Giant impurity effect on anomalous Hall effect of Mn3Sn.

Mn3Sn is an anomalous Hall effect (AHE) antiferromagnet that exhibits the hysteretic AHE in antiferromagnetic (AFM) phase at room temperature. We report that whisker Mn3Sn crystals grown by the flux method exhibit a non-hysteretic AHE at mid-to-low temperatures when the whisker Mn3Sn is surrounded by a thin layer of ferromagnetic Mn2-xSn. These crystals exhibit a hysteretic AHE above 275 K due to the spin alignment of the inverse triangular lattice, which is similar to other crystals. However, upon cooling the crystal, it exhibits a non-hysteretic AHE with a spiral AFM spin structure at 100-200 K. We concluded that the non-hysteretic AHE is induced at the interface of Mn2-xSn/Mn3Sn. We believe that the scalar-spin chirality in the spiral AFM phase of Mn3Sn, modulated by Mn2-xSn through the magnetic proximity effect, produces the AHE. This discovery opens a new avenue for tailoring the AHE by magnetic layers.

Evidence of unconventional superconductivity on the surface of the nodal semimetal CaAg1-xPdxP.

Surface states of topological materials provide extreme electronic states for unconventional superconducting states. CaAg1-xPdxP is an ideal candidate for a nodal-line Dirac semimetal with drumhead surface states and no additional bulk bands. Here, we report that CaAg1-xPdxP has surface states that exhibit unconventional superconductivity (SC) around 1.5 K. Extremely sharp magnetoresistance, tuned by surface-sensitive gating, determines the surface origin of the ultrahigh-mobility "electrons." The Pd-doping elevates the Fermi level towards the surface states, and as a result, the critical temperature (Tc) is increased up to 1.7 K from 1.2 K for undoped CaAgP. Furthermore, a soft point-contact study at the surface of Pd-doped CaAgP proved the emergence of unconventional SC on the surface. We observed the bell-shaped conductance spectra, a hallmark of the unconventional SC. Ultrahigh mobility carriers derived from the surface flat bands generate a new class of unconventional SC.

Magnetic Gap of Fe-Doped BiSbTe2Se Bulk Single Crystals Detected by Tunneling Spectroscopy and Gate-Controlled Transports.

Topological insulators with broken time-reversal symmetry and the Fermi level within the magnetic gap at the Dirac cone provides exotic topological magneto-electronic phenomena. Here, we introduce an improved magnetically doped topological insulator, Fe-doped BiSbTe2Se (Fe-BSTS) bulk single crystal, with an ideal Fermi level. Scanning tunneling microscopy and spectroscopy (STM/STS) measurements revealed that the surface state possesses a Dirac cone with the Dirac point just below the Fermi level by 12 meV. The normalized dI/dV spectra suggest a gap opening with Δmag ∼55 meV, resulting in the Fermi level within the opened gap. Ionic-liquid gated-transport measurements also support the Dirac point just below the Fermi level and the presence of the magnetic gap. The chemical potential of the surface state can be fully tuned by ionic-liquid gating, and thus the Fe-doped BSTS provides an ideal platform to investigate exotic quantum topological phenomena.

System for the remote control and imaging of MW fields for spin manipulation in NV centers in diamond.

Nitrogen-vacancy (NV) centers in diamond have been used as platforms for quantum information, magnetometry and imaging of microwave (MW) fields. The spatial distribution of the MW fields used to drive the electron spin of NV centers plays a key role for these applications. Here, we report a system for the control and characterization of MW magnetic fields used for the NV spin manipulation. The control of the MW field in the vicinity of a diamond surface is mediated by an exchangeable lumped resonator, coupled inductively to a MW planar ring antenna. The characterization of the MW fields in the near-field is performed by an FFT imaging of Rabi oscillations, by using an ensemble of NV centers. We have found that the Rabi frequency over a lumped resonator is enhanced 22 times compared to the Rabi frequency without the presence of the lumped resonator. Our system may find applications in quantum information and magnetometry where a precise and controlled spin manipulation is required, showing NV centers as good candidates for imaging MW fields and characterization of MW devices.

Imaging of current density distributions with a Nb weak-link scanning nano-SQUID microscope.

Superconducting quantum interference devices (SQUIDs) are accepted as one of the highest magnetic field sensitive probes. There are increasing demands to image local magnetic fields to explore spin properties and current density distributions in a two-dimensional layer of semiconductors or superconductors. Nano-SQUIDs have recently attracting much interest for high spatial resolution measurements in nanometer-scale samples. Whereas weak-link Dayem Josephson junction nano-SQUIDs are suitable to miniaturization, hysteresis in current-voltage (I-V) characteristics that is often observed in Dayem Josephson junction is not desirable for a scanning microscope. Here we report on our development of a weak-link nano-SQUIDs scanning microscope with small hysteresis in I-V curve and on reconstructions of two-dimensional current density vector in two-dimensional electron gas from measured magnetic field.

Circularly polarized near-field optical mapping of spin-resolved quantum Hall chiral edge states.

We have successfully developed a circularly polarized near-field scanning optical microscope (NSOM) that enables us to irradiate circularly polarized light with spatial resolution below the diffraction limit. As a demonstration, we perform real-space mapping of the quantum Hall chiral edge states near the edge of a Hall-bar structure by injecting spin polarized electrons optically at low temperature. The obtained real-space mappings show that spin-polarized electrons are injected optically to the two-dimensional electron layer. Our general method to locally inject spins using a circularly polarized NSOM should be broadly applicable to characterize a variety of nanomaterials and nanostructures.

Edge states of Sr2RuO4 detected by in-plane tunneling spectroscopy.

Tunneling spectroscopy has been performed on Sr(2)RuO(4) searching for the edge states peculiar to topological superconductivity. Conductance spectra exhibit broad humps with three types of peak shape: domelike peak, split peak, and two-step peak. By comparing the experiments with predictions for unconventional superconductivity, these varieties are shown to originate from multiband chiral p-wave symmetry with weak anisotropy of pair amplitude. The broad hump in the conductance spectrum is a direct manifestation of the edge state due to chiral p-wave superconductivity.

Josephson pi state in a ferromagnetic insulator.

We predict anomalous atomic-scale 0-pi transitions in a Josephson junction with a ferromagnetic-insulator (FI) barrier. The ground state of such junction alternates between 0 and pi states when thickness of FI is increasing by a single atomic layer. We find that the mechanism of the 0-pi transition can be attributed to thickness-dependent phase shifts between the wave numbers of electrons and holes in FI. Based on these results, we show that a stable pi state can be realized in junctions based on high-T{c} superconductors with a La2BaCuO5 barrier.

Anomalous transport through the p-wave superconducting channel in the 3-K phase of Sr2rRuO4.

Using microfabrication techniques, we extracted individual channels of 3-kelvin (3-K) phase superconductivity in Sr2RuO4-Ru eutectic systems and confirmed odd-parity superconductivity in the 3-K phase, similar to pure Sr2RuO4. Unusual hysteresis in the differential resistance-current and voltage-current characteristics observed below 2 K indicates the internal degrees of freedom of the superconducting state. A possible origin of the hysteresis is current-induced chiral-domain-wall motion due to the chiral p-wave state.

Conductance spectroscopy of spin-triplet superconductors.

We propose a novel experiment to identify the symmetry of superconductivity on the basis of theoretical results for differential conductance of a normal metal connected to a superconductor. The proximity effect from the superconductor modifies the conductance of the remote current depending remarkably on the pairing symmetry: spin singlet or spin triplet. The clear-cut difference in the conductance is explained by symmetry of Cooper pairs in a normal metal with respect to frequency. In the spin-triplet case, the anomalous transport is realized due to an odd-frequency symmetry of Cooper pairs.

Anomalous Josephson effect between even- and odd-frequency superconductors.

We demonstrate that, contrary to standard wisdom, the lowest-order Josephson coupling is possible between odd- and even-frequency superconductors. The origin of this effect is the induced odd- (even-)frequency pairing component at the interface of bulk even- (odd-)frequency superconductors. The resulting current-phase relation is found to be proportional to cosphi, where phi is the macroscopic phase difference between the two superconductors.

Theory of tunneling spectroscopy in the Larkin-Ovchinnikov state.

We present a theory of tunneling spectroscopy for normal metal/Larkin-Ovchinnikov state junctions in which the spatial periodic modulation in the pair potential amplitude is taken into account. The tunneling spectra show the characteristic line shapes reflecting the minigap structures under the periodic pair potentials depending on the boundary condition of the pair potentials at the junction interface. These features are qualitatively different from the tunneling spectra of the Fulde-Ferrell state. We propose an experimental setup which identifies the superconducting state of CeCoIn5.

Anomalous Josephson effect in p-wave dirty junctions.

The Josephson effect in p-wave superconductor/diffusive normal metal/p-wave superconductor junctions is studied theoretically. Amplitudes of Josephson currents are several orders of magnitude larger than those in s-wave junctions. Current-phase (J-phi) relations in low temperatures are close to those in ballistic junctions such as J proportional to sin(phi/2) and J proportional to phi even in the presence of random impurity potentials. A cooperative effect between the midgap Andreev resonant states and the proximity effect causes such anomalous properties and is a character of the spin-triplet superconductor junctions.