Macroscopic discontinuous shear thickening versus local shear jamming in cornstarch.

We study the emergence of discontinuous shear thickening (DST) in cornstarch by combining macroscopic rheometry with local magnetic resonance imaging measurements. We bring evidence that macroscopic DST is observed only when the flow separates into a low-density flowing and a high-density jammed region. In the shear-thickened steady state, the local rheology in the flowing region is not DST but, strikingly, is often shear thinning. Our data thus show that the stress jump measured during DST, in cornstarch, does not capture a secondary, high-viscosity branch of the local steady rheology but results from the existence of a shear jamming limit at volume fractions quite significantly below random close packing.

Solid-liquid transition and rejuvenation similarities in complex flows of thixotropic materials studied by NMR and MRI.

We study the flow of a typical thixotropic material subjected to very different deformation histories (squeeze, shear, and extrusion) with either local (proton NMR and magnetic resonance imaging) or macroscopic measurements after different times of rest. Specifically, we measure the velocity fields and the spin-spin NMR relaxation of the material after different flow histories. The relaxation data exhibits a long relaxing component revealing information about the reversible microstructural evolution of the sample during aging-rejuvenation cycles. We show that for each deformation process, the evolution of the viscosity during the solid-liquid transition is similar by a factor related to the initial state of the material. Moreover, results examining the impact of the rate at which the deformation is imposed suggest that the state of the material during this transition may be described by a single parameter reflecting the average size and deformation of the material's flocs. These results also show that localization of flow occurs as a result of a progressive differential evolution of the material in different regions of the flow, and thus are determined by the boundary conditions of the flow.

Coexistence of liquid and solid phases in flowing soft-glassy materials.

Magnetic-resonance-imaging rheometrical experiments show that concentrated suspensions or emulsions cannot flow steadily at a uniform rate smaller than a critical value (gamma(c)). As a result, a "liquid" region (sheared rapidly, i.e., at a rate larger than gamma(c)) and a "solid" region (static) coexist. The behavior of the fluid in the liquid region follows a simple power-law model, while the extent of the solid region increases with the degree of jamming of the material.

Liquid Bridge between Two Moving Spheres: An Experimental Study of Viscosity Effects.

The effects of viscosity on the mechanical response of a liquid bridge are investigated in the case of small amounts of liquid axially strained between two moving spheres. An experimental setup allows the measurement of capillary and viscous forces exerted on the spheres as a function of the spheres separation distance and the spheres velocity. The experimental results are found to be accurately described over a large range in spheres velocity and liquid viscosity by a simple closed-form expression. In addition, the bridge rupture distance is found to increase like the square root of the separation velocity. Copyright 2000 Academic Press.