe transmission spectroscopy of the system. The atom-cavity coupling for the lattice beams and the probe is dispersive and dissipation results only from the finite photon-storage time. The observation of two well-resolved normal modes demonstrates the regime of strong cooperative coupling. The details of the normal mode spectrum reveal mechanical effects associated with the retroaction of the probe upon the optical lattice.