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1.
Nano Lett ; 24(22): 6538-6544, 2024 Jun 05.
Artigo em Inglês | MEDLINE | ID: mdl-38771703

RESUMO

With a seminal work of Raghu and Haldane in 2008, concepts of topology have been introduced into optical systems, where some of the most promising routes to an application are efficient and highly coherent topological lasers. While some attempts have been made to excite such structures electrically, the majority of published experiments use a form of laser excitation. In this paper, we use a lattice of vertical resonator polariton micropillars to form an exponentially localized topological Su-Schrieffer-Heeger defect. Upon electrical excitation, the system unequivocally shows polariton lasing from the topological defect using a carefully placed gold contact. Despite the presence of doping and electrical contacts, the polariton band structure clearly preserves its topological properties. At high excitation power the Mott density is exceeded, leading to highly efficient lasing in the weak coupling regime. This work is an important step toward applied topological lasers using vertical resonator microcavity structures.

2.
Opt Express ; 32(4): 5088-5094, 2024 Feb 12.
Artigo em Inglês | MEDLINE | ID: mdl-38439244

RESUMO

Two-dimensional transition metal dichalcogenides have shown large second-order nonlinear responses due to their broken crystal inversion symmetry. However, their nonlinear interaction with light is restricted to an atomically thin layer. Placing a sheet of transition metal dichalcogenides on a resonant metasurface enhances the field interacting with the nonlinear material thus compensating for this shortcoming. But, it remains a challenge to tune resonances such, that they coincide with fundamental and second harmonic frequencies simultaneously. Here we demonstrate two independent methods to achieve that goal and numerically illustrate our findings for a MoS2 layer combined with silicon nitride photonic crystals. We numerically demonstrate 20-fold and 170-fold enhancement of second-harmonic generation compared with a design based on a single resonant structure. Although we focus on that specific configuration our approach can likewise be applied to other dielectrics combined with highly nonlinear 2D materials.

3.
Small ; 19(37): e2301126, 2023 Sep.
Artigo em Inglês | MEDLINE | ID: mdl-37226688

RESUMO

With conventional electronics reaching performance and size boundaries, all-optical processes have emerged as ideal building blocks for high speed and low power consumption devices. A promising approach in this direction is provided by valleytronics in atomically thin semiconductors, where light-matter interaction allows to write, store, and read binary information into the two energetically degenerate but non-equivalent valleys. Here, nonlinear valleytronics in monolayer WSe2 is investigated and show that an individual ultrashort pulse with a photon energy tuned to half of the optical band-gap can be used to simultaneously excite (by coherent optical Stark shift) and detect (by a rotation in the polarization of the emitted second harmonic) the valley population.

4.
Opt Express ; 31(2): 3364-3378, 2023 Jan 16.
Artigo em Inglês | MEDLINE | ID: mdl-36785331

RESUMO

Semiconductor nanowire lasers can be subject to modifications of their lasing threshold resulting from a variation of their environment. A promising choice is to use metallic substrates to gain access to low-volume Surface-Plasmon-Polariton (SPP) modes. We introduce a simple, yet quantitatively precise model that can serve to describe mode competition in nanowire lasers on metallic substrates. We show that an aluminum substrate can decrease the lasing threshold for ZnO nanowire lasers while for a silver substrate, the threshold increases compared with a dielectric substrate. Generalizing from these findings, we make predictions describing the interaction between planar metals and semiconductor nanowires, which allow to guide future improvements of highly-integrated laser sources.

5.
Phys Rev Lett ; 127(16): 163901, 2021 Oct 15.
Artigo em Inglês | MEDLINE | ID: mdl-34723580

RESUMO

Hydrodynamic phenomena can be observed with light thanks to the analogy between quantum gases and nonlinear optics. In this Letter, we report an experimental study of the superfluid-like properties of light in a (1+1)-dimensional nonlinear optical mesh lattice, where the arrival time of optical pulses plays the role of a synthetic spatial dimension. A spatially narrow defect at rest is used to excite sound waves in the fluid of light and measure the sound speed. The critical velocity for superfluidity is probed by looking at the threshold in the deposited energy by a moving defect, above which the apparent superfluid behavior breaks down. Our observations establish optical mesh lattices as a promising platform to study fluids of light in novel regimes of interdisciplinary interest, including non-Hermitian and/or topological physics.

6.
Sci Rep ; 9(1): 9518, 2019 Jul 02.
Artigo em Inglês | MEDLINE | ID: mdl-31267020

RESUMO

Power induced wave collapse is one of the most fascinating phenomena in optics as it provides extremely high intensities, thus stimulating a range of nonlinear processes. For low power levels, propagation of beams in bulk media is dominated by diffraction, while above a certain threshold self-focusing is steadily enhanced by the action of a positive nonlinearity. An autocatalytic blow-up occurs, which is only stopped by saturation of the nonlinearity, material damage or the inherent medium discreteness. In the latter case, this leads to energy localization on a single site. It is commonly believed that for cubic nonlinearities, this intriguing effect requires at least two transverse dimensions to occur and is thus out of reach in fiber optics. Following the concept of synthetic dimensions, we demonstrate that mixing short and long-range interaction resembles a two-dimensional mesh lattice and features wave collapse at mW-power levels in a genuine 1D system formed by coupled fiber loops.

7.
Opt Lett ; 44(24): 6013-6016, 2019 Dec 15.
Artigo em Inglês | MEDLINE | ID: mdl-32628207

RESUMO

We experimentally demonstrate the transverse confinement of light in the presence of a longitudinally periodic photonic potential with vanishing average. In agreement with Kapitza's original findings in classical mechanics, we confirm that light undergoes a transverse localization due to the action of an effective potential proportional to the square of the first derivative of the potential. Experiments are performed based on (1+1) D synthetic dimensions realized in a fiber loop system, allowing for complete control of the transverse and longitudinal distributions of the potential.

8.
Phys Rev Lett ; 123(25): 253903, 2019 Dec 20.
Artigo em Inglês | MEDLINE | ID: mdl-31922782

RESUMO

Over the last few years, parity-time (PT) symmetry has been the focus of considerable attention. Ever since, pseudo-Hermitian notions have permeated a number of fields ranging from optics to atomic and topological physics, as well as optomechanics, to mention a few. Unlike their Hermitian counterparts, nonconservative systems do not exhibit a priori real eigenvalues and hence unitary evolution. However, once PT symmetry is introduced, such dissipative systems can surprisingly display a real eigenspectrum, thus ensuring energy conservation during evolution. In optics, PT symmetry can be readily established by incorporating, in a balanced way, regions having an equal amount of optical gain and loss. However, thus far, all optical realizations of such PT symmetry have been restricted to a single transverse dimension (1D), such as arrays of optical waveguides or active coupled cavity arrangements. In most cases, only the loss function was modulated-a restrictive aspect that is only appropriate for linear systems. Here, we present an experimental platform for investigating the interplay between PT symmetry and nonlinearity in two-dimensional (2D) environments, where nonlinear localization and soliton formation can be observed. In contrast to typical dissipative solitons, we demonstrate a one-parameter family of soliton solutions that are capable of displaying attributes similar to those encountered in nonlinear conservative arrangements. For high optical powers, this new family of PT solitons tends to collapse on a discrete network-thus giving rise to an amplified, self-accelerating structure.

9.
Sci Rep ; 8(1): 2125, 2018 02 01.
Artigo em Inglês | MEDLINE | ID: mdl-29391523

RESUMO

As time flow dictates all evolution, its effective reversal is a topic of active research in a broad range of disciplines, including acoustics, hydrodynamics and optics. This multifarious set of environments is reflected by a great diversity of approaches to observe various echoes of wave functions. Here, we experimentally demonstrate time reversal of a pulse sequence propagating through a photonic mesh lattice realized by two coupled loops of telecommunication fibres. Our system features a symmetric band structure, which allows for almost perfect reversal of its evolution by exchanging the population between two opposing bands. The protocol applied is based on a non-adiabatic and instantaneous exchange of eigenstates resulting in highly efficient time reversal of a pulse chain.

10.
Sci Rep ; 6: 27264, 2016 06 09.
Artigo em Inglês | MEDLINE | ID: mdl-27277521

RESUMO

The interaction of light with matter strongly depends on the structure of the latter at wavelength scale. Ordered systems interact with light via collective modes, giving rise to diffraction. In contrast, completely disordered systems are dominated by Mie resonances of individual particles and random scattering. However, less clear is the transition regime in between these two extremes, where diffraction, Mie resonances and near-field interaction between individual scatterers interplay. Here, we probe this transitional regime by creating colloidal crystals with controlled disorder from two-dimensional self-assembly of bidisperse spheres. Choosing the particle size in a way that the small particles are transparent in the spectral region of interest enables us to probe in detail the effect of increasing positional disorder on the optical properties of the large spheres. With increasing disorder a transition from a collective optical response characterized by diffractive resonances to single particles scattering represented by Mie resonances occurs. In between these extremes, we identify an intermediate, hopping-like light transport regime mediated by resonant interactions between individual spheres. These results suggest that different levels of disorder, characterized not only by absence of long range order but also by differences in short-range correlation and interparticle distance, exist in colloidal glasses.

11.
Nano Lett ; 16(4): 2878-84, 2016 Apr 13.
Artigo em Inglês | MEDLINE | ID: mdl-27007261

RESUMO

Coherent light sources confining the light below the vacuum wavelength barrier will drive future concepts of nanosensing, nanospectroscopy, and photonic circuits. Here, we directly image the angular emission of such a light source based on single semiconductor nanowire lasers. It is confirmed that the lasing switches from the fundamental mode in a thin ZnO nanowire to an admixture of several transverse modes in thicker nanowires approximately at the multimode cutoff. The mode competition with higher order modes substantially slows down the laser dynamics. We show that efficient photonic mode filtering in tapered nanowires selects the desired fundamental mode for lasing with improved performance including power, efficiency, and directionality important for an optimal coupling between adjacent nanophotonic waveguides.

12.
ACS Photonics ; 3(1): 1-7, 2016 Jan 20.
Artigo em Inglês | MEDLINE | ID: mdl-26878028

RESUMO

The ability to confine and manipulate light below the diffraction limit is a major goal of future multifunctional optoelectronic/plasmonic systems. Here, we demonstrate the design and realization of a tunable and localized electrical source of excitons coupled to surface plasmons based on a polymer light-emitting field-effect transistor (LEFET). Gold nanorods that are integrated into the channel support localized surface plasmons and serve as nanoantennas for enhanced electroluminescence. By precise spatial control of the near-infrared emission zone in the LEFET via the applied voltages the near-field coupling between electrically generated excitons and the nanorods can be turned on or off as visualized by a change of electroluminescence intensity. Numerical calculations and spectroscopic measurements corroborate significant local electroluminescence enhancement due to the high local density of photonic states in the vicinity of the gold nanorods. Importantly, the integration of plasmonic nanostructures hardly influences the electrical performance of the LEFETs, thus, highlighting their mutual compatibility in novel active plasmonic devices.

13.
Sci Rep ; 5: 17760, 2015 Dec 07.
Artigo em Inglês | MEDLINE | ID: mdl-26639941

RESUMO

Light propagation in periodic environments is often associated with a number of interesting and potentially useful processes. If a crystalline optical potential is also linearly ramped, light can undergo periodic Bloch oscillations, a direct outcome of localized Wannier-Stark states and their equidistant eigenvalue spectrum. Even though these effects have been extensively explored in conservative settings, this is by no means the case in non-Hermitian photonic lattices encompassing both amplification and attenuation. Quite recently, Bloch oscillations have been predicted in parity-time-symmetric structures involving gain and loss in a balanced fashion. While in a complex bulk medium, one intuitively expects that light will typically follow the path of highest amplification, in a periodic system this behavior can be substantially altered by the underlying band structure. Here, we report the first experimental observation of Bloch oscillations in parity-time-symmetric mesh lattices. We show that these revivals exhibit unusual properties like secondary emissions and resonant restoration of PT symmetry. In addition, we present a versatile method for reconstructing the real and imaginary components of the band structure by directly monitoring the light evolution during a cycle of these oscillations.

14.
Nat Commun ; 6: 7782, 2015 Jul 28.
Artigo em Inglês | MEDLINE | ID: mdl-26215165

RESUMO

Controlling light transport in nonlinear active environments is a topic of considerable interest in the field of optics. In such complex arrangements, of particular importance is to devise strategies to subdue chaotic behaviour even in the presence of gain/loss and nonlinearity, which often assume adversarial roles. Quite recently, notions of parity-time (PT) symmetry have been suggested in photonic settings as a means to enforce stable energy flow in platforms that simultaneously employ both amplification and attenuation. Here we report the experimental observation of optical solitons in PT-symmetric lattices. Unlike other non-conservative nonlinear arrangements where self-trapped states appear as fixed points in the parameter space of the governing equations, discrete PT solitons form a continuous parametric family of solutions. The possibility of synthesizing PT-symmetric saturable absorbers, where a nonlinear wave finds a lossless path through an otherwise absorptive system is also demonstrated.

15.
Nano Lett ; 14(11): 6463-8, 2014 Nov 12.
Artigo em Inglês | MEDLINE | ID: mdl-25302668

RESUMO

We experimentally demonstrate an ultracompact PlasMOStor, a plasmon slot waveguide field-effect modulator based on a transparent conducting oxide active region. By electrically modulating the conducting oxide material deposited into the gaps of highly confined plasmonic slot waveguides, we demonstrate field-effect dynamics giving rise to modulation with high dynamic range (2.71 dB/µm) and low waveguide loss (∼0.45 dB/µm). The large modulation strength is due to the large change in complex dielectric function when the signal wavelength approaches the surface plasmon resonance in the voltage-tuned conducting oxide accumulation layer. The results provide insight about the design of ultracompact, nanoscale modulators for future integrated nanophotonic circuits.

16.
Opt Express ; 22(11): 13744-54, 2014 Jun 02.
Artigo em Inglês | MEDLINE | ID: mdl-24921567

RESUMO

We demonstrate experimentally and numerically that in fiber tips as they are used in NSOMs azimuthally polarized electrical fields (|E(azi)|2 / |E(tot)|2 ≈55% ± 5% for λ0 = 1550 nm), respectively subwavelength confined (FWHM ≈450 nm ≈λ0/3.5) magnetic fields, are generated for a certain tip aperture diameter (d = 1.4 µm). We attribute the generation of this field distribution in metal-coated fiber tips to symmetry breaking in the bend and subsequent plasmonic mode filtering in the truncated conical taper.

17.
Nano Lett ; 13(9): 4539-45, 2013 Sep 11.
Artigo em Inglês | MEDLINE | ID: mdl-23962146

RESUMO

We experimentally demonstrate plasmonic nanocircuits operating as subdiffraction directional couplers optically excited with high efficiency from free-space using optical Yagi-Uda style antennas at λ0 = 1550 nm. The optical Yagi-Uda style antennas are designed to feed channel plasmon waveguides with high efficiency (45% in coupling, 60% total emission), narrow angular directivity (<40°), and low insertion loss. SPP channel waveguides exhibit propagation lengths as large as 34 µm with adiabatically tuned confinement and are integrated with ultracompact (5 × 10 µm(2)), highly dispersive directional couplers, which enable 30 dB discrimination over Δλ = 200 nm with only 0.3 dB device loss.


Assuntos
Nanotecnologia/instrumentação , Óptica e Fotônica , Ressonância de Plasmônio de Superfície , Ouro/química , Refratometria
18.
Opt Express ; 21(16): 18611-23, 2013 Aug 12.
Artigo em Inglês | MEDLINE | ID: mdl-23938778

RESUMO

Second Harmonic Generation (SHG) is a widely used tool to study surfaces. Here we investigate SHG from spherical nanoparticles consisting of a dielectric core (radius 100 nm) and a metallic shell of variable thickness. Plasmonic resonances occur that depend on the thickness of the nanoshells and boost the intensity of the Second Harmonic (SH) signal. The origin of the resonances is studied for the fundamental harmonic and the second harmonic frequencies. Mie resonances at the fundamental harmonic frequency dominate resonant effects of the SH-signal at low shell thickness. Resonances excited by a dipole emitting at SH frequency close to the surface explain the enhancement of the SHG-process at a larger shell thickness. All resonances are caused by surface plasmon polaritons, which run on the surface of the spherical particle and are in resonance with the circumference of the sphere. Because their wavelength critically depends on the properties of the metallic layer SHG resonances of core-shell nanoparticles can be easily tuned by varying the thickness of the shell.

19.
Nano Lett ; 13(8): 3602-6, 2013 Aug 14.
Artigo em Inglês | MEDLINE | ID: mdl-23862660

RESUMO

Tin-doped cadmium sulfide nanowires reveal donor-acceptor pair transitions at low-temperature photoluminescence and furthermore exhibit ideal resonator morphology appropriate for lasing at continuous wave pumping. The continuous wave lasing mode is proven by the evolution of the emitted power and spectrum with increasing pump intensity. The high temperature stability up to 120 K at given pumping power is determined by the decreasing optical gain necessary for lasing in an electron-hole plasma.

20.
Phys Rev Lett ; 110(22): 223902, 2013 May 31.
Artigo em Inglês | MEDLINE | ID: mdl-23767725

RESUMO

We provide the first experimental demonstration of defect states in parity-time (PT) symmetric mesh-periodic potentials. Our results indicate that these localized modes can undergo an abrupt phase transition in spite of the fact that they remain localized in a PT-symmetric periodic environment. Even more intriguing is the possibility of observing a linearly growing radiation emission from such defects provided their eigenvalue is associated with an exceptional point that resides within the continuum part of the spectrum. Localized complex modes existing outside the band-gap regions are also reported along with their evolution dynamics.

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