Monocular Metasurface for Structured Light Generation and 3D Imaging with a Large Field-of-View.

Structured light three-dimensional (3D) imaging technology captures the geometric information on 3D objects by recording waves reflected from the objects' surface. The projection angle and point number of the laser dots directly determine the field-of-view (FOV) and the resolution of the reconstructed image. Conventionally, diffractive optical elements with micrometer-scale pixel size have been used to generate laser dot arrays, leading to limited FOV and point number within the projection optical path. Here, we theoretically put forward and experimentally demonstrate a monocular geometric phase metasurface composed of deep subwavelength meta-atoms to generate a 10 798 dot array within an FOV of 163°. Attributed to the vast number and high-density point cloud generated by the metasurface, the 3D reconstructed results showcase a maximum relative error in depth of 5.3 mm and a reconstruction error of 6.07%. Additionally, we propose a spin-multiplexed metasurface design method capable of doubling the number of lattice points. We demonstrate its application in the field of 3D imaging through experiments, where the 3D reconstructed results show a maximum relative depth error of 0.44 cm and a reconstruction error of 2.78%. Our proposed metasurface featuring advanced point cloud generation holds substantial potential for various applications such as facial recognition, autonomous driving, virtual reality, and beyond.

Single-molecule detection of SARS-CoV-2 N protein on multilayered plasmonic nanotraps with surface-enhanced Raman spectroscopy.

The spread of the SARS-CoV-2 virus has had an unprecedented impact, both by posing a serious risk to human health and by amplifying the burden on the global economy. The rapid identification of the SARS-CoV-2 virus has been crucial to preventing and controlling the spread of SARS-CoV-2 infections. In this study, we propose a multilayered plasmonic nanotrap (MPNT) device for the rapid identification of single particles of SARS-CoV-2 virus in ultra-high sensitivity by surface-enhanced Raman scattering (SERS). The MPNT device is composed of arrays of concentric cylindrical cavities with Ag/SiO2/Ag multilayers deposited on the top and at the bottom. By varying the diameter of the cylinders and the thickness of the multilayers, the resonant optical absorption and local electric field were optimized. The SERS enhancement factors of the proposed device are of the order of 108, which enable the rapid identification of SARS-CoV-2 N protein in concentrations as low as 1.25 × 10-15－12.5 × 10-15 g mL-1 within 1 min. The developed MPNT SERS device provides a label-free and rapid detection platform for SARS-CoV-2 virus. The general nature of the device makes it equally suitable to detect other infectious viruses.

Structured-Light 3D Imaging Based on Vector Iterative Fourier Transform Algorithm.

Quasi-continuous-phase metasurfaces overcome the side effects imposed by high-order diffraction on imaging and can impart optical parameters such as amplitude, phase, polarization, and frequency to incident light at sub-wavelength scales with high efficiency. Structured-light three-dimensional (3D) imaging is a hot topic in the field of 3D imaging because of its advantages of low computation cost, high imaging accuracy, fast imaging speed, and cost-effectiveness. Structured-light 3D imaging requires uniform diffractive optical elements (DOEs), which could be realized by quasi-continuous-phase metasurfaces. In this paper, we design a quasi-continuous-phase metasurface beam splitter through a vector iterative Fourier transform algorithm and utilize this device to realize structured-light 3D imaging of a target object with subsequent target reconstruction. A structured-light 3D imaging system is then experimentally implemented by combining the fabricated quasi-continuous-phase metasurface illuminated by the vertical-cavity surface-emitting laser and a binocular recognition system, which eventually provides a new technological path for the 3D imaging field.

Simultaneous Circular Dichroism and Wavefront Manipulation with Generalized Pancharatnam-Berry Phase Metasurfaces.

Simultaneous circular dichroism and wavefront manipulation have gained considerable attention in various applications, such as chiroptical spectroscopy, chiral imaging, sorting and detection of enantiomers, and quantum optics, which can improve the miniaturization and integration of the optical system. Typically, structures with n-fold rotational symmetry (n ≥ 3) are used to improve circular dichroism, as they induce stronger interactions between the electric and magnetic fields. However, manipulating the wavefront with these structures remains challenging because they are commonly considered isotropic and lack a geometric phase response in linear optics. Here, we propose and experimentally demonstrate an approach to achieve simultaneous circular dichroism (with a maximum value of ∼0.62) and wavefront manipulation using a plasmonic metasurface made up of C3 Archimedes spiral nanostructures. The circular dichroism arises from the magnetic dipole-dipole resonance and strong interactions between adjacent meta-atoms. As a proof of concept, two metadevices are fabricated and characterized in the near-infrared regime. This configuration possesses the potential for future applications in photodetection, chiroptical spectroscopy, and the customization of linear and nonlinear optical responses.

Ultra-thin sub-diffraction metalens with a wide field-of-view for UV focusing.

In recent years, wide field-of-view imaging technology based on a metasurface has been widely applied. However, works on the reported sub-diffraction metalens with a wide field-of-view indicate that multiple structures are essential to effectively eliminate aberrations, which results in a heavy device thickness and weakens the advantage of an ultra-thin metasurface. To solve this problem, according to the super-oscillation theory and the translational symmetry of quadratic phase, as well as the principle of virtual aperture diaphragm based on wave vector filter, this Letter demonstrates a sub-diffraction metalens combined with a single quadratic metalens and a wave vector filter. Our design not only realizes the super-resolution effects of 0.74 to 0.75 times the diffraction limit in the wide field-of-view of nearly 180° for the first time to our knowledge but also compresses the device thickness to the subwavelength order in principle. The proposed ultra-thin sub-diffraction metalens with a wide field-of-view is expected to be applied in the fields of super-resolution fast scanning imaging, information detection, small target recognition, and so on.

Visible Meta-Displays for Anti-Counterfeiting with Printable Dielectric Metasurfaces.

Metasurfaces, 2D arrays of nanostructures, have gained significant attention in recent years due to their ability to manipulate light at the subwavelength scale. Their diverse applications range from advanced optical devices to sensing and imaging technologies. However, the mass production of dielectric metasurfaces with tailored properties for visible light has remained a challenge. Therefore, the demand for efficient and cost-effective fabrication methods for metasurfaces has driven the continuing development of various techniques. In this research article, a high-throughput production method is presented for multifunctional dielectric metasurfaces in the visible light range using one-step high-index TiO2-polymer composite (TPC) printing, which is a variant of nanoprinting lithography (NIL) for the direct replication of patterned multifunctional dielectric metasurfaces using a TPC material as the printing ink. The batch fabrication of dielectric metasurfaces is demonstrated with controlled geometry and excellent optical response, enabling high-performance light-matter interactions for potential applications of visible meta-displays.

A Novel Multifunctional Photonic Film for Colored Passive Daytime Radiative Cooling and Energy Harvesting.

Passive daytime radiative cooling (PDRC) materials with sustainable energy harvesting capability is critical to concurrently reduce traditional cooling energy utilized for thermal comfort and transfer natural clean energies into electricity. Herein, a versatile photonic film (Ecoflex@BTO@UAFL) based on a novel fluorescent luminescence color passive radiative cooling with triboelectric and piezoelectric effect is developed by filling the dielectric BaTiO3 (BTO) nanoparticles and ultraviolet absorption fluorescent luminescence (UAFL) powder into the elastic Ecoflex matrix. Test results demonstrate that the Ecoflex@BTO@UAFL photonic film exhibits a maximum passive radiative cooling effect of ∽10.1 °C in the daytime. Meanwhile, its average temperature drop in the daytime is ~4.48 °C, which is 0.91 °C higher than that of the Ecoflex@BTO photonic film (3.56 °C) due to the addition of UAFL material. Owing to the high dielectric constant and piezoelectric effect of BTO nanoparticles, the maximum power density (0.53 W m-2, 1 Hz @ 10 N) of the Ecoflex@BTO photonic film-based hybrid nanogenerator is promoted by 70.9% compared to the Ecoflex film-based TENG. This work provides an ingenious strategy for combining PDRC effects with triboelectric and piezoelectric properties, which can spontaneously achieve thermal comfort and energy conservation, offering a new insight into multifunctional energy saving.

A Versatile Strategy for Concurrent Passive Daytime Radiative Cooling and Sustainable Energy Harvesting.

Developing versatile systems that can concurrently achieve energy saving and energy generation is critical to accelerate carbon neutrality. However, challenges on designing highly effective, large scale, and multifunctional photonic film hinder the concurrent combination of passive daytime radiative cooling (PDRC) and utilization of sustainable clean energies. Herein, a versatile scalable photonic film (Ecoflex@h-BN) with washable property and excellent mechanical stability is developed by combining the excellent scattering efficiency of the hexagonal boron nitride (h-BN) nanoplates with the high infrared emissivity and ideal triboelectric negative property of the Ecoflex matrix. Strikingly, sufficiently high solar reflectance (0.92) and ideal emissivity (0.97) endow the Ecoflex@h-BN film with subambient cooling effect of ≈9.5 °C at midday during the continuous outdoor measurements. In addition, the PDRC Ecoflex@h-BN film-based triboelectric nanogenerator (PDRC-TENG) exhibits a maximum peak power density of 0.5 W m-2 . By reasonable structure design, the PDRC-TENG accomplishes effective wind energy harvesting and can successfully drive the electronic device. Meanwhile, an on-skin PDRC-TENG is fabricated to harvest human motion energy and monitor moving states. This research provides a novel design of a multifunctional PDRC photonic film, and offers a versatile strategy to realize concurrent PDRC and sustainable energies harvesting.

Demonstration of 120 Gbit/s turbulence-resilient coherent optical communication employing cylindrical vector beam multiplexing.

Free space optical (FSO) communication has gained widespread attention due to its advantages, including high confidentiality, high communication capacity, and no limitation of spectrum. One of the great challenges in FSO communication is the transmission performance degradation in atmospheric turbulence channel due to wavefront distortion and scintillation. Here, we proposed and experimentally demonstrated a 120 Gbit/s vector beam multiplexed coherent optical communication system with turbulence-resilient capacity. Four multiplexed vector beams, each carrying a 30 Gbit/s quadrature phase-shift keying signal, propagate through different turbulence conditions. The influence of turbulence channel on the vector beam impairments is experimentally investigated. Under the weaker turbulence conditions, the system bit error rates are below the forward error correction threshold of 3.8 × 10-3. In comparison with the Gaussian mode, the communication interruption probability of the vector beams system decreases from 36% to 12%-18% under stronger turbulence conditions.

Flexible long-wave infrared snapshot multispectral imaging with a pixel-level spectral filter array.

This paper proposes and demonstrates a flexible long-wave infrared snapshot multispectral imaging system consisting of a simple re-imaging system and a pixel-level spectral filter array. A six-band multispectral image in the spectral range of 8-12 µm with full width at half maximum of about 0.7 µm each band is acquired in the experiment. The pixel-level multispectral filter array is placed at the primary imaging plane of the re-imaging system instead of directly encapsulated on the detector chip, which diminishes the complexity of pixel-level chip packaging. Furthermore, the proposed method possesses the merit of flexible functions switching between multispectral imaging and intensity imaging by plugging and unplugging the pixel-level spectral filter array. Our approach could be viable for various practical long-wave infrared detection applications.

High-efficiency in situ amplitude and phase control of infrared light using topological polaritons.

Polaritons - material excitation coupled with light - are thought to hold the potential for the extreme control of light down to the atomic length scale because of their high field confinement and sub-wavelength scales. For practical applications, it is essential but still a formidable challenge to manipulate polaritons with high efficiency and a wide tunable range. These obstacles may be overcome by the topology of polaritons. In photonic systems composed of graphene/α-MoO3 heterostructures, the topology of the hybrid polariton characterized by the isofrequency curve can transform from open hyperbolas to closed ellipse-like curves, driven by the carrier concentrations of graphene. The electronic tunability of such topological polaritons offers a unique platform for two-dimensional energy transfer. Here, by introducing local gates to obtain a tunable spatial carrier density profile in the graphene/α-MoO3 heterostructure, the phase of the polariton is predicted to be efficiently tuned from 0 to 2π in situ. Remarkably, the reflectance and transmittance through the gap between local gates can also be modulated in situ from 0 to 1 with high efficiency, where the device length can be less than 100 nm. The modulation is achieved owing to the dramatic changes in the wave vector of polaritons near the topological transition point. The proposed structures not only have direct applications in two-dimensional optics such as total reflectors, phase (amplitude) modulators, and optical switches but also can serve as an important component for complex nano-optical devices.

Miniaturized solar-blind ultraviolet imaging system enabled by a diffractive/refractive hybrid.

In this paper, we demonstrated a miniaturized diffractive/refractive hybrid system based on a diffractive optical element and three refractive lenses to achieve solar-blind ultraviolet imaging within a range of 240-280 nm. We experimentally demonstrate the optical system has both outstanding resolution and excellent imaging capability. The experiments demonstrate that the system could distinguish the smallest line pair with a width of 16.7 µm. The modulation transfer function (MTF) at the target maximum frequency (77 lines pair/mm) is great than 0.76. The strategy provides significant guidance for the mass production of solar-blind ultraviolet imaging systems towards miniaturization and lightweight.

Ultrasensitive enhanced Raman spectroscopy by hybrid surface-enhanced and interference-enhanced Raman scattering with metal-insulator-metal structures.

High-sensitivity, reproducible, and low-cost substrate has been a major obstacle for practical sensing application of surface-enhancement Raman scattering (SERS). In this work, we report a type of simple SERS substrate which is composed of metal-insulator-metal (MIM) structure of Ag nanoisland (AgNI)-SiO2-Ag film (AgF). The substrates are fabricated by only evaporation and sputtering processes, which are simple, fast and low-cost. By combining the hotspots and interference-enhanced effects in AgNIs and the plasmonic cavity (SiO2) between AgNIs and AgF, the proposed SERS substrate shows an enhancement factor (EF) of 1.83 × 108 with limit of detection (LOD) down to 10-17 mol/L for rhodamine 6 G (R6G) molecules. The EFs are ∼18 times higher than that of conventional AgNIs without MIM structure. In addition, the MIM structure shows excellent reproducibility with relative standard deviation (RSD) less than 9%. The proposed SERS substrate is fabricated only with evaporation and sputtering technique and the conventionally used lithographic methods or chemical synthesis are not required. This work provides a simple way to fabricate ultrasensitive and reproducible SERS substrates which show great promise for developing various biochemical sensors with SERS.

Meta-optics empowered vector visual cryptography for high security and rapid decryption.

Optical encryption is a promising approach to protecting secret information owing to the advantages of low-power consumption, parallel, high-speed, and multi-dimensional processing capabilities. Nevertheless, conventional strategies generally suffer from bulky system volume, relatively low security level, redundant measurement, and/or requirement of digital decryption algorithms. Here, we propose a general optical security strategy dubbed meta-optics-empowered vector visual cryptography, which fully exploits the abundant degrees of freedom of light as well as the spatial dislocation as key parameters, significantly upgrading the security level. We also demonstrate a decryption meta-camera that can implement the reversal coding procedure for real-time imaging display of hidden information, avoiding redundant measurement and digital post-processing. Our strategy features the merits of a compact footprint, high security, and rapid decryption, which may open an avenue for optical information security and anti-counterfeiting.

Simple route for high-throughput fabrication of metasurfaces using one-step UV-curable resin printing.

Phase-gradient metasurfaces are two-dimensional (2D) optical elements that can manipulate light by imposing local, space-variant phase changes on an incident electromagnetic wave. These metasurfaces hold the potential and the promise to revolutionize photonics by providing ultrathin alternatives for a wide range of common optical elements such as bulky refractive optics, waveplates, polarizers, and axicons. However, the fabrication of state-of-the-art metasurfaces typically requires some time-consuming, expensive, and possibly hazardous processing steps. To overcome these limitations on conventional metasurface fabrication, a facile methodology to produce phase-gradient metasurfaces through one-step UV-curable resin printing is developed by our research group. The method dramatically reduces the required processing time and cost, as well as eliminates safety hazards. As a proof-of-concept, the advantages of the method are clearly demonstrated via a rapid reproduction of high-performance metalenses based on the Pancharatnam-Berry phase gradient concept in the visible spectrum.

Polarization-Insensitive Metasurface Cloak for Dynamic Illusions with an Electromagnetic Transparent Window.

Artificial camouflage has garnered long-standing interest in both academia and industry. The metasurface-based cloak has attracted much attention due to the powerful capability of manipulating the electromagnetic wave, convenient multifunctional integration design, and easy fabrication. However, existing metasurface-based cloaks tend to be passive and of single function and monopolarization, which cannot meet the requirement of applications in ever-changing environments. So far, it is still challenging to realize a reconfigurable full-polarization metasurface cloak with multifunctional integration. Herein, we proposed an innovative metasurface cloak, which can simultaneously realize dynamic illusion effects at lower frequencies (e.g., 4.35 GHz) and specific microwave transparency at higher frequencies (e.g., X band) for communication with the outside environment. These electromagnetic functionalities are demonstrated by both numerical simulations and experimental measurements. The simulation and measurement results agree well with each other, indicating that our metasurface cloak can generate various electromagnetic illusions for full polarizations as well as a polarization-insensitive transparent window for the signal transmission to enable the communication between the cloaked device and the outside environment. It is believed that our design can offer powerful camouflage tactics to address the stealth problem in ever-changing environments.

Experimental demonstration of an 8-Gbit/s free-space secure optical communication link using all-optical chaos modulation.

For the first time, to the best of our knowledge, we experimentally demonstrate a high-speed free-space secure optical communication system based on all-optical chaos modulation. The effect of atmospheric turbulence on optical chaos synchronization is experimentally investigated via a hot air convection atmospheric turbulence simulator. It is shown that, even under moderately strong turbulent conditions, high-quality chaos synchronization could be obtained by increasing the transmission power. Moreover, a secure encryption transmission experiment using a high bias current induced chaotic carrier for 8-Gbit/s on-off-keying data over a ∼10-m free-space optical link is successfully demonstrated, with a bit-error rate below the FEC threshold of 3.8 × 10-3. This work favorably shows the feasibility of optical chaotic encryption for the free-space optical transmission system.

High Performance Graphene-C60 -Bismuth Telluride-C60 -Graphene Nanometer Thin Film Phototransistor with Adjustable Positive and Negative Responses.

Graphene is a promising candidate for the next-generation infrared array image sensors at room temperature due to its high mobility, tunable energy band, wide band absorption, and compatibility with complementary metal oxide semiconductor process. However, it is difficult to simultaneously obtain ultrafast response time and ultrahigh responsivity, which limits the further improvement of graphene photoconductive devices. Here, a novel graphene/C60 /bismuth telluride/C60 /graphene vertical heterojunction phototransistor is proposed. The response spectral range covers 400-1800 nm; the responsivity peak is 106 A W-1 ; and the peak detection rate and peak response speed reach 1014 Jones and 250 µs, respectively. In addition, the regulation of positive and negative photocurrents at a gate voltage is characterized and the ionization process in impurities of the designed phototransistor at a low temperature is analyzed. Tunable bidirectional response provides a new degree of freedom for phototransistors' signal resolution. The analysis of the dynamic change process of impurity energy level is conducted to improve the device's performance. From the perspective of manufacturing process, the ultrathin phototransistor (20-30 nm) is compatible with functional metasurface to realize wavelength or polarization selection, making it possible to achieve large-scale production of integrated spectrometer or polarization imaging sensor by nanoimprinting process.

Remote sensing inversion and prediction of land use land cover in the middle reaches of the Yangtze River basin, China.

Land use and land cover (LULC) changes are dynamic and have been extensively studied; the change in LULC has become a crucial factor in decision making for planners and conservationists owing to its impact on natural ecosystems. Deriving accurate LULC data and analyzing their changes are important for assessing the energy balance, carbon balance, and hydrological cycle in a region. Therefore, we investigated the best classification method from the four methods and analyzed the change in LULC in the middle Yangtze River basin (MYRB) from 2001 to 2020 using the Google Earth Engine (GEE). The results suggest that (1) GEE platform enables to rapidly acquire and process remote sensing images for deriving LULC, and the random forest (RF) algorithm was able to calculate the highest overall accuracy and kappa coefficient (KC) of 87.7% and 0.84, respectively; (2) forestland occupied the largest area from 2001 to 2020, followed by water bodies and buildings. During the study period, there was a significant change in area occupied by both water bodies (overall increase of 46.2%) and buildings (decrease of 14.3% from 2001 to 2005); and (3) the simulation of LULC in the MYRB area was based on the primary drivers in the area, of which elevation changes had the largest effect on LULC changes. The patch generated land use simulation model (PLUS) was used to produce the simulation, with an overall accuracy and KC of 89.6% and 0.82, respectively. This study not only was useful for understanding the spatial and temporal characteristics of LULC in the MYRB, but also offered the basis for the simulation of ecological quality in this region.