Nonadiabatic effects in ultracold molecules via anomalous linear and quadratic Zeeman shifts.

Anomalously large linear and quadratic Zeeman shifts are measured for weakly bound ultracold 88Sr2 molecules near the intercombination-line asymptote. Nonadiabatic Coriolis coupling and the nature of long-range molecular potentials explain how this effect arises and scales roughly cubically with the size of the molecule. The linear shifts yield nonadiabatic mixing angles of the molecular states. The quadratic shifts are sensitive to nearby opposite f-parity states and exhibit fourth-order corrections, providing a stringent test of a state-of-the-art ab initio model.

Optical production of stable ultracold (88)Sr(2) molecules.

We have produced large samples of stable ultracold (88)Sr(2) molecules in the electronic ground state in an optical lattice. The fast, all-optical method of molecule creation involves a near-intercombination-line photoassociation pulse followed by spontaneous emission with a near-unity Franck-Condon factor. The detection uses excitation to a weakly bound electronically excited vibrational level corresponding to a very large dimer and yields a high-Q molecular vibronic resonance. This is the first of two steps needed to create deeply bound (88)Sr(2) for frequency metrology and ultracold chemistry.

Optically guided beam splitter for propagating matter waves.

We study experimentally and theoretically a beam splitter setup for guided atomic matter waves. The matter wave is a guided atom laser that can be tuned from quasimonomode to a regime where many transverse modes are populated, and propagates in a horizontal dipole beam until it crosses another horizontal beam at 45°. We show that depending on the parameters of this X configuration, the atoms can all end up in one of the two beams (the system behaves as a perfect guide switch), or be split between the four available channels (the system behaves as a beam splitter). The splitting regime results from a chaotic scattering dynamics. The existence of these different regimes turns out to be robust against small variations of the parameters of the system. From numerical studies, we also propose a scheme that provides a robust and controlled beam splitter in two channels only.

Strong saturation absorption imaging of dense clouds of ultracold atoms.

We report on a far above saturation absorption imaging technique to investigate the characteristics of dense packets of ultracold atoms. The transparency of the cloud is controlled by the incident light intensity as a result of the nonlinear response of the atoms to the probe beam. We detail our experimental procedure to calibrate the imaging system for reliable quantitative measurements and demonstrate the use of this technique to extract the profile and its spatial extent of an optically thick atomic cloud.

Long-lived quantum memory with nuclear atomic spins.

We propose to store nonclassical states of light into the macroscopic collective nuclear spin (10(18) atoms) of a 3He vapor, using metastability exchange collisions. These collisions, commonly used to transfer orientation from the metastable state 2 3S1 to the ground state of 3He, can also transfer quantum correlations. This gives a possible experimental scheme to map a squeezed vacuum field state onto a nuclear spin state with very long storage times (hours).