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1.
Phys Rev Lett ; 132(22): 226503, 2024 May 31.
Artigo em Inglês | MEDLINE | ID: mdl-38877957

RESUMO

We present experimental evidence that a heavy Fermi surface consisting of itinerant, charge-neutral spinons underpins both heavy-fermion-strange-metal (without f electrons) and quantum-spin-liquid states in the 4d-electron trimer lattice, Ba_{4}Nb_{1-x}Ru_{3+x}O_{12}(|x|<0.20). These two exotic states both exhibit an extraordinarily large entropy, a linear heat capacity extending into the milli-Kelvin regime, a linear thermal conductivity at low temperatures, and separation of charges and spins. Furthermore, the insulating spin liquid is a much better thermal conductor than the heavy-fermion-strange-metal that separately is observed to strongly violate the Wiedemann-Franz law. We propose that at the heart of this 4d system is a universal, heavy spinon Fermi surface that provides a unified framework for explaining the exotic phenomena observed throughout the entire series. The control of such exotic ground states provided by variable Nb concentration offers a new paradigm for studies of correlated quantum matter.

2.
Nat Commun ; 15(1): 3579, 2024 Apr 27.
Artigo em Inglês | MEDLINE | ID: mdl-38678048

RESUMO

Chiral orbital currents (COC) underpin a novel colossal magnetoresistance in ferrimagnetic Mn3Si2Te6. Here we report the Hall effect in the COC state which exhibits the following unprecedented features: (1) A sharp, current-sensitive peak in the magnetic field dependence of the Hall resistivity, and (2) A current-sensitive scaling relation between the Hall conductivity σxy and the longitudinal conductivity σxx, namely, σxy ∝ σxxα with α reaching up to 5, which is exceptionally large compared to α ≤ 2 typical of all solids. The novel Hall responses along with a current-sensitive carrier density and a large Hall angle of 15% point to a giant, current-sensitive Hall effect that is unique to the COC state. Here, we show that a magnetic field induced by the fully developed COC combines with the applied magnetic field to exert the greatly enhanced transverse force on charge carriers, which dictates the COC Hall responses.

4.
Phys Rev Lett ; 132(4): 040401, 2024 Jan 26.
Artigo em Inglês | MEDLINE | ID: mdl-38335344

RESUMO

We present a new route to ergodicity breaking via Hilbert space fragmentation that displays an unprecedented level of robustness. Our construction relies on a single emergent (prethermal) conservation law. In the limit when the conservation law is exact, we prove the emergence of Hilbert space fragmentation with an exponential number of frozen configurations. These configurations are low-entanglement states in the middle of the energy spectrum and therefore constitute examples of quantum many-body scars. We further prove that every frozen configuration is absolutely stable to arbitrary perturbations, to all finite orders in perturbation theory. In contrast to previous constructions, our proof is not limited to symmetric perturbations, or to perturbations with compact support, but also applies to perturbations with long-range tails, and even to arbitrary geometrically nonlocal k-body perturbations, as long as k/L→0 in the thermodynamic limit, where L is linear system size. Additionally, we identify one-form U(1) charges characterizing some nonfrozen sectors, and discuss the dynamics starting from typical initial conditions, which we argue is best interpreted in terms of the magnetohydrodynamics of the emergent one-form symmetry.

5.
Nano Lett ; 23(18): 8392-8398, 2023 Sep 27.
Artigo em Inglês | MEDLINE | ID: mdl-37682637

RESUMO

The origin of the pseudogap in many strongly correlated materials has been a longstanding puzzle. Here, we present experimental evidence that many-body interactions among small Holstein polarons, i.e., the formation of bipolarons, are primarily responsible for the pseudogap in (TaSe4)2I. After weak photoexcitation of the material, we observe the appearance of both dispersive (single-particle bare band) and flat bands (single-polaron sub-bands) in the gap by using time- and angle-resolved photoemission spectroscopy. Based on Monte Carlo simulations of the Holstein model, we propose that the melting of pseudogap and emergence of new bands originate from a bipolaron to single-polaron crossover. We also observe dramatically different relaxation times for the excited in-gap states in (TaSe4)2I (∼600 fs) compared with another 1D material Rb0.3MoO3 (∼60 fs), which provides a new method for distinguishing between pseudogaps induced by polaronic or Luttinger-liquid many-body interactions.

6.
Phys Rev E ; 105(4-1): 044103, 2022 Apr.
Artigo em Inglês | MEDLINE | ID: mdl-35590640

RESUMO

We show that the simplest universality classes of fracton hydrodynamics in more than one spatial dimension, including isotropic theories of charge and dipole conservation, can exhibit hidden quasiconservation laws, in which certain higher multipole moments can only decay due to dangerously irrelevant corrections to hydrodynamics. We present two simple examples of this phenomenon. First, an isotropic dipole-conserving fluid in the infinite plane conserves an infinite number of harmonic multipole charges within linear response; we calculate the decay or growth of these charges due to dangerously irrelevant nonlinearities. Second, we consider a model with xy and x^{2}-y^{2} quadrupole conservation, in addition to dipole conservation, which is described by isotropic fourth-order subdiffusion, yet has dangerously irrelevant sixth-order corrections necessary to relax the harmonic multipole charges. We confirm our predictions for the anomalously slow decay of the harmonic conserved charges in each setting by using numerical simulations, both of the nonlinear hydrodynamic differential equations, and in quantum automaton circuits on a square lattice.

7.
Phys Rev E ; 103(2-1): 022142, 2021 Feb.
Artigo em Inglês | MEDLINE | ID: mdl-33736028

RESUMO

Subdiffusion is a generic feature of chaotic many-body dynamics with multipole conservation laws and subsystem symmetries. We numerically study this subdiffusive dynamics, using quantum automaton random unitary circuits, in a broad range of models including one-dimensional models with dipole and quadrupole conservation, two-dimensional models with dipole conservation, and two-dimensional models with subsystem symmetry on the triangular lattice. Our results are in complete agreement with recent hydrodynamic predictions for such theories.

8.
Nat Commun ; 11(1): 2548, 2020 May 21.
Artigo em Inglês | MEDLINE | ID: mdl-32439836

RESUMO

Measurement and control of magnetic order and correlations in real time is a rapidly developing scientific area relevant for magnetic memory and spintronics. In these experiments an ultrashort laser pulse (pump) is first absorbed by excitations carrying electric dipole moment. These then give their energy to the magnetic subsystem monitored by a time-resolved probe. A lot of progress has been made in investigations of ferromagnets but antiferromagnets are more challenging. Here, we introduce time-resolved two-magnon Raman scattering as a real time probe of magnetic correlations especially well-suited for antiferromagnets. Its application to the antiferromagnetic charge transfer insulator YBa2Cu3O6.1 revealed rapid demagnetization within 90 fs of photoexcitation. The relaxation back to thermal equilibrium is characterized by much slower timescales. We interpret these results in terms of slow relaxation of the charge sector and rapid equilibration of the magnetic sector to a prethermal state characterized by parameters that change slowly as the charge sector relaxes.

9.
Phys Rev Lett ; 123(13): 130402, 2019 Sep 27.
Artigo em Inglês | MEDLINE | ID: mdl-31697521

RESUMO

We study a driven, spin-orbit coupled fermionic system in a lattice at the resonant regime where the drive frequency equals the Hubbard repulsion, for which nontrivial constrained dynamics emerge at fast timescales. An effective density-dependent tunneling model is derived, and it is examined in the sparse filling regime in one dimension. The system exhibits entropic self-localization, where while even numbers of atoms propagate ballistically, odd numbers form localized bound states induced by an effective attraction from a higher configurational entropy. These phenomena occur in the strong coupling limit where interactions impose only a constraint with no explicit Hamiltonian term. We show how the constrained dynamics lead to quantum few-body scars and map to an Anderson impurity model with an additional intriguing feature of nonreciprocal scattering. Connections to many-body scars and localization are also discussed.

10.
Proc Natl Acad Sci U S A ; 115(42): 10570-10575, 2018 10 16.
Artigo em Inglês | MEDLINE | ID: mdl-30282733

RESUMO

The rapidly expanding class of quantum materials known as topological semimetals (TSMs) displays unique transport properties, including a striking dependence of resistivity on applied magnetic field, that are of great interest for both scientific and technological reasons. So far, many possible sources of extraordinarily large nonsaturating magnetoresistance have been proposed. However, experimental signatures that can identify or discern the dominant mechanism and connect to available theories are scarce. Here we present the magnetic susceptibility (χ), the tangent of the Hall angle ([Formula: see text]), along with magnetoresistance in four different nonmagnetic semimetals with high mobilities, NbP, TaP, NbSb2, and TaSb2, all of which exhibit nonsaturating large magnetoresistance (MR). We find that the distinctly different temperature dependences, [Formula: see text], and the values of [Formula: see text] in phosphides and antimonates serve as empirical criteria to sort the MR from different origins: NbP and TaP are uncompensated semimetals with linear dispersion, in which the nonsaturating magnetoresistance arises due to guiding center motion, while NbSb2 and TaSb2 are compensated semimetals, with a magnetoresistance emerging from nearly perfect charge compensation of two quadratic bands. Our results illustrate how a combination of magnetotransport and susceptibility measurements may be used to categorize the increasingly ubiquitous nonsaturating large magnetoresistance in TSMs.

11.
Phys Rev Lett ; 114(11): 117401, 2015 Mar 20.
Artigo em Inglês | MEDLINE | ID: mdl-25839306

RESUMO

We use numerical exact diagonalization to analyze which aspects of the many-body localization phenomenon survive in an imperfectly isolated setting, when the system of interest is weakly coupled to a thermalizing environment. We show that widely used diagnostics (such as many-body level statistics and expectation values in exact eigenstates) cease to show signatures of many-body localization above a critical coupling that is exponentially small in the size of the environment. However, we also identify alternative diagnostics for many-body localization, in the spectral functions of local operators. Diagnostics include a discrete spectrum and a hierarchy of energy gaps, including a universal gap at zero frequency. These alternative diagnostics are shown to be robust, and continue to show signatures of many-body localization as long as the coupling to the bath is weaker than the characteristic energy scales in the system. We also examine how these signatures disappear when the coupling to the environment becomes larger than the characteristic energy scales of the system.

12.
Phys Rev Lett ; 108(22): 227204, 2012 Jun 01.
Artigo em Inglês | MEDLINE | ID: mdl-23003647

RESUMO

We consider electrons on a honeycomb or triangular lattice doped to the saddle point of the band structure. We assume the system parameters are such that spin density wave (SDW) order emerges below a temperature T(N) and investigate the nature of the SDW phase. We argue that at T≤T(N), the system develops a uniaxial SDW phase whose ordering pattern breaks O(3)×Z(4) symmetry and corresponds to an eight-site unit cell with nonuniform spin moments on different sites. This state is a half-metal--it preserves the full original Fermi surface, but has gapless charged excitations in one spin branch only. It allows for electrical control of spin currents and is desirable for nanoscience.

13.
Phys Rev Lett ; 107(9): 097402, 2011 Aug 26.
Artigo em Inglês | MEDLINE | ID: mdl-21929269

RESUMO

The unique sensitivity of optical response to different types of symmetry breaking can be used to detect and identify spontaneously ordered many-body states in bilayer graphene. We predict a strong response at optical frequencies, sensitive to electronic phenomena at low energies, which arises because of nonzero interband matrix elements of the electric current operator. In particular, the polar Kerr rotation and reflection anisotropy provide fingerprints of the quantum anomalous Hall state and the nematic state, characterized by spontaneously broken time-reversal symmetry and lattice rotation symmetry, respectively. These optical signatures, which undergo a resonant enhancement in the near-infrared regime, lie well within reach of existing experimental techniques.

14.
Proc Natl Acad Sci U S A ; 108(34): 14021-5, 2011 Aug 23.
Artigo em Inglês | MEDLINE | ID: mdl-21825159

RESUMO

Interference and tunneling are two signature quantum effects that are often perceived as the yin and yang of quantum mechanics: a particle simultaneously propagating along several distinct classical paths versus a particle penetrating through a classically inaccessible region via a single least-action path. Here we demonstrate that the Dirac quasiparticles in graphene provide a dramatic departure from this paradigm. We show that Zener tunneling in gapped bilayer graphene, which governs transport through p-n heterojunctions, exhibits common-path interference that takes place under the tunnel barrier. Due to a symmetry peculiar to the gapped bilayer graphene bandstructure, interfering tunneling paths form conjugate pairs, giving rise to high-contrast oscillations in transmission as a function of the gate-tunable bandgap and other control parameters of the junction. The common-path interference is solely due to forward-propagating waves; in contrast to Fabry-Pérot-type interference in resonant-tunneling structures, it does not rely on multiple backscattering. The oscillations manifest themselves in the junction I-V characteristic as N-shaped branches with negative differential conductivity. The negative dI/dV, which arises solely due to under-barrier interference, can enable new high-speed active-circuit devices with architectures that are not available in electronic semiconductor devices.

15.
Phys Rev Lett ; 104(15): 156803, 2010 Apr 16.
Artigo em Inglês | MEDLINE | ID: mdl-20482006

RESUMO

Electron interactions in undoped bilayer graphene lead to an instability of the gapless state, "which-layer" symmetry breaking, and energy gap opening at the Dirac point. In contrast with single-layer graphene, the bilayer system exhibits instability even for an arbitrarily weak interaction. A controlled theory of this instability for realistic dynamically screened Coulomb interactions is developed, with full account of the dynamically generated ultraviolet cutoff. This leads to an energy gap that scales as a power law of the interaction strength, making the excitonic instability readily observable.

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