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1.
Phys Rev Lett ; 120(1): 013401, 2018 Jan 05.
Artigo em Inglês | MEDLINE | ID: mdl-29350943

RESUMO

Feshbach resonances, which allow for tuning the interactions of ultracold atoms with an external magnetic field, have been widely used to control the properties of quantum gases. We propose a scheme for using scattering resonances as a probe for external fields, showing that by carefully tuning the parameters it is possible to reach a 10^{-5} G (or nT) level of precision with a single pair of atoms. We show that, for our collisional setup, it is possible to saturate the quantum precision bound with a simple measurement protocol.

2.
Nat Commun ; 8: 14854, 2017 03 23.
Artigo em Inglês | MEDLINE | ID: mdl-28332492

RESUMO

Exploring and controlling inelastic and reactive collisions on the quantum level is a main goal of the developing field of ultracold chemistry. For this, the preparation of precisely defined initial atomic and molecular states in tailored environments is necessary. Here we present experimental studies of inelastic collisions of metastable ultracold Rb2 molecules in an array of quasi-1D potential tubes. In particular, we investigate collisions of molecules in the absolute lowest triplet energy level where any inelastic process requires a change of the electronic state. Remarkably, we find similar decay rates as for collisions between rotationally or vibrationally excited triplet molecules where other decay paths are also available. The decay rates are close to the ones for universal reactions but vary considerably when confinement and collision energy are changed. This might be exploited to control the collisional properties of molecules.

3.
Phys Rev Lett ; 112(25): 250502, 2014 Jun 27.
Artigo em Inglês | MEDLINE | ID: mdl-25014799

RESUMO

We propose a simple idea for realizing a quantum gate with two fermions in a double well trap via external optical pulses without addressing the atoms individually. The key components of the scheme are Feshbach resonance and Pauli blocking, which decouple unwanted states from the dynamics. As a physical example we study atoms in the presence of a magnetic Feshbach resonance in a nanoplasmonic trap and discuss the constraints on the operation times for realistic parameters, reaching a fidelity above 99.9% within 42 µs, much shorter than existing atomic gate schemes.

4.
Phys Rev Lett ; 110(21): 213202, 2013 May 24.
Artigo em Inglês | MEDLINE | ID: mdl-23745870

RESUMO

We develop a general quantum theory for reactive collisions involving power-law potentials (-1/r(n)) valid from the ultracold up to the high-temperature limit. Our quantum defect framework extends the conventional capture models to include the nonuniversal case when the short-range reaction probability P(re)<1. We present explicit analytical formulas as well as numerical studies for the van der Waals (n=6) and polarization (n=4) potentials. Our model agrees well with recent merged beam experiments on Penning ionization, spanning collision energies from 10 mK to 30 K [Henson et al., Science 338, 234 (2012)].

5.
Phys Chem Chem Phys ; 13(42): 19114-24, 2011 Nov 14.
Artigo em Inglês | MEDLINE | ID: mdl-21773648

RESUMO

Universal collision rate constants are calculated for ultracold collisions of two like bosonic or fermionic heteronuclear alkali-metal dimers involving the species Li, Na, K, Rb, or Cs. Universal collisions are those for which the short range probability of a reactive or quenching collision is unity such that a collision removes a pair of molecules from the sample. In this case, the collision rates are determined by universal quantum dynamics at very long range compared to the chemical bond length. We calculate the universal rate constants for reaction of the reactive dimers in their ground vibrational state v = 0 and for vibrational quenching of non-reactive dimers with v ≥ 1. Using the known dipole moments and estimated van der Waals coefficients of each species, we calculate electric field dependent loss rate constants for collisions of molecules tightly confined to quasi-two-dimensional geometry by a one-dimensional optical lattice. A simple scaling relation of the quasi-two-dimensional loss rate constants with dipole strength, trap frequency and collision energy is given for like bosons or like fermions. It should be possible to stabilize ultracold dimers of any of these species against destructive collisions by confining them in a lattice and orienting them with an electric field of less than 20 kV cm(-1).

6.
Phys Rev Lett ; 105(7): 073202, 2010 Aug 13.
Artigo em Inglês | MEDLINE | ID: mdl-20868041

RESUMO

Analytic expressions describe universal elastic and reactive rates of quasi-two-dimensional and quasi-one-dimensional collisions of highly reactive ultracold molecules interacting by a van der Waals potential. Exact and approximate calculations for the example species KRb show that stability and evaporative cooling can be realized for spin-polarized fermions at moderate dipole and trapping strength, whereas bosons or unlike fermions require significantly higher dipole or trapping strengths.

7.
Phys Rev Lett ; 104(11): 113202, 2010 Mar 19.
Artigo em Inglês | MEDLINE | ID: mdl-20366474

RESUMO

A simple quantum-defect model gives analytic expressions for the complex scattering length and threshold collision rates of ultracold molecules. If the probability of reaction in the short-range part of the collision is high, the model gives universal rate constants for s- and p-wave collisions that are independent of short-range dynamics. This model explains the magnitudes of the recently measured rate constants for collisions of two ultracold 40K87Rb molecules, or an ultracold 40K atom with the 40K87Rb molecule [S. Ospelkaus et al., Science 327, 853 (2010).

8.
Phys Rev Lett ; 96(1): 013201, 2006 Jan 13.
Artigo em Inglês | MEDLINE | ID: mdl-16486450

RESUMO

We present a zero-range pseudopotential applicable for all partial wave interactions between neutral atoms. For p and d waves, we derive effective pseudopotentials, which are useful for problems involving anisotropic external potentials. Finally, we consider two nontrivial applications of the p-wave pseudopotential: we solve analytically the problem of two interacting spin-polarized fermions confined in a harmonic trap, and we analyze the scattering of p-wave interacting particles in a quasi-two-dimensional system.

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