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1.
Sci Rep ; 10(1): 7880, 2020 May 12.
Artigo em Inglês | MEDLINE | ID: mdl-32398835

RESUMO

We demonstrate a circularly polarized laser with the metal-gallium-nitride gammadion nanocavities. The ultraviolet lasing signal was observed with the high circular dichroism at room temperature under pulsed optical pump conditions. Without external magnetism which breaks the time-reversal symmetry to favor optical transitions of a chosen handedness, the coherent outputs of these chiral nanolasers show a dissymmetry factor as high as 1.1. The small footprint of these lasers are advantageous for applications related to circularly polarized photons in future integrated systems, in contrast to the bulky setup of linearly-polarized lasers and quarter-wave plates.

2.
ACS Appl Mater Interfaces ; 11(29): 26243-26249, 2019 Jul 24.
Artigo em Inglês | MEDLINE | ID: mdl-31283173

RESUMO

Atomically thin membranes of two-dimensional (2-D) transition-metal dichalcogenides (TMDCs) have distinct emission properties, which can be utilized for realizing ultrathin optoelectronic integrated systems in the future. Growing a large-area and strain-reduced monolayer 2-D material on a three-dimensional (3-D) substrate with microstructures or nanostructures is a crucial technique because the electronic band structure of TMDC atomic layers is strongly affected by the number of stacked layers and strain. In this study, a large-area and strain-reduced MoS2 monolayer was fabricated on a 3-D substrate through a two-step growth procedure. The material characteristics and optical properties of monolayer TMDCs fabricated on the nonplanar substrate were examined. The growth of monolayer MoS2 on a cone-shaped sapphire substrate effectively reduced the tensile strain induced by the substrate by decreasing the thermal expansion mismatch between the 2-D material and the substrate. Monolayer MoS2 grown on the nonplanar substrate exhibited uniform strain reduction and luminescence intensity. The fabrication of monolayer MoS2 on a nonplanar substrate increased the light extraction efficiency. In the future, large-area and strain-reduced 2-D TMDC materials grown on a nonplanar substrate can be employed as novel light-emitting devices for applications in lighting, communication, and displays for the development of ultrathin optoelectronic integrated systems.

3.
Sci Rep ; 8(1): 11812, 2018 08 07.
Artigo em Inglês | MEDLINE | ID: mdl-30087401

RESUMO

The small sized, flexible, high-performed and bio-compatible sensing devices are the critical elements to realize the bio-related detection or on-site health monitoring systems. In this work, the flexible localized surface plasmon resonance (LSPR) bio-sensors were demonstrated by integrating the metal-insulator-metal (MIM) nanodisks with bio-compatible polydimethylsiloxane (PDMS) substrate. The different geometries of MIM nanodisk sensors were investigated and optimized to enhance the spatial overlap of the LSPR waves with the environment, which lead to a high sensitivity of 1500 nm/RIU. The omni-directional characteristics of LSPR resonances were beneficial for maintaining the device sensitivity stable under various bending curvatures. Furthermore, the flexible MIM nanodisk LSPR sensor was applied to detect A549 cancer cells in PBS+ solution. The absorption peak of the MIM-disk LSPR sensor obviously redshift to easily distinguish between the phosphate buffered saline (PBS+) solution with A549 cancer cells and without cells. Therefore, the flexible MIM nanodisk LSPR sensor is suitable to develop on-chip microfluidic biosensors for detection of cancer cells on nonplanar surfaces.

4.
Sci Rep ; 7(1): 4531, 2017 07 03.
Artigo em Inglês | MEDLINE | ID: mdl-28674440

RESUMO

We propose a polarization beam splitter (PBS) with a footprint of only 600 × 790 nm2 operating at a wavelength of λ = 1550 nm, which is the smallest PBS ever demonstrated. This device uses CMOS-compatible materials, namely, silicon and silica. The present PBS comprises two Si waveguides with different geometrical aspect ratios adjoined side-by-side, which separates the transverse-electric (TE) and transverse-magnetic (TM) modes without relying on an additional coupling region. The designed PBS achieves a polarization extinction ratio of approximately 25 dB for both modes and insertion losses of approximately 0.87 and 1.09 dB for the TE and TM polarizations, respectively. Over a wide bandwidth of 150 nm (from λ = 1475-1625 nm), a high polarization extinction ratio (greater than 20 dB) and a low inversion loss (lower than 1.3 dB) can be obtained. The proposed PBS allows for geometrical errors of ±15 nm while maintaining a polarization extinction ratio of >20 dB and inversion losses of >1.1 and 1.3 dB for the TE and TM modes, respectively. With the submicron footprint, the reported PBS may be able to be used in high-density photonic integrated circuits and nanophotonic devices.

5.
Guang Pu Xue Yu Guang Pu Fen Xi ; 35(3): 663-7, 2015 Mar.
Artigo em Chinês | MEDLINE | ID: mdl-26117875

RESUMO

Combined with wastewater treatment process, the sewage in sunny and rainy day was collected from a wastewater treatment plant in Chongqing. Three-dimensional fluorescence spectra was used to investigate the characteristic fluorescence of dissolved organic matter (DOM). DOM dissolved organic carbon (DOC), chemical oxygen demand (COD), fluorescence index (ƒ450/500) and fluorescence intensity ratio γ (A, C) of fulvic acid in ultraviolet and visible region were used to analyze the impact of rain runoff pollution on sewage DOM. According to the experimental data, the DOM fluorescence fingerprints of this wastewater treatment plant were quite different from typical municipal sewage, and the main component was tryptophan with low excitation wavelength (Peak S), then the tryptophan with long wavelength excitation (Peak T) followed. A2/O process had an approximative degradation of the protein-like both in sunny day and rainy day, but had a better degradation of fulvic-like, DOC and COD in rainy day than that in sunny day. Morever, the fluorescence peaks got red-shifted after the biological treatment. The differences of DOM fluorescence fingerprint between sunny and rainy day were significant, the fluorescence center of UV fulvic (Peak A) in rainy day getting blue-shifted obviously, shifting from 240 - 248/390 - 440 to 240 - 250/370 - 400 nm. Although the DOM types in sunny and rainy day were the same, the source of fulvic got more complex by runoff and the component ratio of DOM also changed. Compared with the sunny day, the proportion of Peak S in DOM dereased by 10%, and the proportion of Peak A increased by 7% in rainy day.


Assuntos
Águas Residuárias/química , Poluentes Químicos da Água/análise , Purificação da Água , Análise da Demanda Biológica de Oxigênio , Chuva , Esgotos/análise , Espectrometria de Fluorescência , Triptofano/análise , Movimentos da Água
6.
Bioresour Technol ; 149: 51-7, 2013 Dec.
Artigo em Inglês | MEDLINE | ID: mdl-24084204

RESUMO

In this study the effect of different particle sizes of inorganic suspended solids (ISS) on the ISS accumulation in an activated sludge system was investigated. The volume mean particle diameters (Dv) of ISS were 26, 73, 106, 165, and 210 µm. There are four fates of ISS in an activated sludge system: (1) suspending in the activated sludge, (2) depositing at the bottom of the reactors, (3) discharged from the reactors via excess sludge, and lastly (4) discharged from the reactors via effluent. The accumulated ISS in the bioreactor was unevenly distributed. Based on the accumulation proportion of ISS in bioreactor, an ISS accumulation model was established, from which the ISS accumulation concentration and the MLVSS/MLSS could be predicted. The proportion of ISS suspending in activated sludge was 0.22, 0.21, 0.042 and 0.031. The proportion of ISS depositing at the bottom of bioreactors was 0.31, 0.47, 0.75, 0.76 and 0.92.


Assuntos
Compostos Inorgânicos/análise , Compostos Inorgânicos/química , Modelos Teóricos , Tamanho da Partícula , Esgotos/química , Reatores Biológicos , Reprodutibilidade dos Testes , Volatilização , Eliminação de Resíduos Líquidos
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