Search for supersolidity in solid 4He using multiple-mode torsional oscillators.

In 2004, Kim and Chan (KC) reported a decrease in the period of torsional oscillators (TO) containing samples of solid (4)He, as the temperature was lowered below 0.2 K [Kim E, Chan MHW (2004) Science 305(5692):1941-1944]. These unexpected results constituted the first experimental evidence that the long-predicted supersolid state of solid (4)He may exist in nature. The KC results were quickly confirmed in a number of other laboratories and created great excitement in the low-temperature condensed-matter community. Since that time, however, it has become clear that the period shifts seen in the early experiments can in large part be explained by an increase in the shear modulus of the (4)He solid identified by Day and Beamish [Day J, Beamish J (2007) Nature 450(7171):853-856]. Using multiple-frequency torsional oscillators, we can separate frequency-dependent period shifts arising from changes in the elastic properties of the solid (4)He from possible supersolid signals, which are expected to be independent of frequency. We find in our measurements that as the temperature is lowered below 0.2 K, a clear frequency-dependent contribution to the period shift arising from changes in the (4)He elastic properties is always present. For all of the cells reported in this paper, however, there is always an additional small frequency-independent contribution to the total period shift, such as would be expected in the case of a transition to a supersolid state.

Anomalous behavior of solid 4He in porous Vycor glass.

The low temperature properties of solid (4)He contained in porous Vycor glass have been investigated utilizing a two-mode compound torsional oscillator. At low temperatures, we find period-shift signals for the solid similar to those reported by Kim and Chan [Nature (London) 427, 225 (2004)], which were taken at the time as evidence for a supersolid helium phase. The supersolid is expected to have properties analogous to those of a conventional superfluid, where the superfluid behavior is independent of frequency and the ratio of the superfluid signals observed at two different mode periods will depend only on the ratio of the sensitivities of the mode periods to mass loading. In the case of helium studies in Vycor, one can compare the period-shift signals seen for a conventional superfluid film with signals obtained for a supersolid within the same Vycor sample. We find, contrary to our own expectations, that the signals observed for the solid display a marked period dependence not seen in the case of the superfluid film. This surprising result suggests that the low temperature response of solid (4)He in Vycor is more complex than previously assumed and cannot be thought of as a simple superfluid.

Nonsuperfluid origin of the nonclassical rotational inertia in a bulk sample of solid 4He.

The torsional oscillator experiments described here examine the effect of disorder on the nonclassical rotational inertia (NCRI) of a solid 4He sample. The NCRI increases with increasing disorder, but the period changes responsible for this increase occur primarily at higher temperatures. Contrary to expectations based on a supersolid scenario, the oscillator period remains relatively unaffected at the lowest temperatures. This result points to a nonsuperfluid origin for the NCRI.

Probing the upper limit of nonclassical rotational inertia in solid helium 4.

We study the effect of confinement on solid 4He's nonclassical rotational inertia fraction (NCRIF) in a torsional oscillator by constraining it to narrow annular cells of various widths. The NCRIF exhibits an observed maximum value of 20% for annuli of approximately 100 microm width. Samples constrained to porous media or to larger geometries both have smaller NCRIF, mostly below approximately 1%. In addition, we extend the blocked-annulus experiment of Kim and Chan to solid samples with large supersolid fractions. Blocking the annulus suppresses the nonclassical decoupling from 17.1% to below the limit of our detection of 0.8%. This result demonstrates the nonlocal nature of the supersolid phenomena. At 20 mK, NCRIF depends on velocity history showing a closed hysteresis loop in different thin annular cells.

Observation of classical rotational inertia and nonclassical supersolid signals in solid 4He below 250 mK.

We have confirmed the existence, as first reported by Kim and Chan, of a supersolid state in solid 4He at temperatures below 250 mK. We have employed a torsional oscillator cell with a square cross section to insure a locking of the solid to the oscillating cell. We find that the nonclassical rotational inertia signal is not a universal property of solid 4He but can be eliminated through an annealing of the solid helium sample. This result has important implications for our understanding of the supersolid state.