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2.
Environ Sci Pollut Res Int ; 23(17): 17095-104, 2016 Sep.
Artigo em Inglês | MEDLINE | ID: mdl-27211094

RESUMO

In early April 2011, radiostrontium was accidentally released from the Fukushima Daiichi Nuclear Power Plant to the Pacific coast of eastern Japan. We developed a simple procedure to analyze radiostrontium levels in marine mussels (Septifer virgatus) and seawater using crown ether (Sr Resin; Eichrom). Then, we used our method to describe the spatial and temporal distribution of radiostrontium in mussels and seawater on the Pacific coast of eastern Japan from 2011 to 2013 and for 2015. Activity of (90)Sr in mussels and seawater decreased with distance from the Fukushima Daiichi Nuclear Power Plant and between 2011 and 2013 tended to be higher in areas south of the Fukushima Daiichi Nuclear Power Plant than to the north of it. Activity in mussels and seawater also tended to decrease from 2011 to 2013 and by 2015 had reached levels experienced prior to the Fukushima accident. Our results suggest that radiostrontium discharged from the Fukushima Daiichi Nuclear Power Plant was dispersed by coastal currents in a southerly direction along the Pacific coast of eastern Japan from 2011 to 2013, following which its activity decreased to background levels by 2015.


Assuntos
Bivalves/química , Acidente Nuclear de Fukushima , Monitoramento de Radiação , Radioisótopos de Estrôncio/análise , Poluentes Radioativos da Água/análise , Animais , Japão , Oceano Pacífico , Água do Mar
3.
Nature ; 416(6877): 163-5, 2002 Mar 14.
Artigo em Inglês | MEDLINE | ID: mdl-11894090

RESUMO

Methyl chloride is the largest natural source of ozone-depleting chlorine compounds, and accounts for about 15 per cent of the present atmospheric chlorine content. This contribution was likely to have been relatively greater in pre-industrial times, when additional anthropogenic sources-such as chlorofluorocarbons-were absent. Although it has been shown that there are large emissions of methyl chloride from coastal lands in the tropics, there remains a substantial shortfall in the overall methyl chloride budget. Here we present observations of large emissions of methyl chloride from some common tropical plants (certain types of ferns and Dipterocarpaceae), ranging from 0.1 to 3.7 microg per gram of dry leaf per hour. On the basis of these preliminary measurements, the methyl chloride flux from Dipterocarpaceae in southeast Asia alone is estimated at 0.91 Tg yr-1, which could explain a large portion of missing methyl chloride sources. With continuing tropical deforestation, natural sources of chlorine compounds may accordingly decrease in the future. Conversely, the abundance of massive ferns in the Carboniferous period may have created an atmosphere rich in methyl chloride.


Assuntos
Atmosfera/química , Cloreto de Metila/metabolismo , Plantas/metabolismo , Clima Tropical , Sudeste Asiático , Biomassa , Cloro/análise , Gleiquênias/metabolismo , Magnoliopsida/metabolismo , Óxidos de Enxofre/metabolismo , Árvores/metabolismo
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