Fabrication and characterization of iodine photonic microcells for sub-Doppler spectroscopy applications.

We report on the development of all-fiber stand-alone iodine-filled photonic microcells demonstrating record absorption contrast at room temperature. The microcell's fiber is made of inhibited coupling guiding hollow-core photonic crystal fibers. The fiber-core loading with iodine was undertaken at 10-1-10-2mbar vapor pressure using what, to the best of our knowledge, is a novel gas-manifold based on metallic vacuum parts with ceramic coated inner surfaces for corrosion resistance. The fiber is then sealed on the tips and mounted on FC/APC connectors for better integration with standard fiber components. The stand-alone microcells display Doppler lines with contrasts up to 73% in the 633 nm wavelength range, and an off-resonance insertion loss between 3 to 4 dB. Sub-Doppler spectroscopy based on saturable absorption has been carried out to resolve the hyperfine structure of the P(33)6-3 lines at room temperature with a full-width at half maximum of 24 MHz on the b4 component with the help of lock-in amplification. Also, we demonstrate distinguishable hyperfine components on the R(39)6-3 line at room temperature without any recourse to signal-to-noise ratio amplification techniques.

Λ-enhanced grey molasses on the D2 transition of Rubidium-87 atoms.

Laser cooling based on dark states, i.e. states decoupled from light, has proven to be effective to increase the phase-space density of cold trapped atoms. Dark-states cooling requires open atomic transitions, in contrast to the ordinary laser cooling used for example in magneto-optical traps (MOTs), which operate on closed atomic transitions. For alkali atoms, dark-states cooling is therefore commonly operated on the D1 transition nS1/2 → nP1/2. We show that, for 87Rb, thanks to the large hyperfine structure separations the use of this transition is not strictly necessary and that "quasi-dark state" cooling is efficient also on the D2 line, 5S1/2 → 5P3/2. We report temperatures as low as (4.0 ± 0.3) µK and an increase of almost an order of magnitude in the phase space density with respect to ordinary laser sub-Doppler cooling.