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1.
Phys Rev Lett ; 125(2): 027203, 2020 Jul 10.
Artigo em Inglês | MEDLINE | ID: mdl-32701346

RESUMO

The ground state of the simple Heisenberg nearest-neighbor quantum kagome antiferromagnetic model is a magnetically disordered spin liquid, yet various perturbations may lead to fundamentally different states. Here we disclose the origin of magnetic ordering in the structurally perfect kagome material YCu_{3}(OH)_{6}Cl_{3}, which is free of the widespread impurity problem. Ab initio calculations and modeling of its magnetic susceptibility reveal that, similar to the archetypal case of herbertsmithite, the nearest-neighbor exchange is by far the dominant isotropic interaction. Dzyaloshinskii-Moriya (DM) anisotropy deduced from electron spin resonance, susceptibility, and specific-heat data is, however, significantly larger than in herbertsmithite. By enhancing spin correlations within kagome planes, this anisotropy is essential for magnetic ordering. Our study isolates the effect of DM anisotropy from other perturbations and unambiguously confirms the predicted phase diagram.

2.
Phys Rev Lett ; 122(20): 206601, 2019 May 24.
Artigo em Inglês | MEDLINE | ID: mdl-31172751

RESUMO

A quantum particle propagates subdiffusively on a strongly disordered chain when it is coupled to itinerant hard-core bosons. We establish a generalized Einstein relation (GER) that relates such subdiffusive spread to an unusual time-dependent drift velocity, which appears as a consequence of a constant electric field. We show that GER remains valid much beyond the regime of the linear response. Qualitatively, it holds true up to strongest drivings when the nonlinear field effects lead to the Stark-like localization. Numerical calculations based on full quantum evolution are substantiated by much simpler rate equations for the boson-assisted transitions between localized Anderson states.

3.
Phys Rev Lett ; 111(14): 147203, 2013 Oct 04.
Artigo em Inglês | MEDLINE | ID: mdl-24138268

RESUMO

Finite-temperature local dynamical spin correlations S(nn)(ω) are studied numerically within the random spin-1/2 antiferromagnetic Heisenberg chain. The aim is to explain measured NMR spin-lattice relaxation times in BaCu(2)(Si(0.5)Ge(0.5))(2)O(7), which is the realization of a random spin chain. In agreement with experiments we find that the distribution of relaxation times within the model shows a very large span similar to the stretched-exponential form. The distribution is strongly reduced with increasing T, but stays finite also in the high-T limit. Anomalous dynamical correlations can be associated with the random singlet concept but not directly with static quantities. Our results also reveal the crucial role of the spin anisotropy (interaction), since the behavior is in contrast with the ones for the XX model, where we do not find any significant T dependence of the distribution.

4.
Artigo em Inglês | MEDLINE | ID: mdl-23410294

RESUMO

The thermalization phenomenon and many-body quantum statistical properties are studied on the example of several observables in isolated spin-chain systems, both integrable and generic nonintegrable. While diagonal matrix elements for nonintegrable models comply with the eigenstate thermalization hypothesis, the integrable systems show evident deviations and similarity to properties of noninteracting many-fermion models. The finite-size scaling reveals that the crossover between the two regimes is given by a scale closely related to the scattering length. Low-frequency off-diagonal matrix elements related to dc transport quantities also follow in a generic system a behavior analogous to the eigenstate thermalization hypothesis, however, unrelated to one of the diagonal matrix elements.


Assuntos
Modelos Químicos , Modelos Moleculares , Modelos Estatísticos , Simulação por Computador , Teoria Quântica , Marcadores de Spin
5.
Phys Rev Lett ; 110(20): 200602, 2013 May 17.
Artigo em Inglês | MEDLINE | ID: mdl-25167392

RESUMO

We study a subsystem of an isolated one-dimensional correlated metal when it is driven by a steady electric field or when it relaxes after driving. We obtain numerically exact reduced density matrix ρ for subsystems which are sufficiently large to give significant eigenvalue statistics and spectra of log(ρ). We show that both for generic as well as for the integrable model, the statistics follows the universality of Gaussian unitary and orthogonal ensembles for driven and equilibrium systems, respectively. Moreover, the spectra of modestly driven subsystems are well described by the Gibbs thermal distribution with the entropy determined by the time-dependent energy only.

6.
Phys Rev Lett ; 106(19): 196401, 2011 May 13.
Artigo em Inglês | MEDLINE | ID: mdl-21668177

RESUMO

We study real-time dynamics of a charge carrier introduced into an undoped Mott insulator propagating under a constant electric field F on the t-J ladder and a square lattice. We calculate the quasistationary current. In both systems an adiabatic regime is observed followed by a positive differential resistivity (PDR) at moderate fields where the carrier mobility is determined. Quantitative differences between the ladder and two-dimensional (2D) systems emerge when at large fields both systems enter the negative differential resistivity (NDR) regime. In the ladder system Bloch-like oscillations prevail, while in two dimensions the current remains finite, proportional to 1/F. The crossover between the PDR and NDR in two dimensions is accompanied by a change of the spatial structure of the propagating spin polaron.

7.
Phys Rev Lett ; 100(3): 036402, 2008 Jan 25.
Artigo em Inglês | MEDLINE | ID: mdl-18233012

RESUMO

It is shown that spectral functions within the extended t-J model, evaluated using the finite-temperature diagonalization of small clusters, exhibit the high-energy kink in single-particle dispersion consistent with recent angle-resolved photoemission results on hole-doped cuprates. The kink and waterfall-like features persist up to large doping and to temperatures beyond J; hence, the origin can be generally attributed to strong correlations and incoherent hole propagation at large binding energies. In contrast, our analysis predicts that electron-doped cuprates do not exhibit these phenomena in photoemission.

8.
Phys Rev Lett ; 93(20): 207202, 2004 Nov 12.
Artigo em Inglês | MEDLINE | ID: mdl-15600962

RESUMO

A theory of the local magnetic response of a nonmagnetic impurity in a doped antiferromagnet, as relevant to the normal-state in cuprates, is presented. It is based on the assumption of the overdamped collective mode in the bulk system and on the evidence that equal-time spin correlations are only weakly renormalized in the vicinity of the impurity. The theory relates the Kondo-like behavior of the local susceptibility to the anomalous temperature dependence of the bulk magnetic susceptibility.

9.
Phys Rev Lett ; 92(2): 027002, 2004 Jan 16.
Artigo em Inglês | MEDLINE | ID: mdl-14753960

RESUMO

A theory of the anomalous omega/T scaling of the dynamic magnetic response in cuprates at low doping is presented. It is based on the memory function representation of the dynamical spin susceptibility in a doped antiferromagnet where the damping of the collective mode is constant and large, whereas the equal-time spin correlations saturate at low T. Exact diagonalization results within the t-J model are shown to support assumptions. Consequences, for both the scaling function and the normalization amplitude, are well in agreement with neutron scattering results.

10.
Phys Rev Lett ; 85(2): 377-80, 2000 Jul 10.
Artigo em Inglês | MEDLINE | ID: mdl-10991287

RESUMO

The zero temperature Hall constant R(H), described by reactive (nondissipative) conductivities, is analyzed within linear response theory. It is found that in a certain limit R(H) is directly related to the density dependence of the Drude weight, implying a simple picture for the change of sign of charge carriers in the vicinity of a Mott-Hubbard transition. This novel formulation is applied to the calculation of R(H) in quasi-one-dimensional and ladder prototype interacting electron systems.

11.
Phys Rev Lett ; 77(19): 4086-4089, 1996 Nov 04.
Artigo em Inglês | MEDLINE | ID: mdl-10062384
12.
Phys Rev Lett ; 77(5): 892-895, 1996 Jul 29.
Artigo em Inglês | MEDLINE | ID: mdl-10062933
13.
Phys Rev B Condens Matter ; 53(22): 15095-15098, 1996 Jun 01.
Artigo em Inglês | MEDLINE | ID: mdl-9983306
15.
Phys Rev B Condens Matter ; 52(9): 6903-6912, 1995 Sep 01.
Artigo em Inglês | MEDLINE | ID: mdl-9981920
16.
Phys Rev Lett ; 75(7): 1340-1343, 1995 Aug 14.
Artigo em Inglês | MEDLINE | ID: mdl-10060268
17.
Phys Rev Lett ; 74(17): 3411-3414, 1995 Apr 24.
Artigo em Inglês | MEDLINE | ID: mdl-10058194
18.
Phys Rev Lett ; 74(6): 972-975, 1995 Feb 06.
Artigo em Inglês | MEDLINE | ID: mdl-10058895
19.
Phys Rev B Condens Matter ; 50(10): 7129-7132, 1994 Sep 01.
Artigo em Inglês | MEDLINE | ID: mdl-9974669
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