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1.
Sci Rep ; 13(1): 19622, 2023 Nov 10.
Artigo em Inglês | MEDLINE | ID: mdl-37949956

RESUMO

Mirror symmetry plays a major role in determining the properties of matter and is of particular interest in condensed many-body systems undergoing symmetry breaking transitions under non-equilibrium conditions. Typically, in the aftermath of such transitions, one of the two possible broken symmetry states is emergent. However, synthetic systems and those formed under non-equilibrium conditions may exhibit metastable states comprising of both left (L) and right (R) handed symmetry. Here we explore the formation of chiral charge-density wave (CDW) domains after a laser quench in 1T-TaS2 with scanning tunneling microscopy. Typically, we observed transient domains of both chiralities, separated spatially from each other by domain walls with different structure. In addition, we observe transient density of states modulations consistent with interference of L and R-handed charge density waves within the surface monolayer. Theoretical modeling of the intertwined domain structures using a classical charged lattice gas model reproduces the experimental domain wall structures. The superposition (S) state cannot be understood classically within the correlated electron model but is found to be consistent with interferences of L and R-handed charge-density waves within domains, confined by surrounding domain walls, vividly revealing an interference of Fermi electrons with opposite chirality, which is not a result of inter-layer interference, but due to the interaction between electrons within a single layer, confined by domain wall boundaries.

2.
Sci Rep ; 9(1): 15959, 2019 Nov 04.
Artigo em Inglês | MEDLINE | ID: mdl-31685868

RESUMO

Mo8O23 is a low-dimensional chemically robust transition metal oxide coming from a prospective family of functional materials, MoO3-x, ranging from a wide gap insulator (x = 0) to a metal (x = 1). The large number of stoichometric compounds with intermediate x have widely different properties. In Mo8O23, an unusual charge density wave transition has been suggested to occur above room temperature, but its low temperature behaviour is particularly enigmatic. We present a comprehensive experimental study of the electronic structure associated with various ordering phenomena in this compound, complemented by theory. Density-functional theory (DFT) calculations reveal a cross-over from a semi-metal with vanishing band overlap to narrow-gap semiconductor behaviour with decreasing temperature. A buried Dirac crossing at the zone boundary is confirmed by angle-resolved photoemission spectroscopy (ARPES). Tunnelling spectroscopy (STS) reveals a gradual gap opening corresponding to a metal-to-insulator transition at 343 K in resistivity, consistent with CDW formation and DFT results, but with large non-thermal smearing of the spectra implying strong carrier scattering. At low temperatures, the CDW picture is negated by the observation of a metallic Hall contribution, a non-trivial gap structure in STS below ∼170 K and ARPES spectra, that together represent evidence for the onset of the correlated state at 70 K and the rapid increase of gap size below ∼30 K. The intricate interplay between electronic correlations and the presence of multiple narrow bands near the Fermi level set the stage for metastability and suggest suitability for memristor applications.

3.
Phys Rev Lett ; 123(12): 129701, 2019 09 20.
Artigo em Inglês | MEDLINE | ID: mdl-31633966
4.
J Phys Condens Matter ; 25(40): 404206, 2013 Oct 09.
Artigo em Inglês | MEDLINE | ID: mdl-24025217

RESUMO

The control of condensed matter systems out of equilibrium by laser pulses allows us to investigate the system trajectories through symmetry-breaking phase transitions. Thus the evolution of both collective modes and single-particle excitations can be followed through diverse phase transitions with femtosecond resolution. Here we present experimental observations of the order parameter trajectory in the normal â†’ superconductor transition and charge density wave ordering transitions. Of particular interest is the coherent evolution of topological defects forming during the transition via the Kibble-Zurek mechanism, which appears to be measurable in optical pump-probe experiments. Experiments on CDW systems reveal some new phenomena, such as coherent oscillations of the order parameter, the creation and emission of dispersive amplitude modes upon the annihilation of topological defects, and mixing with weakly coupled finite frequency (massive) bosons.


Assuntos
Cristalização , Condutividade Elétrica , Modelos Químicos , Modelos Moleculares , Nanopartículas/química , Nanopartículas/efeitos da radiação , Simulação por Computador , Campos Eletromagnéticos
5.
Phys Rev Lett ; 110(15): 156401, 2013 Apr 12.
Artigo em Inglês | MEDLINE | ID: mdl-25167288

RESUMO

We study the incoherent recombination of topological defects created during a rapid quench of a charge-density-wave system through the electronic ordering transition. Using a specially devised three-pulse femtosecond optical spectroscopy technique we follow the evolution of the order parameter over a wide range of time scales. By careful consideration of thermal processes we can clearly identify intrinsic topological defect annihilation processes on a time scale ∼30 ps and find a possible signature of extrinsic defect-dominated relaxation dynamics occurring on longer time scales.

6.
Phys Rev Lett ; 107(17): 177007, 2011 Oct 21.
Artigo em Inglês | MEDLINE | ID: mdl-22107570

RESUMO

Using time-domain terahertz spectroscopy we performed direct studies of the photoinduced suppression and recovery of the superconducting gap in a conventional BCS superconductor NbN. Both processes are found to be strongly temperature and excitation density dependent. The analysis of the data with the established phenomenological Rothwarf-Taylor model enabled us to determine the bare quasiparticle recombination rate, the Cooper pair-breaking rate and the electron-phonon coupling constant, λ=1.1±0.1, which is in excellent agreement with theoretical estimates.

7.
Phys Rev Lett ; 106(13): 136403, 2011 Apr 01.
Artigo em Inglês | MEDLINE | ID: mdl-21517403

RESUMO

Unconventional symmetries of the order parameter allowed some researchers to maintain that a purely repulsive interaction between electrons provides superconductivity without phonons in a number of high-temperature superconductors. It is shown that the Cooper pairing in p and d states is not possible with the realistic Coulomb repulsion between fermions at relevant temperatures in any dimension.

8.
Phys Rev Lett ; 105(6): 066402, 2010 Aug 06.
Artigo em Inglês | MEDLINE | ID: mdl-20867993

RESUMO

We report on the high resolution studies of the temperature (T) dependence of the q=0 phonon spectrum in the quasi-one-dimensional charge density wave (CDW) compound K(0.3)MoO(3) utilizing time-resolved optical spectroscopy. Numerous modes that appear below T(c) show pronounced T dependences of their amplitudes, frequencies, and dampings. Utilizing the time-dependent Ginzburg-Landau theory we show that these modes result from linear coupling of the electronic part of the order parameter to the 2k(F) phonons, while the (electronic) CDW amplitude mode is overdamped.

9.
Phys Rev Lett ; 105(15): 157005, 2010 Oct 08.
Artigo em Inglês | MEDLINE | ID: mdl-21230932

RESUMO

We consider flux penetration to a 2D superconducting cylinder. We show that in the low field limit the kinetics is deterministic. In the strong field limit the dynamics becomes stochastic. Surprisingly the inhomogeneity in the cylinder reduces the level of stochasticity because of the predominance of Kelvin-Helmholtz vortices.

10.
Phys Rev Lett ; 105(25): 257001, 2010 Dec 17.
Artigo em Inglês | MEDLINE | ID: mdl-21231613

RESUMO

We determined electronic relaxation times via pump-probe optical spectroscopy using sub-15 fs pulses for the normal state of two different cuprate superconductors. We show that the primary relaxation process is the electron-phonon interaction and extract a measure of its strength, the second moment of the Eliashberg function λ[ω2] = 800 ± 200 meV2 for La(1.85)Sr(0.15)CuO4 and λ[ω2] = 400 ± 100 meV2 for YBa(2)Cu(3)O(6.5). These values suggest a possible fundamental role of the electron-phonon interaction in the superconducting pairing mechanism.

11.
Urologiia ; (6): 47-50, 2010.
Artigo em Russo | MEDLINE | ID: mdl-21427995

RESUMO

We made a microbiological study of the urine and prostatic secretion (Meares-Stamey test) of 35 patients with chronic bacterial prostatitis (CBP) aged 35-75 years. We conducted a bacterial assay, determined species, sensitivity to synthetic antibacterial fluoroquinolone drugs. A total of 163 bacterial strains were isolated, of them 13 were staphylococcal. Gram-negative bacteria were identified in the test biomaterial only in 16.6% cases. The analysis of staphylococcal sensitivity showed the highest antistaphylococcal effectiveness of levofloxacin and lomefloxacin. Our study confirms an essential role of staphylococcal bacteria in CBP etiology.


Assuntos
Prostatite/microbiologia , Infecções Estafilocócicas/microbiologia , Adulto , Idoso , Antibacterianos/farmacologia , Secreções Corporais/microbiologia , Doença Crônica , Fluoroquinolonas/farmacologia , Infecções por Bactérias Gram-Negativas/microbiologia , Infecções por Bactérias Gram-Negativas/urina , Humanos , Levofloxacino , Masculino , Testes de Sensibilidade Microbiana , Pessoa de Meia-Idade , Ofloxacino/farmacologia , Próstata/metabolismo , Próstata/microbiologia , Prostatite/urina , Infecções Estafilocócicas/urina , Staphylococcus/efeitos dos fármacos , Staphylococcus/isolamento & purificação , Urina/microbiologia
12.
Phys Rev Lett ; 102(11): 117002, 2009 Mar 20.
Artigo em Inglês | MEDLINE | ID: mdl-19392229

RESUMO

We use femtosecond spectroscopy to investigate the quasiparticle relaxation and low-energy electronic structure in a nearly optimally doped pnictide superconductor with T{c}=49.5 K. Multiple relaxation processes are evident, with distinct superconducting state quasiparticle recombination dynamics exhibiting a T-dependent superconducting gap, and a clear "pseudogaplike" feature with an onset above 180 K indicating the existence of a temperature-independent gap of magnitude Delta{PG}=61+/-9 meV above T{c}. Both the superconducting and pseudogap components show saturation as a function of fluence with distinct saturation fluences 4 and 40 microJ/cm{2}, respectively.

13.
Phys Rev Lett ; 102(8): 086405, 2009 Feb 27.
Artigo em Inglês | MEDLINE | ID: mdl-19257762

RESUMO

We measured the temperature and fluence dependence of the time-resolved photoinduced optical reflectivity in a decagonal Al71.9Ni11.1Co17.0 quasicrystal. We find no evidence for the relaxation of a hot thermalized electron gas as observed in metals. Instead, a quick diffusion of the hot nonthermal carriers approximately 40 nm into the bulk is detected, enhanced by the presence of a broad pseudogap. From the relaxation dynamics we find evidence for the suppression of the electronic density of states (DOS) at the Fermi energy with respect to the electronic DOS at approximately 13 meV away from the Fermi energy which is consistent with recent theoretical calculations.

14.
Phys Rev Lett ; 101(22): 227001, 2008 Nov 28.
Artigo em Inglês | MEDLINE | ID: mdl-19113512

RESUMO

We use ultrashort intense laser pulses to study superconducting state vaporization dynamics in La2-xSrxCuO4 (x=0.1 and 0.15) on the femtosecond time scale. We find that the energy density required to vaporize the superconducting state is 2.0+/-0.8 and 2.6+/-1.0 K/Cu for x=0.1 and 0.15, respectively. This is significantly greater than the condensation energy density, indicating that the quasiparticles share a large amount of energy with the boson glue bath on this time scale. Considering in detail both spin and lattice energy relaxation pathways which take place on the relevant time scale of approximately 10(-12) s, the experiments appear to favor phonon-mediated pair-breaking mechanisms over spin-mediated pair breaking.

15.
Vestn Otorinolaringol ; (2): 34-6, 2008.
Artigo em Russo | MEDLINE | ID: mdl-18454075

RESUMO

The results of tracheostomy and prevention of airway stenosis depend much on preoperative examination, adequate management of postoperative period. Introduction of the treatment algorithm including rational surgical approaches, wide-spectrum antibiotics, drugs improving tissue repair, local and general antihypoxic therapy significantly raises effectiveness of post-tracheostomy rehabilitation.


Assuntos
Laringoestenose/etiologia , Laringoestenose/cirurgia , Estenose Traqueal/etiologia , Estenose Traqueal/cirurgia , Traqueostomia/métodos , Humanos , Laringoestenose/epidemiologia , Prevalência , Estenose Traqueal/epidemiologia
16.
Vestn Otorinolaringol ; (2): 20-4, 2006.
Artigo em Russo | MEDLINE | ID: mdl-16710176

RESUMO

An algorithm of the treatment of laryngo- tracheal stenosis (LTS) is proposed to raise efficacy of surgical treatment of LTS and to reduce the number of postoperative complications. The algorithm comprises adequate preoperative preparation of the patients including pharmacological prophylaxis of inflammation in the operative zone; effective use of laryngotracheoplasty; prophylaxis of postoperative scarring including reconstruction of created laryngotracheal passage and administration of medicines influencing general and local immunity, tissue metabolism, repair in the region of postoperative inflammation. The efficacy of the algorithm was followed up un 54 (33.7%) patients with laryngostenosis and 106 (66.3%) patients with laryngo-tracheal stenosis. The algorithm application help rehabilitate all the patients with laryngeal stenosis and 92 (86.8%) patients with laryngo-tracheal stenosis.


Assuntos
Algoritmos , Laringoestenose/cirurgia , Procedimentos de Cirurgia Plástica/métodos , Guias de Prática Clínica como Assunto , Estenose Traqueal/cirurgia , Seguimentos , Humanos , Laringoestenose/etiologia , Estenose Traqueal/etiologia
17.
Phys Rev Lett ; 96(11): 117003, 2006 Mar 24.
Artigo em Inglês | MEDLINE | ID: mdl-16605853

RESUMO

Pairing of oxygen holes into heavy bipolarons in the paramagnetic phase and their magnetic pair breaking in the ferromagnetic phase (the so-called current-carrier density collapse) has accounted for the first-order ferromagnetic-phase transition, colossal magnetoresistance, isotope effect, and pseudogap in doped manganites. Here we propose an explanation of the phase coexistence and describe the magnetization and resistivity of manganites near the ferromagnetic transition in the framework of the current-carrier density collapse. The present quantitative description of resistivity is obtained without any fitting parameters, by using the experimental resistivities far away from the transition and the experimental magnetization, and is essentially model-independent.

18.
Phys Rev Lett ; 95(14): 147002, 2005 Sep 30.
Artigo em Inglês | MEDLINE | ID: mdl-16241687

RESUMO

Superconducting state dynamics following excitation of a superconductor with a femtosecond optical pulse is studied in terms of a phenomenological Rothwarf and Taylor model. Analytical solutions for various limiting cases are obtained. The model is found to account for the intensity and temperature dependence of both photoinduced quasiparticle density, as well as pair-breaking and superconducting state recovery dynamics in conventional as well as cuprate superconductors.

19.
Phys Rev Lett ; 95(7): 076601, 2005 Aug 12.
Artigo em Inglês | MEDLINE | ID: mdl-16196806

RESUMO

Analytical expressions for the magnetization and the longitudinal conductivity of nanowires are derived in a magnetic field, B. We show that the interplay between size and magnetic field energy-level quantizations manifests itself through novel magnetic quantum oscillations in metallic nanowires. There are three characteristic frequencies of de Haas-van Alphen (dHvA) and Shubnikov-de Haas (SdH) oscillations, F = F(0)/(1 + gamma)(3/2), and F(+/-) = 2F(0)/|1 + gamma +/- (1 + gamma)(1/2)|, in contrast with a single frequency F(0) = S(F)plankc/(2pie) in simple bulk metals. The amplitude of oscillations is strongly enhanced in some magic magnetic fields. The wire cross-section area S can be measured using the oscillations as S = 4pi(2)S(F)plank(2)c(2)/(gammae(2)B(2)) along with the Fermi-surface cross-section area, S(F).

20.
Phys Rev Lett ; 94(14): 147003, 2005 Apr 15.
Artigo em Inglês | MEDLINE | ID: mdl-15904096

RESUMO

The properties of a system of charged particles on a 2D lattice, subject to an anisotropic Jahn-Teller-type interaction and 3D Coulomb repulsion, are investigated. In the mean-field approximation without Coulomb interaction, the system displays a phase transition of first order. When the long-range Coulomb interaction is included, Monte Carlo simulations show that the system displays very diverse mesoscopic textures, ranging from spatially disordered pairs to ordered arrays of stripes, or charged clusters, depending only on the ratio of the two interactions (and the particle density). Remarkably, charged objects with an even number of particles are more stable than with an odd number of particles. We suggest that the diverse functional behavior-including superconductivity-observed in oxides can be thought to arise from the self-organization of this type.

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