Radioactivity concentration levels and potential radiotoxicity risk assessment of aquatic superfoods case study of algae supplements.

It has been found that algae have a variety of health benefits, although investigations showed that they contain radiotoxic elements, including 226Ra, 232Th, 40K, and 137Cs, which may affect human health. This study is connected to activity concentration measurements of the above radionuclides in the algae supplements available in the Middle East markets. The annual effective radiation doses of measured radionuclides in analyzed algal supplements have been calculated. The highest values of annual effective doses have been estimated for 226Ra in Ecklonia (13.39 µSv/y) and for 232Th in Red Marine Algae (11.80 µSv/y), both from South Korea. In algal "superfoods", the effective dose of 137Cs is not significantly affected by the Fukushima Nuclear Power Plant. Based on these results, it can be concluded that the activity levels of radionuclides are low, the naturally occurring radionuclides provide the most effective doses, and algae supplements can be considered safe.

Nuclear power plant biological complications on marine biota from a probabilistic accident - A case study.

An accident at the Barakah Nuclear Power Plant (BNPP) would result in a significant radionuclide release into the semi-closed marine environment. In this research, the released radionuclide distribution pattern and dose rate in the Persian/Arabian (Gulf) were calculated using a combined hydrodynamic/radiobiological model. Simulations of the dispersion of artificial radionuclide concentrations were conducted using a HYSPLIT model. To assess prospective hazards in case of an incident, environmental risk from ionizing contaminants: assessment and management (ERICA) tools were used. Using the Fukushima nuclear power accident as a model, the scenario source term profile was developed. The volumetric concentrations levels of pollutants ranged between 1 × 104 mBq m-3 to 1 × 1010 mBq m-3 in the radius of 200 km after 48 h. Based on the dose rates of the various marine biotas, Polychaete worms, and Pelagic fish, they had the highest and lowest dose contribution.

Tungsten (VI) oxide reinforced antimony glasses for radiation safety applications: A throughout investigation for determination of radiation shielding properties and transmission factors.

We report the functional assessment of tungsten (VI) oxide on gamma-ray attenuation properties of 60Sb2O3-(40-x)NaPO3-xWO3 antimony glasses. The elemental mass-fractions and glass-densities of each glass sample are specified separately for the MCNPX Monte Carlo code. In addition to fundamental gamma absorption properties, Transmission Factors throughout a broad radioisotope energy range were measured. According to findings, holmium (Ho) incorporation into the glass structure resulted in a net increase of 0.3406 g/cm3, whereas cerium (Ce) addition resulted in a net increase of 0.2047 g/cm3. The 40% WO3 reinforced S7 sample was found to have the greatest LAC value, even though seven glass samples exhibited identical behavior. The S2 sample had the lowest HVL values among the glass groups evaluated in this work, computed in the energy range of 0.015-15 MeV. The lowest EBF and EABF values were reported for 40% WO3 reinforced S7 sample with the highest LAC and density values. According to the findings of this research, WO3 will likely make a significant contribution to the gamma ray absorption properties of antimony glasses, which are employed for optical and structural modification. Therefore, it can be concluded that WO3 may be treated monotonically and can be employed successfully in circumstances where gamma-ray absorption characteristics, optical properties, and structural qualities need to be enhanced.

Exploring the Potential of Zirconium-89 in Diagnostic Radiopharmaceutical Applications: An Analytical Investigation.

This study highlights the use of 89Zr-oxalate in diagnostic applications with the help of WinAct and IDAC2.1 software. It presents the biodistribution of the drug in various organs and tissues, including bone, blood, muscle, liver, lung, spleen, kidneys, inflammations, and tumors, and analyzes the maximum amount of nuclear transformation per Bq intake for each organ. The retention time of the maximum nuclear transformation and the absorbed doses of the drug in various organs and tissues are also examined. Data from clinical and laboratory studies on radiopharmaceuticals are used to estimate the coefficients of transition. The accumulation and excretion of the radiopharmaceutical in the organs is assumed to follow an exponential law. The coefficients of transition from the organs to the blood and vice versa are estimated using a combination of statistical programs and digitized data from the literature. WinAct and IDAC 2.1 software are used to calculate the distribution of the radiopharmaceutical in the human body and to estimate the absorbed doses in organs and tissues. The results of this study can provide valuable information for the biokinetic modeling of wide-spectrum diagnostic radiopharmaceuticals. The results show that 89Zr-oxalate has a high affinity for bones and a relatively low impact on healthy organs, making it helpful in targeting bone metastases. This study provides valuable information for further research on the development of this drug for potential clinical applications.

Lead-Free Ternary Glass for Radiation Protection: Composition and Performance Evaluation for Solar Cell Coverage.

Solar cells in superstrate arrangement need a protective cover glass as one of its main components. The effectiveness of these cells is determined by the cover glass's low weight, radiation resistance, optical clarity, and structural integrity. Damage to the cell covers brought on by exposure to UV irradiation and energetic radiation is thought to be the root cause of the ongoing issue of a reduction in the amount of electricity that can be generated by solar panels installed on spacecraft. Lead-free glasses made of xBi2O3-(40 - x)CaO-60P2O5 (x = 5, 10, 15, 20, 25, and 30 mol%) were created using the usual approach of melting at a high temperature. The amorphous nature of the glass samples was confirmed using X-ray diffraction. At energies of 81, 238, 356, 662, 911, 1173, 1332, and 2614 keV, the impact of various chemical compositions on gamma shielding in a phospho-bismuth glass structure was measured. The evaluation of gamma shielding revealed that the results of the mass attenuation coefficient of glasses increase as the Bi2O3 content increases but decrease as the photon energy increases. As a result of the study conducted on the radiation-deflecting properties of ternary glass, a lead-free low-melting phosphate glass that exhibited outstanding overall performance was developed, and the optimal composition of a glass sample was identified. The 60P2O5-30Bi2O3-10CaO glass combination is a viable option for use in radiation shielding that does not include lead.

Production of Hybrid Nanocomposites Based on Iron Waste Reinforced with Niobium Carbide/Granite Nanoparticles with Outstanding Strength and Wear Resistance for Use in Industrial Applications.

The main objective of this work is to recycle unwanted industrial waste in order to produce innovative nanocomposites with improved mechanical, tribological, and thermal properties for use in various industrial purposes. In this context, powder metallurgy (PM) technique was used to fabricate iron (Fe)/copper (Cu)/niobium carbide (NbC)/granite nanocomposites having outstanding mechanical, wear and thermal properties. Transmission electron microscopy (TEM) and X-ray diffraction (XRD) examinations were used to investigate the particle size, crystal size, and phase composition of the milled samples. Additionally, it was investigated how different volume percentages of the NbC and granite affected the sintered specimens in terms of density, microstructure, mechanical and wear properties, and coefficient of thermal expansion (CTE). According to the findings, the milled powders included particles that were around 55 nm in size and clearly contained agglomerates. The results showed that the addition of 4 vol.% NbC and 8 vol.% granite nanoparticles caused a reduction in the Fe-Cu alloy matrix particle sizes up to 47.8 nm and served as a barrier to the migration of dislocations. In addition, the successive increase in the hybrid concentrations led to a significant decrease in the crystal size of the samples prepared as follows: 29.73, 27.58, 22.69, 19.95 and 15.8 nm. Furthermore, compared with the base Fe-Cu alloy, the nanocomposite having 12 vol.% of hybrid reinforcement demonstrated a significant improvement in the microhardness, ultimate strength, Young's modulus, longitudinal modulus, shear modulus, bulk modulus, CTE and wear rate by 94.3, 96.4, 61.1, 78.2, 57.1, 73.6, 25.6 and 61.9%, respectively. This indicates that both NbC and granite can actually act as excellent reinforcements in the Fe alloy.

A closer look at the efficiency calibration of LaBr3(Ce) and NaI(Tl) scintillation detectors using MCNPX for various types of nuclear investigations.

The nuclear spectroscopy method has long been used for advanced studies on nuclear physics. In order to decrease costs and increase the efficiency of nuclear radiation investigations, quick and efficient solutions are required. The purpose of this research was to calculate the whole energy peak efficiency values for a range of gamma-ray energies, from 30.973 keV to 1408 keV, at various source-detector distances using the MCNPX Monte Carlo code, which is extensively used in nuclear medicine, industry, and scientific research. As a result, the modeled detectors' full-energy peak efficiencies were calculated and compared to both experimental data and Monte Carlo simulations. Experiment results and prior studies using Monte Carlo simulations were found to be very consistent with these results. The counting efficiency against source-detector distance is then calculated using the modeled detectors. The data we have show that LaBr3(Ce) has outstanding detection properties. This study's findings might be used to improve the design of detectors for use in wide range of high-tech gamma spectroscopy and nuclear research applications.

Structure, Mössbauer, electrical, and γ-ray attenuation-properties of magnesium zinc ferrite synthesized co-precipitation method.

For technical and radioprotection causes, it has become essential to find new trends of smart materials which used as protection from ionizing radiation. To overcome the undesirable properties in lead aprons and provide the proper or better shielding properties against ionizing radiation, the tendency is now going to use ferrite as a shielding material. The co-precipitation method was utilized to prevent any foreign phases in the investigated MZN nano-ferrite. X-ray diffraction (XRD) and Fourier transmission infrared spectroscopy (FTIR) methods were used to analyze the manufactured sample. As proven by XRD and FTIR, the studied materials have their unique spinel phase with cubic structure Fd3m space group. The DC resistivity of Mg-Zn ferrite was carried out in the temperature range (77-295 K), and its dependence on temperature indicates that there are different charge transport mechanisms. The Mössbauer spectra analysis confirmed that the ferrimagnetic to superparamagnetic phase transition behaviour depends on Zn concentration. The incorporation of Zn to MZF enhanced the nano-ferrite density, whereas the addition of different Zn-oxides reduced the density for nano-ferrite samples. This variation in density changed the radiation shielding results. The sample containing high Zn (MZF-0.5) gives us better results in radiation shielding properties at low gamma, so this sample is superior in shielding results for charged particles at low energy. Finally, the possibility to use MZN nano-ferrite with various content in different ionizing radiation shielding fields can be concluded.

Distribution of Radionuclides and Radiological Health Assessment in Seih-Sidri Area, Southwestern Sinai.

The current contribution goal is to measure the distribution of the radionuclide within the exposed rock units of southwestern Sinai, Seih-Sidri area, and assess the radiological risk. Gneisses, older granites, younger gabbro, younger granites, and post granitic dikes (pegmatites) are the main rock units copout in the target area. Radioactivity, as well as radiological implications, were investigated for forty-three samples from gneisses (seven hornblende biotite gneiss and seven biotite gneiss), older granites (fourteen samples), and younger granites (fifteen samples of syenogranites) using NaI (Tl) scintillation detector. External and internal hazard index (Hex, Hin), internal and external level indices (Iα, Iγ), absorbed dose rates in the air (D), the annual effective dose equivalent (AED), radium equivalent activity (Raeq), annual gonadal dose (AGDE), excess lifetime cancer risk (ELCR), and the value of Upper Continental Core 232Th/238U mass fractions were determined from the obtained values of 238U, 232Th and 40K for the examined rocks of Seih-Sidri area. The average 238U mg/kg in hornblende biotite gneiss and biotite gneiss, older granites, and syenogranites is 2.3, 2.1, 2.7, and 8.4 mg/kg, respectively, reflecting a relatively higher concentration of uranium content in syenogranites. The results suggest that using these materials may pose risks to one's radiological health.

Utilization of artificial intelligence approach for prediction of DLP values for abdominal CT scans: A high accuracy estimation for risk assessment.

Purpose: This study aimed to evaluate Artificial Neural Network (ANN) modeling to estimate the significant dose length product (DLP) value during the abdominal CT examinations for quality assurance in a retrospective, cross-sectional study. Methods: The structure of the ANN model was designed considering various input parameters, namely patient weight, patient size, body mass index, mean CTDI volume, scanning length, kVp, mAs, exposure time per rotation, and pitch factor. The aforementioned examination details of 551 abdominal CT scans were used as retrospective data. Different types of learning algorithms such as Levenberg-Marquardt, Bayesian and Scaled-Conjugate Gradient were checked in terms of the accuracy of the training data. Results: The R-value representing the correlation coefficient for the real system and system output is given as 0.925, 0.785, and 0.854 for the Levenberg-Marquardt, Bayesian, and Scaled-Conjugate Gradient algorithms, respectively. The findings showed that the Levenberg-Marquardt algorithm comprehensively detects DLP values for abdominal CT examinations. It can be a helpful approach to simplify CT quality assurance. Conclusion: It can be concluded that outcomes of this novel artificial intelligence method can be used for high accuracy DLP estimations before the abdominal CT examinations, where the radiation-related risk factors are high or risk evaluation of multiple CT scans is needed for patients in terms of ALARA. Likewise, it can be concluded that artificial learning methods are powerful tools and can be used for different types of radiation-related risk assessments for quality assurance in diagnostic radiology.

Adsorption Study of Congo Red Dye from Synthetic Wastewater at Different Concentrations Using Zinc Sulfide Nanoparticles.

Zinc sulfide (ZnS) nanoparticles were fabricated using the chemical precipitation method. The X-ray diffraction (XRD), Raman spectroscopy, and scanning electron microscopy (SEM) techniques were used to investigate the structural parameters of the formed ZnS. The hexagonal crystal structure of the Zn and ZnS phases was formed. The average crystallite size of the ZnS phase is 10.3 nm, which is much smaller than that of the Zn phase (54.5 nm). Several frequencies and phonon modes were detected in the Raman scattering spectrum belonging to the ZnS nanoparticles. The synthesized ZnS nanoparticles were used as catalysts to eliminate the Congo red (CR) dye, with different concentrations, from synthetic wastewater. The impact of the CR dye concentration and shaking period on the adsorption of CR was thoroughly investigated, and various adsorption kinetic models were tested. After 3 h of shaking, the adsorption efficiency reached 26.01% for 40 mg/L CR dye and 27.84% for 20 mg/L CR dye. The adsorption capacities of the CR dye in the presence of ZnS are 16% and 9% for 40 and 20 mg/L, respectively. Based on the correlation factor, the intraparticle diffusion kinetic model was considered the best of the tested models.

An In-Depth Examination of the Natural Radiation and Radioactive Dangers Associated with Regularly Used Medicinal Herbs.

The specific activity of U-238 and Th-232, as well as K-40 radionuclides, in twenty-nine investigated medicinal herbs used in Egypt has been measured using a high-purity germanium (HP Ge) detector. The measured values ranged from the BDL to 20.71 ± 1.52 with a mean of 7.25 ± 0.54 (Bq kg-1) for uranium-238, from the BDL to 29.35 ± 1.33 with a mean of 7.78 ± 0.633 (Bq kg-1) for thorium-232, and from 172 ± 5.85 to 1181.2 ± 25.5 with a mean of 471.4 ± 11.33 (Bq kg-1) for potassium-40. Individual herbs with the highest activity levels were found to be 20.71 ± 1.52 (Bq kg-1) for uranium-238 (H4, Thyme herb), 29.35 ± 1.33 (Bq kg-1) for thorium-232 (H20, Cinnamon), and 1181.2 ± 25.5 (Bq kg-1) for potassium-40 (H24, Worm-wood). (AACED) Ingestion-related effective doses over the course of a year of uranium-238 and thorium-232, as well as potassium-40 estimated from measured activity concentrations, are 0.002304 ± 0.00009 (minimum), 0.50869 ± 0.0002 (maximum), and 0.0373 ± 0.0004 (average)(mSv/yr). Radium equivalent activity (Raeq), annual gonadal dose equivalent (AGDE), absorbed gamma dose rate (Doutdoor, Dindoor), gamma representative level index (I), annual effective dose (AEDtotal), external and internal hazard index (Hex, Hin), and excess lifetime cancer risk were determined in medicinal plants (ELCR). The radiological hazards assessment revealed that the investigated plant species have natural radioactivity levels that are well within the internationally recommended limit. This is the first time that the natural radioactivity of therapeutic plants has been measured in Egypt. In addition, no artificial radionuclide (for example, 137Cs) was discovered in any of the samples. Therefore, the current findings are intended to serve as the foundation for establishing a standard safety and guideline for using these therapeutic plants in Egypt.

A Comprehensive Evaluation of the Attenuation Characteristics of Some Sliding Bearing Alloys under 0.015-15 MeV Gamma-Ray Exposure.

In this study, three different sliding bearing alloy samples were investigated in terms of their performance on attenuation characteristics and behavioral attitudes under 0.015-15 MeV gamma-ray exposure. Accordingly, different types of advanced calculation methods were utilized to calculate the radiation shielding parameters. Next, several gamma-ray shielding parameters and exposure rates in addition to fast neutron removal cross-section were determined. Furthermore, exposure and energy absorption buildup factors were determined by using G-P fitting method. Mass attenuation coefficients (MAC) values were recorded as 2.5246, 2.5703, and 2.5827 (cm2/g) for Alloy1, Alloy2, and Alloy3 samples at 15 MeV photon energy, respectively. At 40 mfp, the highest EBF values were reported as 1,376,274, 1,003,593, and 969,373 for Alloy1, Alloy2, and Alloy3 samples. The results of this extended investigation showed that the Alloy3 sample with the highest Pb reinforcement amount has superior shielding capability among the investigated samples. It can be concluded from the results that substitution of Pb with Bi in the recent alloy structure has a monotonic effect on different types of shielding parameters. Therefore, it can also be concluded that Pb is a remarkable tool for the improvement of the shielding properties of studied alloy structures.

Enhancement of Gamma-ray Shielding Properties in Cobalt-Doped Heavy Metal Borate Glasses: The Role of Lanthanum Oxide Reinforcement.

The direct influence of La3+ ions on the gamma-ray shielding properties of cobalt-doped heavy metal borate glasses with the chemical formula 0.3CoO-(80-x)B2O3-19.7PbO-xLa2O3: x = 0, 0.5, 1, 1.5, and 2 mol% was examined herein. Several significant radiation shielding parameters were evaluated. The glass density was increased from 3.11 to 3.36 g/cm3 with increasing La3+ ion content from 0 to 2 mol%. The S5 glass sample, which contained the highest concentration of La3+ ions (2 mol%), had the maximum linear (µ) and mass (µm) attenuation coefficients for all photon energies entering, while the S1 glass sample free of La3+ ions possessed the minimum values of µ and µm. Both the half value layer (T1/2) and tenth value layer (TVL) of all investigated glasses showed a similar trend of (T1/2, TVL)S1 > (T1/2, TVL)S2 > (T1/2, TVL)S3 > (T1/2, TVL)S4 > (T1/2, TVL)S5. Our results revealed that the S5 sample had the highest effective atomic number (Zeff) values over the whole range of gamma-ray energy. S5 had the lowest exposure (EBF) and energy absorption (EABF) build-up factor values across the whole photon energy and penetration depth range. Our findings give a strong indication of the S5 sample's superior gamma-ray shielding characteristics due to the highest contribution of lanthanum oxide.

Impact of Eye and Breast Shielding on Organ Doses During Cervical Spine Radiography: Design and Validation of MIRD Computational Phantom.

Purpose: The study aimed to design and validate computational phantoms (MIRD) using the MCNPX code to assess the impact of shielding on organ doses. Method: To validate the optimized phantom, the obtained results were compared with experimental results. The validation of the optimized MIRD phantom was provided by using the results of a previous anthropomorphic phantom study. MIRD phantom was designed by considering the parameters used in the anthropomorphic phantom study. A test simulation was performed to compare the dose reduction percentages (%) between the experimental anthropomorphic phantom study and the MCNPX-MIRD phantom. The simulation was performed twice, with and without shielding materials, using the same number and locations of the detector. Results: The absorbed dose amounts were directly extracted from the required organ and tissue cell parts of output files. Dose reduction percentages between the simulation with shielding and simulation without shielding were compared. The highest dose reduction was noted in the thymus (95%) and breasts (88%). The obtained dose reduction percentages between the anthropomorphic phantom study and the MCNPX-MIRD phantom were highly consistent and correlated values with experimental anthropomorphic data. Both methods showed Relative Difference (%) ranges between 0.88 and 2.22. Moreover, the MCNPX-MIRD optimized phantom provides detailed dose analysis for target and non-target organs and can be used to assess the efficiency of shielding in radiological examination. Conclusion: Shielding breasts and eyes during cervical radiography reduced the radiation dose to many organs. The decision to not shield patients should be based on research evidence as this approach does not apply to all cases.

The Influence of CoO/P2O5 Substitutions on the Structural, Mechanical, and Radiation Shielding of Boro-Phosphate Glasses.

A new glass system (50-x)P2O5-20B2O3-5Al2O3-25Na2O-xCoO was manufactured using a standard melt quenching procedure, where 1≤ x ≤ 12 mol%. The characteristics of boro-phosphate-glasses containing CoO have been studied. The effect of CoO on the radiation-protective properties of glasses was established. The density of the prepared glasses as a function of CoO increased. XRD was used to check the vitreous structure of samples. Fourier-transform infrared (FTIR) spectroscopy was used to study the structure of each sample. FTIR demonstrated that connections grew as CoO/P2O5 levels increased, and the FTIR spectra shifted to higher wavenumbers. The increment of CoO converts non-bridging oxygens associated with phosphate structural units into bridging oxygens. This process increases the concentration of BO4 structural units and creates new, strong and stable bonds B-O-P, i.e., there is polymerization of the boro-phosphate glass network. With an increase in the ratio of CoO/P2O5 in the produced samples, ultrasonic velocities and elastic moduli were observed to increase. The coefficients of linear and mass attenuation, the transmittance of photons in relation to the photon energy, the efficiency of radiation protection in relation to the photon energy, and the thickness of the absorber were modeled using these two methods (experimental and theoretical). From the obtained values, it can be concluded that the 12Co sample containing 12 mol% will play the most influential role in radiation protection. An increase in the content of cobalt-I oxide led to a significant increase in the linear and mass attenuation coefficient values, which directly contributes to the development of the radiation-protective properties of glass.

Gamma-Ray Protection Properties of Bismuth-Silicate Glasses against Some Diagnostic Nuclear Medicine Radioisotopes: A Comprehensive Study.

This study aimed to perform an investigation for the potential implementation of bismuth silicate glasses as novel shield equipment instead of ordinary shields in nuclear medicine facilities. Accordingly, a group of Bi2O3 reinforced silicate glass system were investigated and compared with ordinary shields in terms of their gamma-ray attenuation properties in diagnostic nuclear medicine radioisotope energies emitted from 99mTc, 111In, 67Ga, 123I, 131I, 81mKr, 201Tl, 133Xe. Mass attenuation coefficient (µm) results for glass samples were calculated comparatively with the XCOM program and MCNPX code. The gamma-ray attenuation parameters such as half value layer (HVL), tenth value layer (TVL), mean free path (MFP), effective atomic number (Zeff) were obtained in the diagnostic gamma ray energy range from 75 to 336 keV. To confirm the attenuation performance of superior sample, obtained results were extensively compared with ordinary shielding materials. According to the results obtained, BISI6 glass sample with the highest Bi2O3 additive has an excellent gamma-ray protection.

Trivalent Ions and Their Impacts on Effective Conductivity at 300 K and Radio-Protective Behaviors of Bismo-Borate Glasses: A Comparative Investigation for Al, Y, Nd, Sm, Eu.

We aimed to determine the contribution of various trivalent ions like Al and rare-earths (Y, Nd, Sm, Eu) on resistance behaviors of different types of bismo-borate glasses. Accordingly, eight different bismuth borate glasses from the system: 40Bi2O3-59B2O3-1Tv2O3 (where Tv = Al, Y, Nd, Sm, and Eu) and three glasses of (40Bi2O3-60B2O3; 37.5Bi2O3-62.5B2O3; and 38Bi2O3-60B2O3-2Al2O3) compositions were extensively investigated in terms of their nuclear attenuation shielding properties, along with effective conductivity and buildup factors. The Py-MLBUF online platform was also utilized for determination of some essential parameters. Next, attenuation coefficients, along with half and tenth value layers, have been determined in the 0.015 MeV-15 MeV photon energy range. Moreover, effective atomic numbers and effective atomic weight, along with exposure and energy absorption buildup factors, were determined in the same energy range. The result showed that the type of trivalent ion has a direct effect on behaviors of bismo-borate glasses against ionizing gamma-rays. As incident photon energy increases, the effective thermal conductivity decreases rapidly, especially in the low energy range, where photoelectric effects dominate the photon-matter interaction. Sample 8 had the minimum heat conductivity at low photon energies; our findings showed that Eu-reinforced bismo-borate glass composition, namely 40Bi2O3-59B2O3-1Eu2O3, with a glass density of 6.328 g/cm3 had superior gamma-ray attenuation properties. These outcomes would be useful for the scientific community to observe the most suitable additive rareearth type and related glass composition for providing the aforementioned shielding properties, in terms of needs and utilization requirements.

A Closer Look on Nuclear Radiation Shielding Properties of Eu3+ Doped Heavy Metal Oxide Glasses: Impact of Al2O3/PbO Substitution.

In this study, a group of heavy metal oxide glasses with a nominal composition of 55B2O3 + 19.5TeO2 + 10K2O + (15-x) PbO + xAl2O3 + 0.5Eu2O3 (where x = 0, 2.5, 5, 7.5, 10, 12.5, and 15 in wt.%) were investigated in terms of their nuclear radiation shielding properties. These glasses containing lanthanide-doped heavy metal oxide were envisioned to yield valuable results in respect to radiation shielding, and thus a detailed investigation was carried out; the obtained results were compared with traditional and new generation shields. Advanced simulation and theoretical methods have been utilized in a wide range of energy regions. Our results showed that the AL0.0 sample with the highest PbO contribution had superior shielding properties in the entire energy range. The effective removal of cross-sections for fast neutrons (ΣR) was also examined. The results indicated that AL5.0 had the greatest value. While increasing the concentration of Al2O3 in samples had a negative effect on the radiation shielding characteristics, it can be concluded that using PbO in the Eu3+ doped heavy metal oxide glasses could be a useful tool to keep gamma-ray shielding properties at a maximum level.