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1.
J Air Waste Manag Assoc ; 72(12): 1341-1365, 2022 12.
Artigo em Inglês | MEDLINE | ID: mdl-34569916

RESUMO

The landfill leachate is considered a toxic effluent composed of recalcitrant contaminants that requires innovative alternatives for its decontamination. Coupling between advanced oxidation processes (AOPs) and aerobic biological treatments are highlighted in this research. Therefore, a bibliographic review of the research made from 2010 to 2021 was developed. These combined alternatives were applied in leachates, and it is oriented toward the analysis of knowledge gaps, trends, and future proposals of the treatment combined that contribute to researchers who wish to work on the subject. These kinds of treatments were chosen due to a bibliometric analysis made. Also, the information was searched in several scientific database. This work was found to be unpublished, as no reviews were found so far that agglomerate studies of coupling between photocatalytic and aerobic biological processes to treat leachates. Besides, AOPs are ideal for treating wastewater of complex composition, however, when it is used as the only treatment, they are usually unprofitable, which justifies their coupling with biological treatments. Subsequently, it was determined that the knowledge main gap is the lack of documentation of treatment costs, which makes it difficult to implement on a real scale. In addition to this, the couplings trends are toward doping with metallic and nonmetallic ions of the catalyst used in the photocatalytic process to improve the efficiency of these. Finally, future research should work on finding alternatives that allow the optimization of the resources used in the combined systems and on promoting the recovery of existing products in the leachate.Implications: Leachates generate several environmental impacts due to their toxic composition. Even when coupling between heterogeneous photocatalysis and biologic treatment can solve them, issues like cost analysis and the scaling-up factor have not been developed, and futures researchers should work on that. Besides, the trend founded in almost all investigations was the catalyst doping with metals and nonmetals ions, particularly when they use TiO2 because it gives the possibility of improving efficiencies just with a structural variation. Finally, these treatment combinations require more analyses and comparison of their remotion over emerging pollutants and their performance with new designs.


Assuntos
Fenômenos Biológicos , Poluentes Químicos da Água , Descontaminação , Oxirredução , Poluentes Químicos da Água/química
2.
Water Sci Technol ; 82(2): 315-329, 2020 Jul.
Artigo em Inglês | MEDLINE | ID: mdl-32941173

RESUMO

Reuse of wastewater, as well as recovery of valuable, toxic or harmful products in industrial discharges, still represents an important issue, not only because it reduces the effect on receiving water bodies, but also because of the economic resources it represents for industry itself. In this research, in situ regeneration of Mn2SO4 is evaluated, for its reuse as the main raw material in the original process of a fungicide plant. The regeneration is evaluated by selective recovery of Mn2+, Zn2+ and SO4 = present in the wastewater produced by the industrial plant, and utilizing nanofiltration, electro-electrodialysis and chemical precipitation as separation alternatives. Each alternative was designed and evaluated technically and economically through simulations in Aspen Plus®, with data and information of the real process supplied by the company. Because zinc concentration is relatively low, its selective recovery was not attractive. The resulting Mn2SO4 solution and treated water quality in conventional alternatives were significantly poor with high costs. In contrast, nanofiltration and electro-electrodialysis alternatives generate water and by-products of higher quality and reuse potential with significantly lower costs. However, their viability depends on the membrane performance. The results were satisfactory, but future experimental studies are required to optimize the alternatives and define the correct pretreatment process.


Assuntos
Praguicidas , Purificação da Água , Compostos de Manganês , Sulfatos , Eliminação de Resíduos Líquidos , Águas Residuárias
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