Transmission filters forming orthogonal basis for spectral imaging purposes.

Hyperspectral imaging has become a common technique in many different applications, enabling accurate identification of materials based on their optical properties; however, it requires complex and expensive technical implementation. A less expensive way to produce spectral data, spectral estimation, suffers from complex mathematics and limited accuracy. We introduce a novel, to the best of our knowledge, method where spectral reflectance curves can be reconstructed from the measured camera responses without complex mathematics. We have simulated the method with seven non-negative broadband transmission filters extracted from Munsell color data through principal component analysis and used sensitivity and noise levels characteristic of the Retiga 4000DC 12-bit monochrome camera. The method is sensitive to noise but produces sufficient reproduction accuracy even with six filters.

Surface lattice resonances in second-harmonic generation from metasurfaces.

We investigate the role of surface-lattice resonances (SLRs) in second-harmonic generation (SHG) from arrays of metal nanoparticles. The SLRs affect the generated signal when the sample is rotated away from normal incidence. The adjustment of the incident angle tunes the SLRs to the fundamental wavelength for SHG and improves the quality of the resonance for better resonance enhancement of SHG. Compared to normal incidence, an enhancement by a factor of 10 is observed. However, at certain incident angles, the enhancement is interrupted by diffraction anomalies, which redirect light into the substrate, increasing radiation damping and compromising the quality of the resonance.

Detection of partial polarization of light beams with dipolar nanocubes.

We confirm experimentally that the degree and state of polarization of a random, partially polarized electromagnetic beam can be obtained by probing the field with a nanoscatterer. We use a gold nanocube on silicon substrate as a local scatterer and detect the polarization characteristics of the scattered far field, which enables us to deduce the state of partial polarization of the field at the nanoprobe site. In contrast to previous beam characterization methods where spatial resolution is limited by the pixel size of the detector, the accuracy of the current technique is specified by the particle size. Our work is the first step towards polarization-state detection of random optical near fields for which the use of nanoprobes is required.

Coherence modulation by deterministic rotating diffusers.

We design rotating diffusers with deterministic complex-amplitude transmission functions, which give rise to tailored spatial coherence modulation when transilluminated by an axially incident coherent Gaussian beam. Mathematical expressions are derived for the immediate diffuser output as well as for the far-field response. An experimental demonstration is given using a diffuser fabricated by lithographic techniques.

Second-harmonic generation from metal nanoparticles: resonance enhancement versus particle geometry.

We demonstrate that optical second-harmonic generation (SHG) from arrays of noncentrosymmetric gold nanoparticles depends essentially on particle geometry. We prepare nanoparticles with different geometrical shapes (L and T) but similar wavelengths for the polarization-dependent plasmon resonances. In contrast to recent interpretations emphasizing resonances at the fundamental frequency, the T shape leads to stronger SHG when only one, instead of both, polarization component of the fundamental field is resonant. This is explained by the character of plasmon oscillations supported by the two shapes. Our numerical simulations for both linear and second-order responses display unprecedented agreement with measurements.

Enhancement of second-harmonic generation from metal nanoparticles by passive elements.

We prepare arrays of gold nanoparticles that include both noncentrosymmetric particles with a second-order nonlinear optical response (active particles) and centrosymmetric particles with no second-order response (passive particles). The plasmon resonances of the active and passive particles are at distinct wavelengths, yet the passive particles modify the electromagnetic modes of the structure in such a way that second-harmonic generation from the active particles is enhanced. Our results provide a completely new concept for optimizing the nonlinear responses of metamaterials.

Metamaterials with tailored nonlinear optical response.

We demonstrate that the second-order nonlinear optical response of noncentrosymmetric metal nanoparticles (metamolecules) can be efficiently controlled by their mutual ordering in an array. Two samples with minor change in ordering have nonlinear responses differing by a factor of up to 50. The results arise from polarization-dependent plasmonic resonances modified by long-range coupling associated with metamolecular ordering. The approach opens new ways for tailoring the nonlinear responses of metamaterials and their tensorial properties.

Spectral control in anisotropic resonance-domain metamaterials.

We introduce a concept to control the spectral and dichroic properties of metamaterials. The approach is based on anisotropic metal nanoparticles and on varying their mutual orientation in a periodic lattice. Even seemingly inconsequential changes in particle ordering strongly modify the dichroic properties of the arrays and result in either very narrow resonances or ultrabroad extinction ranges. The results arise from long-range diffractive coupling between the particles, as determined by the dependence of the array unit cell size on particle ordering.