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1.
Nanoscale Adv ; 6(11): 2892-2902, 2024 May 29.
Artigo em Inglês | MEDLINE | ID: mdl-38817425

RESUMO

Bayesian networks and Bayesian inference, which forecast uncertain causal relationships within a stochastic framework, are used in various artificial intelligence applications. However, implementing hardware circuits for the Bayesian inference has shortcomings regarding device performance and circuit complexity. This work proposed a Bayesian network and inference circuit using a Cu0.1Te0.9/HfO2/Pt volatile memristor, a probabilistic bit neuron that can control the probability of being 'true' or 'false.' Nodal probabilities within the network are feasibly sampled with low errors, even with the device's cycle-to-cycle variations. Furthermore, Bayesian inference of all conditional probabilities within the network is implemented with low power (<186 nW) and energy consumption (441.4 fJ), and a normalized mean squared error of ∼7.5 × 10-4 through division feedback logic with a variational learning rate to suppress the inherent variation of the memristor. The suggested memristor-based Bayesian network shows the potential to replace the conventional complementary metal oxide semiconductor-based Bayesian estimation method with power efficiency using a stochastic computing method.

2.
ACS Appl Mater Interfaces ; 16(12): 15032-15042, 2024 Mar 27.
Artigo em Inglês | MEDLINE | ID: mdl-38491936

RESUMO

Nanodevice oscillators (nano-oscillators) have received considerable attention to implement in neuromorphic computing as hardware because they can significantly improve the device integration density and energy efficiency compared to complementary metal oxide semiconductor circuit-based oscillators. This work demonstrates vertically stackable nano-oscillators using an ovonic threshold switch (OTS) for high-density neuromorphic hardware. A vertically stackable Ge0.6Se0.4 OTS-oscillator (VOTS-OSC) is fabricated with a vertical crossbar array structure by growing Ge0.6Se0.4 film conformally on a contact hole structure using atomic layer deposition. The VOTS-OSC can be vertically integrated onto peripheral circuits without causing thermal damage because the fabrication temperature is <400 °C. The fabricated device exhibits oscillation characteristics, which can serve as leaky integrate-and-fire neurons in spiking neural networks (SNNs) and coupled oscillators in oscillatory neural networks (ONNs). For practical applications, pattern recognition and vertex coloring are demonstrated with SNNs and ONNs, respectively, using semiempirical simulations. This structure increases the oscillator integration density significantly, enabling complex tasks with a large number of oscillators. Moreover, it can enhance the computational speed of neural networks due to its rapid switching speed.

3.
Small ; 20(25): e2306585, 2024 Jun.
Artigo em Inglês | MEDLINE | ID: mdl-38212281

RESUMO

Compact but precise feature-extracting ability is core to processing complex computational tasks in neuromorphic hardware. Physical reservoir computing (RC) offers a robust framework to map temporal data into a high-dimensional space using the time dynamics of a material system, such as a volatile memristor. However, conventional physical RC systems have limited dynamics for the given material properties, restricting the methods to increase their dimensionality. This study proposes an integrated temporal kernel composed of a 2-memristor and 1-capacitor (2M1C) using a W/HfO2/TiN memristor and TiN/ZrO2/Al2O3/ZrO2/TiN capacitor to achieve higher dimensionality and tunable dynamics. The kernel elements are carefully designed and fabricated into an integrated array, of which performances are evaluated under diverse conditions. By optimizing the time dynamics of the 2M1C kernel, each memristor simultaneously extracts complementary information from input signals. The MNIST benchmark digit classification task achieves a high accuracy of 94.3% with a (196×10) single-layer network. Analog input mapping ability is tested with a Mackey-Glass time series prediction, and the system records a normalized root mean square error of 0.04 with a 20×1 readout network, the smallest readout network ever used for Mackey-Glass prediction in RC. These performances demonstrate its high potential for efficient temporal data analysis.

4.
Nanoscale Horiz ; 9(3): 427-437, 2024 Feb 26.
Artigo em Inglês | MEDLINE | ID: mdl-38086679

RESUMO

Multiple switching modes in a Ta2O5/HfO2 memristor are studied experimentally and numerically through a reservoir computing (RC) simulation to reveal the importance of nonlinearity and heterogeneity in the RC framework. Unlike most studies, where homogeneous reservoirs are used, heterogeneity is introduced by combining different behaviors of the memristor units. The chosen memristor for the reservoir units is based on a Ta2O5/HfO2 bilayer, in which the conductances of the Ta2O5 and HfO2 layers are controlled by the oxygen vacancies and deep/shallow traps, respectively, providing both volatile and non-volatile resistive switching modes. These several control parameters make the second-order Ta2O5/HfO2 memristor system present different behaviors in agreement with its history-dependent conductance and allow the fine-tuning of the behavior of each reservoir unit. The heterogeneity in the reservoir units improves the pattern recognition performance in the heterogeneous memristor RC system with a similar physical structure.

5.
Mater Horiz ; 11(2): 499-509, 2024 Jan 22.
Artigo em Inglês | MEDLINE | ID: mdl-37966888

RESUMO

In-sensor reservoir computing (RC) is a promising technology to reduce power consumption and training costs of machine vision systems by processing optical signals temporally. This study demonstrates a high-dimensional in-sensor RC system with optoelectronic memristors to enhance the performance of the in-sensor RC system. Because optoelectronic memristors can respond to both optical and electrical stimuli, optical and electrical masks are proposed to improve the dimensionality and performance of the in-sensor RC system. An optical mask is employed to regulate the wavelength of light, while an electrical mask is used to control the initial conductance of zinc oxide optoelectronic memristors. The distinct characteristics of these two masks contribute to the representation of various distinguishable reservoir states, making it possible to implement diverse reservoir configurations with minimal correlation and to increase the dimensionality of the in-sensor RC system. Using the high-dimensional in-sensor RC system, handwritten digits are successfully classified with an accuracy of 94.1%. Furthermore, human action pattern recognition is achieved with a high accuracy of 99.4%. These high accuracies are achieved with the use of a single-layer readout network, which can significantly reduce the network size and training costs.

6.
Adv Mater ; 36(7): e2309314, 2024 Feb.
Artigo em Inglês | MEDLINE | ID: mdl-37879643

RESUMO

Memristor-based physical reservoir computing (RC) is a robust framework for processing complex spatiotemporal data parallelly. However, conventional memristor-based reservoirs cannot capture the spatial relationship between the time-varying inputs due to the specific mapping scheme assigning one input signal to one memristor conductance. Here, a physical "graph reservoir" is introduced using a metal cell at the diagonal-crossbar array (mCBA) with dynamic self-rectifying memristors. Input and inverted input signals are applied to the word and bit lines of the mCBA, respectively, storing the correlation information between input signals in the memristors. In this way, the mCBA graph reservoirs can map the spatiotemporal correlation of the input data in a high-dimensional feature space. The high-dimensional mapping characteristics of the graph reservoir achieve notable results, including a normalized root-mean-square error of 0.09 in Mackey-Glass time series prediction, a 97.21% accuracy in MNIST recognition, and an 80.0% diagnostic accuracy in human connectome classification.

7.
Adv Mater ; 36(13): e2311040, 2024 Mar.
Artigo em Inglês | MEDLINE | ID: mdl-38145578

RESUMO

Graphs adequately represent the enormous interconnections among numerous entities in big data, incurring high computational costs in analyzing them with conventional hardware. Physical graph representation (PGR) is an approach that replicates the graph within a physical system, allowing for efficient analysis. This study introduces a cross-wired crossbar array (cwCBA), uniquely connecting diagonal and non-diagonal components in a CBA by a cross-wiring process. The cross-wired diagonal cells enable cwCBA to achieve precise PGR and dynamic node state control. For this purpose, a cwCBA is fabricated using Pt/Ta2O5/HfO2/TiN (PTHT) memristor with high on/off and self-rectifying characteristics. The structural and device benefits of PTHT cwCBA for enhanced PGR precision are highlighted, and the practical efficacy is demonstrated for two applications. First, it executes a dynamic path-finding algorithm, identifying the shortest paths in a dynamic graph. PTHT cwCBA shows a more accurate inferred distance and ≈1/3800 lower processing complexity than the conventional method. Second, it analyzes the protein-protein interaction (PPI) networks containing self-interacting proteins, which possess intricate characteristics compared to typical graphs. The PPI prediction results exhibit an average of 30.5% and 21.3% improvement in area under the curve and F1-score, respectively, compared to existing algorithms.

8.
Adv Mater ; 35(10): e2209503, 2023 Mar.
Artigo em Inglês | MEDLINE | ID: mdl-36495559

RESUMO

Many big data have interconnected and dynamic graph structures growing over time. Analyzing these graphical data requires the hidden relationship between the nodes in the graphs to be identified, which has conventionally been achieved by finding the effective similarity. However, graphs are generally non-Euclidean, which does not allow finding it. In this study, the non-Euclidean graphs are mapped to a specific crossbar array (CBA) composed of self-rectifying memristors and metal cells at the diagonal positions. The sneak current, an intrinsic physical property in the CBA, allows for the identification of the similarity function. The sneak-current-based similarity function indicates the distance between the nodes, which can be used to predict the probability that unconnected nodes will be connected in the future, connectivity between communities, and neural connections in a brain. When all bit lines of the CBA are connected to the ground, the sneak current is suppressed, and the CBA can be used to search for adjacent nodes. This work demonstrates the physical calculation methods applied to various graphical problems using the CBA composed of the self-rectifying memristor based on the HfO2 switching layer. Moreover, such applications suffer less from the memristors' inherent issues related to their stochastic nature.

9.
Nat Commun ; 13(1): 5762, 2022 Sep 30.
Artigo em Inglês | MEDLINE | ID: mdl-36180426

RESUMO

A computing scheme that can solve complex tasks is necessary as the big data field proliferates. Probabilistic computing (p-computing) paves the way to efficiently handle problems based on stochastic units called probabilistic bits (p-bits). This study proposes p-computing based on the threshold switching (TS) behavior of a Cu0.1Te0.9/HfO2/Pt (CTHP) diffusive memristor. The theoretical background of the p-computing resembling the Hopfield network structure is introduced to explain the p-computing system. P-bits are realized by the stochastic TS behavior of CTHP diffusive memristors, and they are connected to form the p-computing network. The memristor-based p-bit is likely to be '0' and '1', of which probability is controlled by an input voltage. The memristor-based p-computing enables all 16 Boolean logic operations in both forward and inverted operations, showing the possibility of expanding its uses for complex operations, such as full adder and factorization.

10.
Nat Commun ; 12(1): 5727, 2021 09 30.
Artigo em Inglês | MEDLINE | ID: mdl-34593800

RESUMO

Recent advances in physical reservoir computing, which is a type of temporal kernel, have made it possible to perform complicated timing-related tasks using a linear classifier. However, the fixed reservoir dynamics in previous studies have limited application fields. In this study, temporal kernel computing was implemented with a physical kernel that consisted of a W/HfO2/TiN memristor, a capacitor, and a resistor, in which the kernel dynamics could be arbitrarily controlled by changing the circuit parameters. After the capability of the temporal kernel to identify the static MNIST data was proven, the system was adopted to recognize the sequential data, ultrasound (malignancy of lesions) and electrocardiogram (arrhythmia), that had a significantly different time constant (10-7 vs. 1 s). The suggested system feasibly performed the tasks by simply varying the capacitance and resistance. These functionalities demonstrate the high adaptability of the present temporal kernel compared to the previous ones.

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