Intracavity optical trapping of microscopic particles in a ring-cavity fiber laser.

Standard optical tweezers rely on optical forces arising when a focused laser beam interacts with a microscopic particle: scattering forces, pushing the particle along the beam direction, and gradient forces, attracting it towards the high-intensity focal spot. Importantly, the incoming laser beam is not affected by the particle position because the particle is outside the laser cavity. Here, we demonstrate that intracavity nonlinear feedback forces emerge when the particle is placed inside the optical cavity, resulting in orders-of-magnitude higher confinement along the three axes per unit laser intensity on the sample. This scheme allows trapping at very low numerical apertures and reduces the laser intensity to which the particle is exposed by two orders of magnitude compared to a standard 3D optical tweezers. These results are highly relevant for many applications requiring manipulation of samples that are subject to photodamage, such as in biophysics and nanosciences.

Breaking crosstalk limits to dynamic holography using orthogonality of high-dimensional random vectors.

Holography is the most promising route to true-to-life 3D projections, but the incorporation of complex images with full depth control remains elusive. Digitally synthesised holograms1-7, which do not require real objects to create a hologram, offer the possibility of dynamic projection of 3D video8,9. Extensive efforts aimed 3D holographic projection10-17, however available methods remain limited to creating images on a few planes10-12, over a narrow depth-of-field13,14 or with low resolution15-17. Truly 3D holography also requires full depth control and dynamic projection capabilities, which are hampered by high crosstalk9,18. The fundamental difficulty is in storing all the information necessary to depict a complex 3D image in the 2D form of a hologram without letting projections at different depths contaminate each other. Here, we solve this problem by preshaping the wavefronts to locally reduce Fresnel diffraction to Fourier holography, which allows inclusion of random phase for each depth without altering image projection at that particular depth, but eliminates crosstalk due to near-orthogonality of large-dimensional random vectors. We demonstrate Fresnel holograms that form on-axis with full depth control without any crosstalk, producing large-volume, high-density, dynamic 3D projections with 1000 image planes simultaneously, improving the state-of-the-art12,17 for number of simultaneously created planes by two orders of magnitude. While our proof-of-principle experiments use spatial light modulators, our solution is applicable to all types of holographic media.

NLL-Assisted Multilayer Graphene Patterning.

The range of applications of diverse graphene-based devices could be limited by insufficient surface reactivity, unsatisfied shaping, or null energy gap of graphene. Engineering the graphene structure by laser techniques can adjust the transport properties and the surface area of graphene, providing devices of different nature with a higher capacitance. Additionally, the created periodic potential and appearance of the active external/inner/edge surface centers determine the multifunctionality of the graphene surface and corresponding devices. Here, we report on the first implementation of nonlinear laser lithography (NLL) for multilayer graphene (MLG) structuring, which offers a low-cost, single-step, and high-speed nanofabrication process. The NLL relies on the employment of a high repetition rate femtosecond Yb fiber laser that provides generation of highly reproducible, robust, uniform, and periodic nanostructures over a large surface area (1 cm2/15 s). NLL allows one to obtain clearly predesigned patterned graphene structures without fabrication tolerances, which are caused by contacting mask contamination, polymer residuals, and direct laser exposure of the graphene layers. We represent regularly patterned MLG (p-MLG) obtained by the chemical vapor deposition method on an NLL-structured Ni foil. We also demonstrate tuning of chemical (wettability) and electro-optical (transmittance and sheet resistance) properties of p-MLG by laser power adjustments. In conclusion, we show the great promise of fabricated devices, namely, supercapacitors, and Li-ion batteries by using NLL-assisted graphene patterning. Our approach demonstrates a new avenue to pattern graphene for multifunctional device engineering in optics, photonics, and bioelectronics.

High-power Yb-based all-fiber laser delivering 300 fs pulses for high-speed ablation-cooled material removal.

We report on a 72 W Yb all-fiber ultrafast laser system with 1.6 GHz intra-burst and 200 kHz burst repetition rate developed to demonstrate ablation-cooled material removal at high speeds. Up to 24 W is applied on Cu and Si samples with pulses of ∼300 fs, and record-high ablation efficiencies are obtained, compared to published results to date, despite using only ∼100 nJ pulses. Ablation speeds approaching 1 mm3/s are reported with 24 W of average power, limited by available laser power and beam scanning speed. More significantly, these results experimentally confirm the theoretically expected linear scaling of the ablation-cooled regime to higher average powers without sacrificing efficiency, which implies that further scaling is possible with further increases in laser power and scanning speeds.

In-chip microstructures and photonic devices fabricated by nonlinear laser lithography deep inside silicon.

Silicon is an excellent material for microelectronics and integrated photonics1-3 with untapped potential for mid-IR optics4. Despite broad recognition of the importance of the third dimension5,6, current lithography methods do not allow fabrication of photonic devices and functional microelements directly inside silicon chips. Even relatively simple curved geometries cannot be realised with techniques like reactive ion etching. Embedded optical elements, like in glass7, electronic devices, and better electronic-photonic integration are lacking8. Here, we demonstrate laser-based fabrication of complex 3D structures deep inside silicon using 1 µm-sized dots and rod-like structures of adjustable length as basic building blocks. The laser-modified Si has a different optical index than unmodified parts, which enables numerous photonic devices. Optionally, these parts are chemically etched to produce desired 3D shapes. We exemplify a plethora of subsurface, i.e., "in-chip" microstructures for microfluidic cooling of chips, vias, MEMS, photovoltaic applications and photonic devices that match or surpass the corresponding state-of-the-art device performances.

Rich complex behaviour of self-assembled nanoparticles far from equilibrium.

A profoundly fundamental question at the interface between physics and biology remains open: what are the minimum requirements for emergence of complex behaviour from nonliving systems? Here, we address this question and report complex behaviour of tens to thousands of colloidal nanoparticles in a system designed to be as plain as possible: the system is driven far from equilibrium by ultrafast laser pulses that create spatiotemporal temperature gradients, inducing Marangoni flow that drags particles towards aggregation; strong Brownian motion, used as source of fluctuations, opposes aggregation. Nonlinear feedback mechanisms naturally arise between flow, aggregate and Brownian motion, allowing fast external control with minimal intervention. Consequently, complex behaviour, analogous to those seen in living organisms, emerges, whereby aggregates can self-sustain, self-regulate, self-replicate, self-heal and can be transferred from one location to another, all within seconds. Aggregates can comprise only one pattern or bifurcated patterns can coexist, compete, endure or perish.

Nonlinearity-tailored fiber laser technology for low-noise, ultra-wideband tunable femtosecond light generation.

The emission wavelength of a laser is physically predetermined by the gain medium used. Consequently, arbitrary wavelength generation is a fundamental challenge in the science of light. Present solutions include optical parametric generation, requiring complex optical setups and spectrally sliced supercontinuum, taking advantage of a simpler fiber technology: a fixed-wavelength pump laser pulse is converted into a spectrally very broadband output, from which the required resulting wavelength is then optically filtered. Unfortunately, this process is associated with an inherently poor noise figure, which often precludes many realistic applications of such super-continuum sources. Here, we show that by adding only one passive optical element-a tapered photonic crystal fiber-to a fixed-wavelength femtosecond laser, one can in a very simple manner resonantly convert the laser emission wavelength into an ultra-wide and continuous range of desired wavelengths, with very low inherent noise, and without mechanical realignment of the laser. This is achieved by exploiting the double interplay of nonlinearity and chirp in the laser source and chirp and phase matching in the tapered fiber. As a first demonstration of this simple and inexpensive technology, we present a femtosecond fiber laser continuously tunable across the entire red-green-blue spectral range.

Multiscale Self-Assembly of Silicon Quantum Dots into an Anisotropic Three-Dimensional Random Network.

Multiscale self-assembly is ubiquitous in nature but its deliberate use to synthesize multifunctional three-dimensional materials remains rare, partly due to the notoriously difficult problem of controlling topology from atomic to macroscopic scales to obtain intended material properties. Here, we propose a simple, modular, noncolloidal methodology that is based on exploiting universality in stochastic growth dynamics and driving the growth process under far-from-equilibrium conditions toward a preplanned structure. As proof of principle, we demonstrate a confined-but-connected solid structure, comprising an anisotropic random network of silicon quantum-dots that hierarchically self-assembles from the atomic to the microscopic scales. First, quantum-dots form to subsequently interconnect without inflating their diameters to form a random network, and this network then grows in a preferential direction to form undulated and branching nanowire-like structures. This specific topology simultaneously achieves two scale-dependent features, which were previously thought to be mutually exclusive: good electrical conduction on the microscale and a bandgap tunable over a range of energies on the nanoscale.

Focus issue introduction: Advanced Solid-State Lasers (ASSL) 2015.

The editors introduce the focus issue on "Advanced Solid-State Lasers (ASSL) 2015", which is based on the topics presented at a congress of the same name held in Berlin, Germany, from October 4 to October 9, 2015. This focus issue, jointly prepared by Optics Express and Optical Materials Express, includes 23 contributed papers (17 for Optics Express and 6 for Optical Materials Express) selected from the voluntary submissions from attendees who presented at the congress and have extended their work into complete research articles. We hope this focus issue offers a good snapshot of a variety of topical discussions held at the congress and will contribute to the further expansion of the associated research areas.

Focus issue introduction: Advanced solid-state lasers (ASSL) 2014.

The editors introduce the focus issue on "Advanced Solid-State Lasers (ASSL) 2014," which is based on the topics presented at a congress of the same name held in Shanghai, China, from October 27 to November 1, 2014. This focus issue, jointly prepared by Optics Express and Optical Materials Express, includes 28 contributed papers (21 for Optics Express and 7 for Optical Materials Express) selected from the voluntary submissions by attendees who presented at the congress and have extended their work into complete research articles. We hope this focus issue offers a useful snapshot of the variety of topical discussions held at the congress and will contribute to the further expansion of the associated research areas.

High-power high-repetition-rate single-mode Er-Yb-doped fiber laser system.

We demonstrate an all-fiber-integrated, high-power chirped-pulse-amplification system operating at 1550 nm. The seed source is a soliton fiber laser with 156 MHz repetition rate. Two-stage single mode amplifier provides an amplification of more than 40 dB without significant spontaneous amplified emission. The power amplifier is based on cladding-pumped 10 µm-core Er-Yb co-doped fiber, the output of which was spliced into standard singlemode fiber. We obtain 10 W average power in a strictly singlemode operation. After dechirping with a grating compressor, near transform-limited, 450 fs-long pulses are obtained. The laser source exhibits excellent short and long-term intensity stability, with relative intensity noise measurements characterizing the short-term stability.

Fiber laser-microscope system for femtosecond photodisruption of biological samples.

We report on the development of a ultrafast fiber laser-microscope system for femtosecond photodisruption of biological targets. A mode-locked Yb-fiber laser oscillator generates few-nJ pulses at 32.7 MHz repetition rate, amplified up to ∼125 nJ at 1030 nm. Following dechirping in a grating compressor, ∼240 fs-long pulses are delivered to the sample through a diffraction-limited microscope, which allows real-time imaging and control. The laser can generate arbitrary pulse patterns, formed by two acousto-optic modulators (AOM) controlled by a custom-developed field-programmable gate array (FPGA) controller. This capability opens the route to fine optimization of the ablation processes and management of thermal effects. Sample position, exposure time and imaging are all computerized. The capability of the system to perform femtosecond photodisruption is demonstrated through experiments on tissue and individual cells.

83 W, 3.1 MHz, square-shaped, 1 ns-pulsed all-fiber-integrated laser for micromachining.

We demonstrate an all-fiber-integrated laser based on off-the-shelf components producing square-shaped, 1 ns-long pulses at 1.03 µm wavelength with 3.1 MHz repetition rate and 83 W of average power. The master-oscillator power-amplifier system is seeded by a fiber oscillator utilizing a nonlinear optical loop mirror and producing incompressible pulses. A simple technique is employed to demonstrate that the pulses indeed have a random chirp. We propose that the long pulse duration should result in more efficient material removal relative to picosecond pulses, while being short enough to minimize heat effects, relative to nanosecond pulses commonly used in micromachining. Micromachining of Ti surfaces using 0.1 ns, 1 ns and 100 ns pulses supports these expectations.

Texturing of titanium (Ti6Al4V) medical implant surfaces with MHz-repetition-rate femtosecond and picosecond Yb-doped fiber lasers.

We propose and demonstrate the use of short pulsed fiber lasers in surface texturing using MHz-repetition-rate, microjoule- and sub-microjoule-energy pulses. Texturing of titanium-based (Ti6Al4V) dental implant surfaces is achieved using femtosecond, picosecond and (for comparison) nanosecond pulses with the aim of controlling attachment of human cells onto the surface. Femtosecond and picosecond pulses yield similar results in the creation of micron-scale textures with greatly reduced or no thermal heat effects, whereas nanosecond pulses result in strong thermal effects. Various surface textures are created with excellent uniformity and repeatability on a desired portion of the surface. The effects of the surface texturing on the attachment and proliferation of cells are characterized under cell culture conditions. Our data indicate that picosecond-pulsed laser modification can be utilized effectively in low-cost laser surface engineering of medical implants, where different areas on the surface can be made cell-attachment friendly or hostile through the use of different patterns.

Demonstration of a cavity-enhanced optical parametric chirped-pulse amplification system.

The use of a low finesse enhancement cavity resonant with a low average power (<1 W) and a high repetition rate (78 MHz) pump source is shown to achieve 55% conversion efficiency into signal and idler from the coupled pump in an optical parametric process, whereas an equivalent amount of pump power in a single-pass configuration leads to negligible conversion. Careful comparison of the intracavity conversion process to the single-pass case is performed to assess the underlying impedance matching that yields the high conversion results.

Generation of 287 W, 5.5 ps pulses at 78 MHz repetition rate from a cryogenically cooled Yb:YAG amplifier seeded by a fiber chirped-pulse amplification system.

We generate linearly polarized, 287 W average-power, 5.5 ps pulses using a cryogenically cooled Yb:YAG amplifier at a repetition rate of 78 MHz. An optical-to-optical efficiency of 41% is obtained at 700 W pump power. A 6 W, 0.4 nm bandwidth picosecond seed source at 1029 nm wavelength is constructed using a chirped-pulse fiber amplification chain based on chirped volume Bragg gratings. The combination of a fiber amplifier system and a cryogenically cooled Yb:YAG amplifier results in good spatial beam quality at large average power. Low nonlinear phase accumulation as small as 5.1 x 10(-3) rad in the bulk Yb:YAG amplifier supports power scalability to a > 10 kW level without being affected by self-phase modulation. This amplification system is well suited for pumping high-power high-repetition-rate optical parametric chirped-pulse amplifiers.