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1.
Phys Rev Lett ; 130(4): 046701, 2023 Jan 27.
Artigo em Inglês | MEDLINE | ID: mdl-36763421

RESUMO

A leading nonlinear effect in magnonics is the interaction that splits a high-frequency magnon into two low-frequency magnons with conserved linear momentum. Here, we report experimental observation of nonlocal three-magnon scattering between spatially separated magnetic systems, viz. a CoFeB nanowire and a yttrium iron garnet (YIG) thin film. Above a certain threshold power of an applied microwave field, a CoFeB Kittel magnon splits into a pair of counterpropagating YIG magnons that induce voltage signals in Pt electrodes on each side, in excellent agreement with model calculations based on the interlayer dipolar interaction. The excited YIG magnon pairs reside mainly in the first excited (n=1) perpendicular standing spin-wave mode. With increasing power, the n=1 magnons successively scatter into nodeless (n=0) magnons through a four-magnon process. Our results demonstrate nonlocal detection of two separately propagating magnons emerging from one common source that may enable quantum entanglement between distant magnons for quantum information applications.

2.
Entropy (Basel) ; 23(12)2021 Dec 06.
Artigo em Inglês | MEDLINE | ID: mdl-34945945

RESUMO

Entropy is a quantity expressing the measure of disorder or unpredictability in a system, and, from a more general point of view, it can be regarded as an irreversible source of energy [...].

3.
Chemphyschem ; 18(12): 1642-1652, 2017 Jun 20.
Artigo em Inglês | MEDLINE | ID: mdl-28380275

RESUMO

Periodic dispersion-corrected DFT is used to investigate the adsorption of I2 and ICH3 , which may be released during a severe nuclear accident, for three divalent cation (Cu2+ , Pb2+ and Hg2+ )-exchanged mordenites with an Si/Al ratio of 23. Gases such as H2 O, CO, ClCH3 , and Cl2 present in the containment atmosphere can inhibit the selective adsorption of iodine species. To identify the most promising adsorbents, a systematic study is performed in which all the possible cationic sites in the main channel of the mordenite structure are considered. For the energetically most stable sites, the divalent cation is located in the small rings (five- or six-membered) containing two Al atoms, while in the energetically less stable configurations, the two Al atoms are far apart (>7 Å) and the cation is close to only one Al atom. Upon adsorption of the various molecules, the coordination number of the cation decreases with increasing interaction energy, as the molecules can attract the divalent cations from the framework. Finally, the computed interaction energies show that Hg-mordenite (MOR) could be a suitable material for selective adsorption of volatile iodine species, contrary to Cu-MOR and Pb-MOR.

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