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1.
Artigo em Inglês | MEDLINE | ID: mdl-37044113

RESUMO

Electric field control of magnetodynamics in magnetoelectric (ME) heterostructures has been the subject of recent interest due to its fundamental complexity and promising applications in room temperature devices. The present work focuses on the tuning of magnetodynamic parameters of epitaxially grown ferromagnetic (FM) La0.7Sr0.3MnO3(LSMO) on a ferro(piezo)electric (FE) Pb(Mg0.33Nb0.67)O3-PbTiO3(PMN-PT) single crystal substrate. The uniaxial magnetic anisotropy of LSMO on PMN-PT confirms the ME coupling at the FM/FE heterointerface. The magnitude of the Gilbert damping constant (α) of this uniaxial LSMO film measured along the hard magnetic axis is significantly small compared to the easy axis. Furthermore, a marked decrease in the α values of LSMO at positive and negative electrical remanence of PMN-PT is observed, which is interpreted in the framework of strain induced spin dependent electronic structure. The present results clearly encourage the prospects of electric field controlled magnetodynamics, thereby realising the room temperature spin-wave based device applications with ultra-low power consumption.

2.
ACS Appl Mater Interfaces ; 12(26): 29971-29978, 2020 Jul 01.
Artigo em Inglês | MEDLINE | ID: mdl-32490655

RESUMO

Parasitic magnetism plays an important role in magnetoelectric spin switching of antiferromagnetic oxides, but its mechanism has not been clearly investigated. Unlike the widely obtained surface boundary magnetization in magnetoelectric Cr2O3 antiferromagnet, we previously reported that Al doping could produce volume-dependent parasitic magnetism (Mpara) in Cr2O3 with the remaining magnetoelectric effect and antiferromagnetic properties. In this work, we systematically investigated the magnetic properties of Mpara in Cr2O3 through its different exchange coupling characteristics with the ferromagnet at various conditions. The columnar grain boundaries cause an antiferromagnetic sublattice breaking to produce uncompensated spins and thus are considered to be responsible for Mpara in both undoped and Al-doped Cr2O3. Finally, a model was proposed for the formation mechanism of the parasitic magnetism in Cr2O3, which explains the reported magnetic characteristics of Cr2O3, and some current topics such as the domain formation and motion in Cr2O3 during magnetoelectric spin switching. This work contributes to a deep understanding of antiferromagnetic spintronics and provides a method to realize the low-energy operation of antiferromagnetic-based magnetic random access memory.

3.
Phys Chem Chem Phys ; 18(22): 15218-22, 2016 06 01.
Artigo em Inglês | MEDLINE | ID: mdl-27212586

RESUMO

Niobium carbide (NbC) nanoparticles embedded on the surface of carbon spheres (CS) were synthesized at 1350 °C by the carbothermal reduction of niobium oxide precursor in flowing argon (Nbc@CS). The morphology, crystal structure, and magnetic properties of the hybrid nanocomposite were investigated by means of electron microscopy, X-ray diffraction and a superconducting quantum interference device. It was found that the NbC@CS nanocomposites exhibit type-II superconductivity with a critical temperature (Tc) of 8-12 K, typical for stoichiometric NbC. The superconducting hysteresis loop reveals several interesting traits, including strong vortex pinning, the presence of asymmetry and a high penetration field. Moreover, the sample shows much improved irreversible (Hirr), lower (Hc1) and upper (Hc2) critical fields. The coherence length (ξ), penetration depth (λ), and Ginzburg-Landau (κ) parameters for the sample were estimated to be 9.78 nm, 33 nm and 3.39, respectively.

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