Respiratory Monitoring by Ultrafast Humidity Sensors with Nanomaterials: A Review.

Respiratory monitoring is a fundamental method to understand the physiological and psychological relationships between respiration and the human body. In this review, we overview recent developments on ultrafast humidity sensors with functional nanomaterials for monitoring human respiration. Key advances in design and materials have resulted in humidity sensors with response and recovery times reaching 8 ms. In addition, these sensors are particularly beneficial for respiratory monitoring by being portable and noninvasive. We systematically classify the reported sensors according to four types of output signals: impedance, light, frequency, and voltage. Design strategies for preparing ultrafast humidity sensors using nanomaterials are discussed with regard to physical parameters such as the nanomaterial film thickness, porosity, and hydrophilicity. We also summarize other applications that require ultrafast humidity sensors for physiological studies. This review provides key guidelines and directions for preparing and applying such sensors in practical applications.

Mesoporous Solid and Yolk-Shell Titania Microspheres as Touchless Colorimetric Sensors with High Responsivity and Ultrashort Response Times.

Touchless user interfaces offer an attractive pathway toward hygienic, remote, and interactive control over devices. Exploiting the humidity generated from fingers or human speech is a viable avenue for realizing such technology. Herein, titania microspheres including solid and yolk-shell structures with varying microstructural characteristics were demonstrated as high-performance, ultrafast, and stable optical humidity sensors aimed for touchless control. When water molecules enter the microporous network of the microspheres, the effective refractive index of the microsphere increases, causing a detectable change in the light scattering behavior. The microstructural properties of the microspheres, namely, the pore characteristics, crystallinity, and particle size, were examined in relation to the humidity-sensing performance, establishing optimum structural conditions for realizing humidity-responsive wavelength shifts above 100 nm, near full-scale relative humidity (RH) responsivity, ultrashort response times below 30 ms, and prolonged lifetimes. These optimized microspheres were used to demonstrate a colorimetric touchless sensor that responds to humidity from a finger and a microcontroller-based detector that translates the moisture pattern from human speech to electrical signals in real time. These results provide practical strategies for enabling humidity-based touchless user interfaces.

Mie Resonant Structural Colors.

Structural colors refer to colors produced by the interference of light scattered by judiciously arranged nano- or microscopic structures. In this Forum Article, we discuss the use of Mie resonant scattering in structural colors with dielectric and metal-dielectric hybrid structures to achieve notable figures of merit in pixel size and gamut range. Compared with plasmonic structures, resonant dielectric and hybrid structures are subjected to less loss while providing strong field confinement and large scattering cross sections, making them appealing for realizing vibrant colors at ultrahigh resolutions. We outline the basic principles behind Mie resonances in analytically solvable structures and highlight the relation between these resonances and color with demonstrations in dielectric metasurfaces. Mie resonant colors occurring in nonplanar designs including disordered systems are also explored. We review recent advances in dynamic and reversibly tunable Mie resonant colors and conclude by providing an outlook for future research directions.