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Polymers (Basel) ; 16(7)2024 Apr 03.
Artigo em Inglês | MEDLINE | ID: mdl-38611234

RESUMO

The objective of this paper is to investigate the debonding behavior of the interface between continuously and discontinuously fiber reinforced thermoplastics using the climbing drum peel test. The study emphasizes on the importance of considering different climatic boundary conditions on the properties of thermoplastics. Specimens with varying moisture contents, from 0m.% up to above 6m.% are prepared and tested. It is observed that an increase in moisture content from 0m.% to 2m.% results in an increase of the fracture surface energy from 1.07·103J/m2 to 2.40·103J/m2 required to separate the two materials, but a further increase in moisture to 6.35m.% conversely results in a subsequent decrease of the required energy to 1.91·103J/m2. The study presents an explanatory model of increasing plasticization of the polymer due to increased polymer chain mobility, which results in more deformation energy being required to propagate the crack, which is corroborated in SEM investigations of the fracture surface. A further increase in humidity leads to polymer degradation due to hydrolysis, which explains the subsequent reduction of the fracture energy. The experimental set up is modeled numerically for the first time with cohesive surfaces, which could successfully reproduce the effective force-displacement curve in the experiment by varying the interface parameters in the model over an influence length, allowing the conclusion of a process induced variation in the interface properties over a specific consolidation length.

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