Laser-Rewriteable Ferromagnetism at Thin-Film Surfaces.

Manipulation of magnetism using laser light is considered as a key to the advancement of data storage technologies. Until now, most approaches seek to optically switch the direction of magnetization rather than to reversibly manipulate the ferromagnetism itself. Here, we use ∼100 fs laser pulses to reversibly switch ferromagnetic ordering on and off by exploiting a chemical order-disorder phase transition in Fe60Al40, from the B2 to the A2 structure and vice versa. A single laser pulse above a threshold fluence causes nonferromagnetic B2 Fe60Al40 to disorder and form the ferromagnetic A2 structure. Subsequent laser pulsing below the threshold reverses the surface to B2 Fe60Al40, erasing the laser-induced ferromagnetism. Simulations reveal that the order-disorder transition is regulated by the extent of surface supercooling; above the threshold for complete melting throughout the film thickness, the liquid phase can be deeply undercooled before solidification. As a result, the vacancy diffusion in the resolidified region is limited and the region is trapped in the metastable chemically disordered state. Laser pulsing below the threshold forms a limited supercooled surface region that solidifies at sufficiently high temperatures, enabling diffusion-assisted reordering. This demonstrates that ultrafast lasers can achieve subtle atomic rearrangements in bimetallic alloys in a reversible and nonvolatile fashion.

Combined electron resonance driven by an all-oscillating potential of patterned magnets.

A novel mechanism is proposed for the phenomenon of combined electron resonance. It is shown that the spatially localized microwave fields of an Fe stripe array mediate the intense electronic transitions involving the changes in both spin and orbital quantum numbers when the electron moves along a cyclotron orbit in a semiconductor (e.g., InGaAs-based) quantum well. This discovery bridges the fields of spintronics and quantum computing, paving the way for conceptually new hybrid devices based on ferromagnetic and semiconductor structured materials.

Evidence of long-wavelength collective excitations in magnetic superlattices.

We report on a mechanism of dynamic dipolar coupling in magnetic superlattices via long-wavelength nonevanescent fields. In the spin excitation spectra of our heterophase stripe structures, such interactions mediate a singlet<-->doublet crossover in the frequency regime driven by the orientation of an external static field. This crossover is a new feature observed in collective behavior of superlattices, though there is some analogy of this phenomenon with birefringence taking place in optical superlattices. We envision applying the collective effects described here in microwave photonic devices.