Plutonium isotopes and radionuclides in corals around Weizhou land in Beibu Gulf, China.

Plutonium isotopes in the coral were determined with chemical separation method using AG 1-X8 and AG-MP-1M anion exchange resins and sector field inductively coupled plasma mass spectrometry (SF-ICP-MS) in order to elucidate the activity concentration and source of Pu around Weizhou land in Beibu Gulf, China. Furthermore, the activity concentrations of other radionuclides (238U, 226Ra, 232Th, 137Cs, 40K and 210Pb) were measured by a HPGe spectrometer. The activity concentration of 240+239Pu in the coral is determined to be in the range of 8.95-27.84 mBq/kg. The 240Pu/239Pu atom ratios in the samples range from 0.173 to 0.225, indicating that the main source of plutonium in this area is global fallout while the contribution of PPG is about 30%. Further, the activity concentrations of 238U, 232Th, 40K and 226Ra are determined to be in the range of 18.72-64.63, 1.37-20.8, 29.78-72.52 and 3.48-61.97 Bq/kg, respectively.

Radionuclides in the environment around the uranium mines in Guangxi, China.

Uranium and plutonium are both poisonous radioactive elements, which are very harmful to human health and environment. Therefore, it is of great significance to study the distribution of 238U concentration and 239+240Pu activity in the uranium mine surrounding soils. We have collected some surface soil sediments within 2 km of two uranium mines and a solid waste management center in Guangxi Province. The 238U concentration in these study areas is in the range of 1.44-83.91 mg/g, and the 238U concentration in the A uranium mine surrounding surface soils is higher than that in the B uranium mine and the solid waste management center. While the B uranium mine and the solid waster management center don't pollute the surrounding soils because the 238U concentrations in their surrounding soils are similar to the average 238U concentration in the soil. The 239+240Pu activities in soil samples collected around the two uranium mines and the solid waste management center are close ranged from 0.06 mBq/g to 0.51 mBq/g. Moreover, the 240Pu/239Pu atom ratios in our study samples are ranged from 0.15 to 0.23, which indicate the Pu may come from the global fallout. In addition, we study heavy metals in our collected samples, only heavy metal Tl has weak positive correlations with 238U concentrations and 239+240Pu activities. And there is a weak positive correlation between 238U concentrations and 239+240Pu activities.

Characteristic of Pu from urban wetland and lacustrine sediments in Suzhou Industrial Park, China.

In this study, plutonium activity concentrations in the urban wetlands and lacustrine sediment of Suzhou Industrial Park (SIP) are studied for the first time. Results show 239+240Pu activity concentrations in the wetland surface soils of SIP range from 0.035 to 0.426 mBq/g and the 240Pu/239Pu atom ratio ranges from 0.171±0.024 to 0.226±0.049. Judging from the atom ratio of 240Pu/239Pu, the main source of Pu in the wetland is global fallout. The correlations of Pu between organic matter and heavy metals are also studied. The correlation coefficients show Pu has significant positive correlations with Cu, Sn and Pb but negative correlation with As. Unlike distributions of Pu in other places, Pu in SIP has weak correlation with organic matter content. A sediment core from Lake Yangcheng is also analyzed to investigate the historical record of Pu deposition. The atom ratios of each layer in the sediment core indicate the area is mainly influenced by global fallout. Using Pu as a discrete-time maker, the deposition rate in Lake Yangcheng is 0.396±0.019 cm/yr. The calculated inventory of 239+240Pu is 58.5 Bq/m2, which is in the range of inventories of the corresponding latitudes according to UNSCEAR.