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1.
J Air Waste Manag Assoc ; 72(11): 1241-1258, 2022 Nov.
Artigo em Inglês | MEDLINE | ID: mdl-36318721

RESUMO

The Western Regional Air Partnership (WRAP) has developed a modeling platform to simulate the formation of haze-causing particles that impact federally-protected lands in the western United States. To assist state air quality planners in determining which emission sources are likely candidates for future mitigation, several source apportionment scenarios were evaluated, and two sets of results for the year 2028 are presented here: 1) a "high-level important regional sources" version, with broad emission categories (i.e. U.S. anthropogenic, international anthropogenic, natural, and fires), and 2) a "low-level anthropogenic emission sources within individual states" version, which refines the U.S. anthropogenic contribution to specific emission sectors within individual WRAP region states. Eight examples are discussed, which reflect the variation in source apportionment results at national parks, wilderness areas, and wildlife refuges in the western U.S. and suggest which emission sectors are candidates for mitigation to improve future visibility. In 2028, the contribution of domestic anthropogenic emissions at the eight sites ranges from 17% to 58%, with significant impacts from oil and gas production, fossil fuel electric generation, and federally-regulated mobile sources. The contribution from international anthropogenic sources can also be considerable, and ranges from 17% to 43%. Most sectors that are emitting sulfur dioxide (SO2) and nitrogen oxides (NOx), which are the two most likely particle precursors to be curtailed in the states' Regional Haze plans, are declining. For example, in the 13 contiguous WRAP region states, NOx emissions from on-road mobile sources and electric generating units (EGUs) declined by 738 kton/yr (29% decrease) and 65 kton/yr (31% decrease), respectively, in 2028 as compared to current emission estimates, and SO2 emissions from EGUs declined by 42 kton/yr (29% decrease). NOx emissions from oil and gas development also declined by 25 kton/yr (9% decrease) but rose for SO2 emissions by 12 kton/yr (20% increase).Implications: The goal of the Regional Haze Rule (RHR) is to improve visibility at federally-protected areas, and to eventually arrive at natural conditions by the year 2064. Source apportionment tools within regional air quality models are useful for identifying which emission regions and sectors are contributing to haze-causing particles and can indicate to air quality planners where additional emission controls may be warranted.


Assuntos
Poluentes Atmosféricos , Poluição do Ar , Incêndios , Estados Unidos , Poluição do Ar/análise , Poluentes Atmosféricos/análise , Óxidos de Nitrogênio/análise , Dióxido de Enxofre , Monitoramento Ambiental/métodos
2.
J Air Waste Manag Assoc ; 72(11): 1259-1278, 2022 Nov.
Artigo em Inglês | MEDLINE | ID: mdl-36205721

RESUMO

The U.S. EPA developed the Regional Haze Rule to address Section 7491 of the 1977 Clean Air Act Amendments to prevent any future and remedy any existing visibility impairment due to manmade air pollution at Federal Class I areas (CIAs). The rule addresses this national goal by requiring states to show they are making progress toward estimated natural conditions by 2064 for the 20% anthropogenically Most Impaired Days (MID). For the MID, days that have high haze contributions from wildfires and windblown dust tend to be excluded using haze contributions from Carbon and crustal material as surrogates. To show progress toward natural conditions in 2064, a Uniform Rate of Progress Glidepath is defined as a straight line from measured 2000-2004 IMPROVE MID Baseline to natural conditions in 2064. Photochemical modeling is used to project the observed IMPROVE 2014-2018 MID visibility to 2028 that is compared to the Glidepath at 2028 to determine whether the MID visibility at a CIA is on a path toward natural visibility conditions in 2064. This paper discusses an alternative approach for showing progress toward no manmade impairment by using modeling results to generate a U.S. Anthropogenic Emissions Rate of Progress (RoP). The CAMx photochemical grid model was run for a current year (representing 2014-2018), 2028 future year and a 2002 past year and source apportionment was used to isolate the contributions of U.S. anthropogenic emissions to PM concentrations and visibility extinction. A RoP slope line is drawn from the 2002 visibility extinction due to U.S. anthropogenic emissions to zero in 2064 and the CAMx 2028 visibility for U.S. anthropogenic emissions is compared with the RoP slope line at 2028 to determine whether visibility due to U.S. anthropogenic emissions is on a path toward no U.S. manmade impairment in 2064.Implications: The U.S. EPA Regional Haze Rule guidance to show progress toward no U.S. manmade visibility impairment at Class I Areas by 2064 backs into the U.S. manmade impairment contribution by using total atmospheric haze based on measured PM concentrations and subtracting uncertain estimates of routine natural and episodic (i.e. wildfires and windblown dust) natural conditions. The guidance also recommends accounting for visibility contributions due to international anthropogenic and prescribed fire emissions that are also uncertain. This paper presents an alternative approach that models the contributions of U.S. anthropogenic emissions to visibility for past, current and future years using source apportionment to show that U.S. anthropogenic emissions visibility impairment at Class I areas are on a path toward no contribution in 2064. Many U.S. anthropogenic emissions (e.g. power plants with continuous emissions monitoring systems) are better known and characterized than international, fire and natural emissions so the alternative approach should provide a better assessment of whether U.S. anthropogenic emissions are on a path toward no manmade impairment in 2064 than using trends in the measured visibility most impaired days that rely on uncertain estimates of haze due to wildfire, windblown dust, and international emissions and uncertain estimates of natural conditions in 2064.


Assuntos
Poluentes Atmosféricos , Poluição do Ar , Incêndios , Incêndios Florestais , Estados Unidos , Objetivos , Poeira , Monitoramento Ambiental , Material Particulado
3.
J Air Waste Manag Assoc ; 69(3): 373-390, 2019 03.
Artigo em Inglês | MEDLINE | ID: mdl-30339494

RESUMO

The 2017 revisions to the Regional Haze Rule clarify that visibility progress at Class I national parks and wilderness areas should be tracked on days with the highest anthropogenic contributions to haze (impairment). We compare the natural and anthropogenic contributions to haze in the western United States in 2011 estimated using the Environmental Protection Agency (EPA) recommended method and using model projections from the Comprehensive Air Quality Model with Extensions (CAMx) and the Particulate Source Apportionment Tool (PSAT). We do so because these two methods will be used by states to demonstrate visibility progress by 2028. If the two methods assume different natural and anthropogenic contributions, the projected benefits of reducing U.S. anthropogenic emissions will differ. The EPA method assumes that episodic elevated carbonaceous aerosols greater than an annual 95th percentile threshold are natural events. For western U.S. IMPROVE monitoring sites reviewed in this paper, CAMx-PSAT confirms these episodes are impacted by carbon from wildfire or prescribed fire events. The EPA method assumes that most of the ammonium sulfate is anthropogenic in origin. At most western sites CAMx-PSAT apportions more of the ammonium sulfate on the most impaired days to global boundary conditions and anthropogenic Canadian, Mexican, and offshore shipping emissions than to U.S. anthropogenic sources. For ammonium nitrate and coarse mass, CAMx-PSAT apportions greater contributions to U.S. anthropogenic sources than the EPA method assigns to total anthropogenic contributions. We conclude that for western IMPROVE sites, the EPA method is effective in selecting days that are likely to be impacted by anthropogenic emissions and that CAMx-PSAT is an effective approach to estimate U.S. source contributions. Improved inventories, particularly international and natural emissions, and further evaluation of global and regional model performance and PSAT attribution methods are recommended to increase confidence in modeled source characterization. Implications: The western states intend to use the CAMx model to project visibility progress by 2028. Modeled visibility response to changes in U.S. anthropogenic emissions may be less than estimated using the EPA assumptions based on total U.S. and international anthropogenic contributions to visibility impairment. Additional model improvements are needed to better account for contributions to haze from natural and international emissions in current and future modeling years. These improvements will allow more direct comparison of model and EPA estimates of natural and anthropogenic contributions to haze and future visibility progress.


Assuntos
Poluentes Atmosféricos/análise , Poluentes Atmosféricos/normas , Poluição do Ar/análise , Poluição do Ar/prevenção & controle , Monitoramento Ambiental/métodos , Oxidantes Fotoquímicos/análise , Canadá , México , Estados Unidos , United States Environmental Protection Agency
4.
Environ Sci Technol ; 43(17): 6669-75, 2009 Sep 01.
Artigo em Inglês | MEDLINE | ID: mdl-19764233

RESUMO

Two efficient methods to study relationships between particulate matter (PM) concentrations and emission sources are compared in the three-dimensional comprehensive air quality model with extensions (CAMx). Particulate source apportionment technology (PSAT) is a tagged species method that apportions concentrations of PM components to their respective primary precursors, e.g., sulfate is apportioned to SOx, nitrate to NOx, etc. The decoupled direct method (DDM) calculates first-order sensitivities of PM concentrations to model inputs. Both tools were applied to two month long (February and July) PM modeling episodes and evaluated against changes in PM concentrations due to various emission reductions. The results show that source contributions calculated by PSAT start to deviate from the actual model responses as indirect effects from limiting reactants or nonprimary precursor emissions become important The DDM first-order sensitivity is useful for determining source contributions only if the model response to input changes is reasonably linear. For secondary inorganic PM, the response is linear for emission reductions of 20% in all cases considered and reasonably linear for reductions of 100% inthe case of on-road mobile sources. The model response for secondary organic aerosols and primary PM remains nearly linear to 100% reductions in anthropogenic emissions.


Assuntos
Poluentes Atmosféricos/análise , Ar/análise , Modelos Teóricos , Material Particulado/análise , Emissões de Veículos/análise , Ar/normas , Estados Unidos
5.
J Air Waste Manag Assoc ; 55(11): 1683-93, 2005 Nov.
Artigo em Inglês | MEDLINE | ID: mdl-16350366

RESUMO

Version 4.10s of the comprehensive air-quality model with extensions (CAMx) photochemical grid model has been developed, which includes two options for representing particulate matter (PM) size distribution: (1) a two-section representation that consists of fine (PM2.5) and coarse (PM2.5-10) modes that has no interactions between the sections and assumes all of the secondary PM is fine; and (2) a multisectional representation that divides the PM size distribution into N sections (e.g., N = 10) and simulates the mass transfer between sections because of coagulation, accumulation, evaporation, and other processes. The model was applied to Southern California using the two-section and multisection representation of PM size distribution, and we found that allowing secondary PM to grow into the coarse mode had a substantial effect on PM concentration estimates. CAMx was then applied to the Western United States for the 1996 annual period with a 36-km grid resolution using both the two-section and multisection PM representation. The Community Multiscale Air Quality (CMAQ) and Regional Modeling for Aerosol and Deposition (REMSAD) models were also applied to the 1996 annual period. Similar model performance was exhibited by the four models across the Interagency Monitoring of Protected Visual Environments (IMPROVE) and Clean Air Status and Trends Network monitoring networks. All four of the models exhibited fairly low annual bias for secondary PM sulfate and nitrate but with a winter overestimation and summer underestimation bias. The CAMx multisectional model estimated that coarse mode secondary sulfate and nitrate typically contribute <10% of the total sulfate and nitrate when averaged across the more rural IMPROVE monitoring network.


Assuntos
Poluentes Ocupacionais do Ar/análise , Poluição do Ar/análise , Oxidantes Fotoquímicos/análise , Algoritmos , California , Carbono/análise , Monitoramento Ambiental , Modelos Estatísticos , Nitratos/análise , Sudoeste dos Estados Unidos
6.
J Air Waste Manag Assoc ; 55(11): 1694-708, 2005 Nov.
Artigo em Inglês | MEDLINE | ID: mdl-16350367

RESUMO

The Visibility Improvement State and Tribal Association of the Southeast (VISTAS) is one of five Regional Planning Organizations that is charged with the management of haze, visibility, and other regional air quality issues in the United States. The VISTAS Phase I work effort modeled three episodes (January 2002, July 1999, and July 2001) to identify the optimal model configuration(s) to be used for the 2002 annual modeling in Phase II. Using model configurations recommended in the Phase I analysis, 2002 annual meteorological (Mesoscale Meterological Model [MM5]), emissions (Sparse Matrix Operator Kernal Emissions [SMOKE]), and air quality (Community Multiscale Air Quality [CMAQ]) simulations were performed on a 36-km grid covering the continental United States and a 12-km grid covering the Eastern United States. Model estimates were then compared against observations. This paper presents the results of the preliminary CMAQ model performance evaluation for the initial 2002 annual base case simulation. Model performance is presented for the Eastern United States using speciated fine particle concentration and wet deposition measurements from several monitoring networks. Initial results indicate fairly good performance for sulfate with fractional bias values generally within +/-20%. Nitrate is overestimated in the winter by approximately +50% and underestimated in the summer by more than -100%. Organic carbon exhibits a large summer underestimation bias of approximately -100% with much improved performance seen in the winter with a bias near zero. Performance for elemental carbon is reasonable with fractional bias values within +/- 40%. Other fine particulate (soil) and coarse particular matter exhibit large (80-150%) overestimation in the winter but improved performance in the summer. The preliminary 2002 CMAQ runs identified several areas of enhancements to improve model performance, including revised temporal allocation factors for ammonia emissions to improve nitrate performance and addressing missing processes in the secondary organic aerosol module to improve OC performance.


Assuntos
Poluição do Ar/análise , Ar/normas , Modelos Estatísticos , Nitratos/análise , Sudeste dos Estados Unidos
7.
Am J Emerg Med ; 20(1): 14-7, 2002 Jan.
Artigo em Inglês | MEDLINE | ID: mdl-11781905

RESUMO

As the elderly population increases and they lead more active and healthy lifestyles, their exposure to the threats of injury multiply. Undoubtedly, the geriatric population will comprise a growing percentage of trauma patients. The role of alcohol and drug use in geriatric trauma has not been clearly defined. The purpose of this study is to determine the incidence of alcohol and illicit drug use in association with mechanism of injury in all elderly trauma patients presenting to level I and II trauma centers in the State of Illinois over 3 years. A retrospective analysis was performed on 3 years of data (January 1, 1994 to December 31, 1996), provided by the Illinois Department of Public Health as the Illinois Trauma Registry, which describes consecutive trauma patients presenting to level I and II trauma facilities in the State of Illinois. During the study period, there were a total of 134,846 trauma patient entries. Of these 32,382 (24.0%) were for patients 65 years of age or older. In those patients 65 and older, 1699 (5.2%) were tested for the presence of alcohol and 845 (49.7%) tested positive. Of the elderly patients who tested positive for alcohol, 71.8% were considered intoxicated (BAC >80 mg/dL). Urine toxicology screens were performed on 1785 (5.5%) elderly trauma patients, and 208 (11.6%) were positive. Besides alcohol, benzodiazipines and opiates were the most frequently detected drugs. For elderly patients under the influence of alcohol falls (49.5%) and motor vehicle crashes (36.7%) were the most common mechanism of injury. For geriatric patients testing negative for alcohol, motor vehicle crashes were a much more common mechanism of injury than falls (65.0% v 25.1%). Falls were a much more common cause of injury in elderly patients using alcohol than in those not using alcohol. Alcohol and substance abuse are possibly significant factors in geriatric trauma. Although only 5% of elderly trauma patients were tested for alcohol, nearly half had alcohol present on presentation to a trauma center, and the majority of these patients were intoxicated. Prospective studies are needed to determine the true incidence of alcohol use/abuse in the geriatric trauma population and the need for routine alcohol screening of these patients. Detection of alcohol abuse in elderly trauma patients could help identify individuals in need of counseling and rehabilitative treatment. It may also reduce future injuries in these patients.


Assuntos
Intoxicação Alcoólica/epidemiologia , Transtornos Relacionados ao Uso de Substâncias/epidemiologia , Ferimentos e Lesões/epidemiologia , Acidentes por Quedas/estatística & dados numéricos , Acidentes de Trânsito/estatística & dados numéricos , Idoso , Feminino , Humanos , Illinois/epidemiologia , Incidência , Masculino , Estudos Retrospectivos , Suicídio/estatística & dados numéricos , Violência/estatística & dados numéricos
8.
J Law Med Ethics ; 30(3 Suppl): 48-51, 2002.
Artigo em Inglês | MEDLINE | ID: mdl-12508502

RESUMO

Work has been underway nationally since the mid-1990s to equip state and community public health systems with the infrastructure needed to perform essential public health services. Key components of that infrastructure are a competent workforce, information and communication systems, health department and laboratory capacity, and legal authorities. As part of this transformative work, standards and assessment tools have been developed to measure the capacity and actual performance of public health systems. In addition, a number of states have examined the legal foundation for public health services and have revised and updated those authorities to improve their system's capacity in the context of evolving health challenges. Among those states are Nebraska, New Jersey, and Texas, all of which, beginning in 1999, have adopted dynamic new approaches to aligning public health's legal authorities with new missions and expectations for performance and accountability. This article describes the approaches that these three states have taken to strengthen their legal foundation for public health practice, to illuminate the perspectives legislators and health officials bring to the process, and to give decision makers in other states practical insight into the potential benefits of reviewing and restructuring public health's legal authorities. The underlying stimuli for the states' initiatives differed significantly, yet shared an important, common core. What they held in common was concern that outdated elements of the public health system and infrastructure hindrered delivery of essential public health services at the community level. Where they differed was in the type of tools they found most suitable for the job of rejuvenating those structures. The approaches taken, and the policy tools selected, reflect the unique health needs of each state, establish relationships among state and community health authorities and agencies, and provide guidance by elected and appointed policy makers. Each state continues to refine its approach as it gains experience with the new authorities.


Assuntos
Serviços de Saúde Comunitária/legislação & jurisprudência , Administração em Saúde Pública/legislação & jurisprudência , Saúde Pública/legislação & jurisprudência , Planos Governamentais de Saúde/legislação & jurisprudência , Serviços de Saúde Comunitária/economia , Tomada de Decisões Gerenciais , Necessidades e Demandas de Serviços de Saúde , Humanos , Nebraska , New Jersey , Objetivos Organizacionais , Saúde Pública/economia , Administração em Saúde Pública/economia , Planos Governamentais de Saúde/economia , Texas , Estados Unidos , United States Dept. of Health and Human Services
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