Observation of Josephson-like Tunneling Junction Characteristics and Positive Magnetoresistance in Oxygen Deficient Nickelate Films of Nd0.8Sr0.2NiO3-δ.

Nickelate films have recently attracted broad attention due to the observation of superconductivity in the infinite layer phase of Nd0.8Sr0.2NiO2 (obtained by reducing Sr doped NdNiO3 films) and their similarity to the cuprates high temperature superconductors. Here, we report on the observation of a new type of transport in oxygen poor Nd0.8Sr0.2NiO3-δ films. At high temperatures, variable range hopping is observed while at low temperatures a novel tunneling behavior is found where a Josephson-like tunneling junction characteristic with serial resistance is revealed. We attribute this phenomenon to coupling between superconductive (S) surfaces of the grains in our Oxygen poor films via the insulating (I) grain boundaries, which yields SIS junctions in series with the normal (N) resistance of the grains themselves. The similarity of the observed conductance spectra to the tunneling junction characteristic with Josephson-like current is striking, and seems to support the existence of superconductivity in our samples.

What can Andreev bound states tell us about superconductors?

Zero-energy Andreev bound states, which manifest themselves in the tunnelling spectra as zero-bias conductance peaks (ZBCPs), are abundant at interfaces between superconductors and other materials and on the nodal surface of high-temperature superconductors. In this review, we focus on the information such excitations can provide on the properties of superconductor systems. First, a general introduction to the physics of Andreev bound states in superconductor/normal metal interfaces is given with a particular emphasis on why they appear at zero energy in d-wave superconductors. Then, specific spectroscopic tunnelling studies of thin films, bilayers and junctions are described, focusing on the corresponding ZBCP features. Scanning tunnelling spectroscopy (STS) studies show that the ZBCPs on the c-axis YBa2Cu3O7-δ (YBCO) films are correlated with the surface morphology and appear only in proximity to (110) facets. STS on c-axis La1.88Sr0.12CuO4 (LSCO) films exhibiting the 1/8 anomaly shows spatially modulated peaks near zero bias associated with the anti-phase ordering of the d-wave order parameter predicted at this doping level. ZBCPs were also found in micrometre-size edge junctions of YBCO/SrRuO3/YBCO, where SrRuO3 is ferromagnetic. Here, the results are consistent with a crossed Andreev reflection effect (CARE) at the narrow domain walls of the SrRuO3 ZBCPs measured in STS studies of manganite/cuprate bilayers could not be attributed to CARE because the manganite's domain wall is much larger than the coherence length in YBCO, and instead are attributed to proximity-induced triplet-pairing superconductivity with non-conventional symmetry. And finally, ZBCPs found in junctions of non-intentionally doped topological insulator films of Bi2Se3 and the s-wave superconductor NbN are attributed to proximity-induced px + ipy triplet order parameter in the topological material.This article is part of the theme issue 'Andreev bound states'.

Pairing and the phase diagram of the normal coherence length ξN(T, x) above Tc of La(2-x)Sr(x)CuO4 thin films probed by the Josephson effect.

The long range proximity effect in high-Tc c-axis Josephson junctions with a high-Tc barrier of lower Tc is still a puzzling phenomenon. It leads to supercurrents in junctions with much thicker barriers than would be allowed by the conventional proximity effect. Here we measured the T - x (Temperature-doping level) phase diagram of the barrier coherence length ξN(T, x), and found an enhancement of ξN at moderate under-doping and high temperatures. This indicates that a possible origin of the long range proximity effect in the cuprate barrier is the conjectured pre-formed pairs in the pseudogap regime, which increase the length scale over which superconducting correlations survive in the seemingly normal barrier. In more details, we measured the supercurrents Ic of Superconducting - Normal - Superconducting SNS c-axis junctions, where S was optimally doped Y Ba2Cu3O(7-δ) below Tc (90 K) and N was La(2-x)Sr(x)CuO4 above its Tc (<25 K) but in the pseudogap regime. From the exponential decay of Ic(T) ∝ exp[-d/ξN(T)], where d is the barrier thickness, the ξN(T) values were extracted. By repeating these measurements for different barrier doping levels x, the whole phase diagram of ξN(T, x) was obtained.

Evidence for long-range correlations within arrays of spontaneously created magnetic vortices in a Nb thin-film superconductor.

We have imaged spontaneously created arrays of vortices (magnetic flux quanta), generated in a superconducting film quenched through its transition temperature at rates around 10(9) K/s. The spontaneous appearance of vortices is predicted by the Kibble-Zurek and by the Hindmarsh-Rajantie models of phase transitions under nonequilibrium conditions. Differentiating between these models requires a measurement of the internal correlations within the emerging vortex array. In addition to short-range correlations predicted by Kibble and Zurek, we found unexpected long-range correlations which are not described by any of the existing models.

A high resolution magneto-optical system for imaging of individual magnetic flux quanta.

A high-resolution magneto-optical imaging system is described. In this system magneto-optical Kerr effect is utilized for resolving individual flux quanta in a type II superconductor. Using an ultra thin EuSe indicator a spatial resolution of 0.8 microm is achieved.

Proximity-induced pseudogap: evidence for preformed pairs.

The temperature evolution of the proximity effect in Au/La(2-x)Sr(x)CuO(4) and La(1.55)Sr(0.45)CuO(4)/La(2-x)Sr(x)CuO(4) bilayers was investigated using scanning tunneling microscopy. Proximity-induced gaps, centered at the chemical potential, were found to persist above the superconducting transition temperature, T(c), and up to nearly the pseudogap crossover temperature in both systems. Such independence of the spectra on the details of the normal-metal cap layer is incompatible with a density-wave order origin. However, our results can be accounted for by a penetration of incoherent Cooper pairs into the normal metal above T(c).

Enhancement of the superconducting transition temperature of La2-xSrxCuO4 bilayers: role of pairing and phase stiffness.

The superconducting transition temperature T(c) of bilayers comprising underdoped La(2-x)Sr(x)CuO(4) films capped by a thin heavily overdoped metallic La(1.65)Sr(0.35)CuO(4) layer, is found to increase with respect to T(c) of the bare underdoped films. The highest T(c) is achieved for x=0.12, close to the "anomalous" 1/8 doping level, and exceeds that of the optimally doped bare film. Our data suggest that the enhanced superconductivity is confined to the interface between the layers. We attribute the effect to a combination of the high pairing scale in the underdoped layer with an enhanced phase stiffness induced by the overdoped film.

Design of magneto-optical system for imaging of magnetic flux created during a conductor-superconductor phase transition.

According to the Kibble-Zurek model, flux lines are spontaneously created during a fast conductor-superconductor phase transition. The model predicts both the spatial density and the correlations of the flux array. We present the design of a magneto-optical system with a projected single-flux-line resolution. Such a system can allow detailed measurements of the distribution of flux created spontaneously during a conductor-superconductor phase transition.

Anomalous proximity effect in gold coated (110) YBa2Cu3O7-delta films: penetration of the Andreev bound states.

Scanning tunneling spectroscopy of (110)YBa(2)Cu(3)O(7-delta)/Au bilayers reveal a proximity effect markedly different from the conventional one. While proximity-induced mini-gaps rarely appear in the Au layer, the Andreev bound states clearly penetrate into the metal. Zero bias conductance peaks are measured on Au layers thinner than 7 nm with a magnitude similar to those detected on the bare superconductor films. The peaks then decay abruptly with Au thickness and disappear above 10 nm. This length is shorter than the normal coherence length and corresponds to the (ballistic) mean free path.

Proximity effect in gold-coated YBa(2)Cu(3)O(7-delta) films studied by scanning tunneling spectroscopy.

Scanning tunneling spectroscopy on gold layers overcoating c-axis YBa(2)Cu(3)O(7-delta) (YBCO) films reveals proximity-induced gap structures. The gap size reduces exponentially with the distance from a-axis facets, indicating that the proximity effect is primarily due to the (100) YBCO facets. The penetration depth of superconductivity into the gold is approximately 30 nm, in good agreement with estimations for the dirty limit. The extrapolated gap at the interface is approximately 15 meV, similar to the value of an s-wave component of the order parameter measured at the YBCO surface in recent point-contact experiments.