RESUMO
We report on the potential of a new spin noise spectroscopy approach by demonstrating all-optical probing of spatiotemporal spin fluctuations. This is achieved by homodyne mixing of a spatially phase-modulated local oscillator with spin-flip scattered light, from which the frequency and wave vector dependence of the spin noise power is unveiled. As a first application of the method we measure the spatiotemporal spin noise in weakly n-doped CdTe layers, from which the electron spin diffusion constant and spin relaxation rates are determined. The absence of spatial spin correlations is also shown for this particular system.
RESUMO
Spin noise spectroscopy is a powerful technique for studying spin relaxation in semiconductors. In this article, we propose an extension of this technique based on optical heterodyne detection of spin noise, which provides several key advantages compared to conventional spin noise spectroscopy: detection of high frequency spin noise not limited by detector bandwidth or sampling rates of digitizers, quantum limited sensitivity even in case of very weak probe power, and possible amplification of the spin noise signal. Heterodyne detection of spin noise is demonstrated on insulating n-doped GaAs. From measurements of spin noise spectra up to 0.4 Tesla, we determined the distribution of g-factors, Δg/g = 0.49%.
RESUMO
Spin noise spectroscopy is an optical technique which can probe spin resonances non-perturbatively. First applied to atomic vapours, it revealed detailed information about nuclear magnetism and the hyperfine interaction. In solids, this approach has been limited to carriers in semiconductor heterostructures. Here we show that atomic-like spin fluctuations of Mn ions diluted in CdTe (bulk and quantum wells) can be detected through the Kerr rotation associated to excitonic transitions. Zeeman transitions within and between hyperfine multiplets are clearly observed in zero and small magnetic fields and reveal the local symmetry because of crystal field and strain. The linewidths of these resonances are close to the dipolar limit. The sensitivity is high enough to open the way towards the detection of a few spins in systems where the decoherence due to nuclear spins can be suppressed by isotopic enrichment, and towards spin resonance microscopy with important applications in biology and materials science.
RESUMO
We report on the nondestructive measurement of nuclear magnetization in n-GaAs via cavity enhanced Faraday rotation. In contrast with the existing optical methods, this detection scheme does not require the presence of detrimental out-of-equilibrium electrons. Specific mechanisms of the Faraday rotation are identified for (i) nuclear spins situated within the localized electron orbits, these spins are characterized by fast dynamics, (ii) all other nuclear spins in the sample characterized by much slower dynamics. Our results suggest that even in degenerate semiconductors nuclear spin relaxation is limited by the presence of localized electron states and spin diffusion, rather than by Korringa mechanism.
RESUMO
Optical pump-probe experiments reveal spin beats of manganese ions in (Cd,Mn)Te, due to hyperfine and crystal fields. At "magic" orientations of the magnetic field, the effect of local crystal field is strongly suppressed. In this case, the spin precession of Mn(2+) embedded in the lattice approaches the precession expected for the free ion. Following optical excitation, regular spin pulses show up, revealing the one-to-one correspondence between precession frequency and Mn(2+) nuclear spin state. The period of the spin pulses accurately determines the hyperfine constant |A|=705 neV. The manganese spin coherence time up to T(2)(Mn)≃15 ns is measured for a manganese concentration x=0.0011.
RESUMO
We report the first observation of oscillations of the electromagnetic field in an optical superlattice based on porous silicon. These oscillations are an optical equivalent of well-known electronic Bloch oscillations in crystals. Elementary cells of our structure are composed by microcavities whose coupling gives rise to the extended collective modes forming optical minigaps and minibands. By varying thicknesses of the cavities along the structure axis, we have created an effective electric field for photons. A very high quality factor of the confined optical state of the Wannier-Stark ladder may allow lasing in porous silicon-based superlattices.
