Giant lattice softening at a Lifshitz transition in Sr2RuO4.

The interplay of electronic and structural degrees of freedom in solids is a topic of intense research. More than 60 years ago, Lifshitz discussed a counterintuitive possibility: lattice softening driven by conduction electrons at topological Fermi surface transitions. The effect that he predicted, however, was small and has not been convincingly observed. Using a piezo-based uniaxial pressure cell to tune the ultraclean metal strontium ruthenate while measuring the stress-strain relationship, we reveal a huge softening of the Young's modulus at a Lifshitz transition of a two-dimensional Fermi surface and show that it is indeed driven entirely by the conduction electrons of the relevant energy band.

Emergent Continuous Symmetry in Anisotropic Flexible Two-Dimensional Materials.

We develop the theory of anomalous elasticity in two-dimensional flexible materials with orthorhombic crystal symmetry. Remarkably, in the universal region, where characteristic length scales are larger than the rather small Ginzburg scale ∼10 nm, these materials possess an infinite set of flat phases. These phases corresponds to a stable line of fixed points and are connected by an emergent continuous symmetry. This symmetry enforces power law scaling with momentum of the anisotropic bending rigidity and Young's modulus, controlled by a single universal exponent-the very same along the whole line of fixed points. These anisotropic flat phases are uniquely labeled by the ratio of absolute Poisson's ratios. We apply our theory to phosphorene.

Strange semimetal dynamics in SrIrO3.

The interplay of electronic correlations, multi-orbital excitations, and spin-orbit coupling is a fertile ground for new states of matter in quantum materials. Here, we report on a polarized Raman scattering study of semimetallic SrIrO3. The momentum-space selectivity of Raman scattering allows to circumvent the challenge to resolve the dynamics of charges with very different mobilities. The Raman responses of both holes and electrons display an electronic continuum extending far beyond the energies allowed in a regular Fermi liquid. Analyzing this response within a memory function formalism, we extract their frequency dependent scattering rate and mass enhancement, from which we determine their DC-mobilities and electrical resistivities that agree well with transport measurement. We demonstrate that its charge dynamics is well described by a marginal Fermi liquid phenomenology, with a scattering rate close to the Planckian limit. This demonstrates the potential of this approach to investigate the charge dynamics in multi-band systems.

Anomalous density fluctuations in a strange metal.

A central mystery in high-temperature superconductivity is the origin of the so-called strange metal (i.e., the anomalous conductor from which superconductivity emerges at low temperature). Measuring the dynamic charge response of the copper oxides, [Formula: see text], would directly reveal the collective properties of the strange metal, but it has never been possible to measure this quantity with millielectronvolt resolution. Here, we present a measurement of [Formula: see text] for a cuprate, optimally doped Bi2.1Sr1.9CaCu2O8+x (Tc = 91 K), using momentum-resolved inelastic electron scattering. In the medium energy range 0.1-2 eV relevant to the strange metal, the spectra are dominated by a featureless, temperature- and momentum-independent continuum persisting to the electronvolt energy scale. This continuum displays a simple power-law form, exhibiting q2 behavior at low energy and q2/ω2 behavior at high energy. Measurements of an overdoped crystal (Tc = 50 K) showed the emergence of a gap-like feature at low temperature, indicating deviation from power law form outside the strange-metal regime. Our study suggests the strange metal exhibits a new type of charge dynamics in which excitations are local to such a degree that space and time axes are decoupled.

Anomalous quantum criticality in an itinerant ferromagnet.

The dynamics of continuous phase transitions is governed by the dynamic scaling exponent relating the correlation length and correlation time. For transitions at finite temperature, thermodynamic critical properties are independent of the dynamic scaling exponent. In contrast, at quantum phase transitions where the transition temperature becomes zero, static and dynamic properties are inherently entangled by virtue of the uncertainty principle. Consequently, thermodynamic scaling equations explicitly contain the dynamic exponent. Here we report on thermodynamic measurements (as a function of temperature and magnetic field) for the itinerant ferromagnet Sr1-xCaxRuO3 where the transition temperature becomes zero for x=0.7. We find dynamic scaling of the magnetization and specific heat with highly unusual quantum critical dynamics. We observe a small dynamic scaling exponent of 1.76 strongly deviating from current models of ferromagnetic quantum criticality and likely being governed by strong disorder in conjunction with strong electron-electron coupling.

Evidence of strong correlations and coherence-incoherence crossover in the iron pnictide superconductor KFe2As2.

Using resistivity, heat-capacity, thermal-expansion, and susceptibility measurements we study the normal-state behavior of KFe2As2. Both the Sommerfeld coefficient (γ≈103 mJ mol(-1) K(-2)) and the Pauli susceptibility (χ≈4×10(-4)) are strongly enhanced, which confirm the existence of heavy quasiparticles inferred from previous de Haas-van Alphen and angle-resolved photoemission spectroscopy experiments. We discuss this large enhancement using a Gutzwiller slave-boson mean-field calculation, which shows the proximity of KFe2As2 to an orbital-selective Mott transition. The temperature dependence of the magnetic susceptibility and the thermal expansion provide strong experimental evidence for the existence of a coherence-incoherence crossover, similar to what is found in heavy fermion and ruthenate compounds, due to Hund's coupling between orbitals.

Sign-reversal of the in-plane resistivity anisotropy in hole-doped iron pnictides.

Unconventional superconductivity usually originates from several strongly coupled degrees of freedom, such as magnetic, charge and elastic. A highly anisotropic electronic phase, not driven by lattice degrees of freedom, has been proposed in some of these superconductors, from cuprates to iron-based compounds. In the iron pnictide BaFe2As2, this nematic phase arises in the paramagnetic phase and is present for wide doping and temperature ranges. Here we probe the in-plane electronic anisotropy of electron- and hole-doped BaFe2As2 compounds. Unlike other materials, the resistivity anisotropy behaves very differently for electron- and hole-type dopants and even changes sign on the hole-doped side. This behaviour is explained by Fermi surface reconstruction in the magnetic phase and spin-fluctuation scattering in the paramagnetic phase. This unique transport anisotropy unveils the primary role played by magnetic scattering, demonstrating the close connection between magnetism, nematicity and unconventional superconductivity.

Unbinding of giant vortices in states of competing order.

We consider a two-dimensional system with two order parameters, one with O(2) symmetry and one with O(M), near a point in parameter space where they couple to become a single O(2+M) order. While the O(2) sector supports vortex excitations, these vortices must somehow disappear as the high symmetry point is approached. We develop a variational argument which shows that the size of the vortex cores diverges as 1/âˆšΔ and the Berezinskii-Kosterlitz-Thouless transition temperature of the O(2) order vanishes as 1/ln(1/Δ), where Δ denotes the distance from the high-symmetry point. Our physical picture is confirmed by a renormalization group analysis which gives further logarithmic corrections, and demonstrates full symmetry restoration within the cores.

Conductivity close to antiferromagnetic criticality.

We study the conductivity of a three-dimensional disordered metal close to antiferromagnetic instability within the framework of the spin-fermion model using the diagrammatic technique. We calculate the interaction correction δσ(ω,T) to the conductivity, assuming that the latter is dominated by the disorder scattering, and the interaction is weak. Although the fermionic scattering rate shows critical behavior on the entire Fermi surface, the interaction correction is dominated by the processes near the hot spots, narrow regions of the Fermi surface corresponding to the strongest spin-fermion scattering. Exactly at the critical point δσ is proportional to [max(ω,T)](3/2). At sufficiently large frequencies ω the conductivity is independent of the temperature, and δσ is proportional to (τ(-1)-iω)(-2), τ being the elastic scattering time. In a certain intermediate frequency range δσ(ω) is proportional to iω(τ(-1)-iω)(-2).

Femtosecond population inversion and stimulated emission of dense Dirac fermions in graphene.

We show that strongly photoexcited graphene monolayers with 35 fs pulses quasi-instantaneously build up a broadband, inverted Dirac fermion population. Optical gain emerges and directly manifests itself via a negative conductivity at the near-infrared region for the first 200 fs, where stimulated emission completely compensates absorption loss in the graphene layer. Our experiment-theory comparison with two distinct electron and hole chemical potentials reproduce absorption saturation and gain at 40 fs, revealing, particularly, the evolution of the transient state from a hot classical gas to a dense quantum fluid with increasing the photoexcitation.

Anomalous suppression of the orthorhombic lattice distortion in superconducting Ba(Fe1-xCox)2As2 single crystals.

High-resolution x-ray diffraction measurements reveal an unusually strong response of the lattice to superconductivity in Ba(Fe1-xCox)2As2. The orthorhombic distortion of the lattice is suppressed and, for Co doping near x=0.063, the orthorhombic structure evolves smoothly back to a tetragonal structure. We propose that the coupling between orthorhombicity and superconductivity is indirect and arises due to the magnetoelastic coupling, in the form of emergent nematic order, and the strong competition between magnetism and superconductivity.

Effects of nematic fluctuations on the elastic properties of iron arsenide superconductors.

We demonstrate that the changes in the elastic properties of the FeAs systems, as seen in our resonant ultrasound spectroscopy data, can be naturally understood in terms of fluctuations of emerging nematic degrees of freedom. Both the softening of the lattice in the normal, tetragonal phase as well as its hardening in the superconducting phase are consistently described by our model. Our results confirm the view that structural order is induced by magnetic fluctuations.

Anomalies in the Fermi surface and band dispersion of quasi-one-dimensional CuO chains in the high-temperature superconductor YBa2Cu4O8.

We have investigated the electronic states in quasi-one-dimensional CuO chains by microprobe angle resolved photoemission spectroscopy. We find that the quasiparticle Fermi surface consists of six disconnected segments, consistent with recent theoretical calculations that predict the formation of narrow, elongated Fermi surface pockets for coupled CuO chains. In addition, we find a strong renormalization effect with a significant kink structure in the band dispersion. The properties of this latter effect [energy scale (∼40 meV), temperature dependence, and behavior with Zn-doping] are identical to those of the bosonic mode observed in CuO2 planes of high-temperature superconductors, indicating they have a common origin.

Unconventional London penetration depth in single-crystal Ba(Fe0.93Co0.07)2As2 superconductors.

The London penetration depth lambda(T) has been measured in single crystals of Ba(Fe0.93Co0.07)2As2. The observed low-temperature variation of lambda(T) follows a power law, Deltalambda(T) approximately T(n) with n approximately 2.4+/-0.1, indicating the existence of normal quasiparticles down to at least 0.02T(c). This is in contrast with previous penetration depth measurements on single crystals of NdFeAsO1-xFx and SmFeAsO1-xFx, which indicate an anisotropic but nodeless gap. We discuss possible explanations of the observed power law behavior.

Momentum dependence of the superconducting gap in NdFeAsO0.9F0.1 single crystals measured by angle resolved photoemission spectroscopy.

We use angle resolved photoemission spectroscopy to study the momentum dependence of the superconducting gap in NdFeAsO0.9F0.1 single crystals. We find that the Gamma hole pocket is fully gapped below the superconducting transition temperature. The value of the superconducting gap is 15+/-1.5 meV and its anisotropy around the hole pocket is smaller than 20% of this value-consistent with an isotropic or anisotropic s-wave symmetry of the order parameter. This is a significant departure from the situation in the cuprates, pointing to the possibility that the superconductivity in the iron arsenic based system arises from a different mechanism.

Geometric frustration and dimensional reduction at a quantum critical point.

We show that the spatial dimensionality of the quantum critical point associated with Bose-Einstein condensation at T=0 is reduced when the underlying lattice comprises layers coupled by a frustrating interaction. Our theoretical predictions for the critical behavior correspond very well with recent measurements in BaCuSi(2)O(6) [ S. E. Sebastian et al., Nature (London) 441, 617 (2006)].

Quantum critical end point for the Kondo volume collapse model.

The Kondo volume collapse describes valence transitions in f-electron metals and is characterized by a line of first order transitions in the pressure-temperature phase plane terminated at critical end points. We analyze the quantum critical end point, when the lower end point is tuned to T=0, and determine the specific heat, thermal expansion, and compressibility. We find that the inclusion of quantum critical fluctuations leads to a novel bifurcation of the first order phase line. Finally, we show that critical strain fluctuations can cause both, superconductivity and non-Fermi liquid behavior near the critical point.

Dynamics of magnetic defects in heavy fermion LiV2O4 from stretched exponential 7Li NMR relaxation.

7Li NMR measurements on LiV2O4 from 0.5 to 4.2 K are reported. A small concentration of magnetic defects within the structure drastically changes the nuclear magnetization relaxation versus time from a pure exponential as in pure LiV2O4 to a stretched exponential, indicating glassy behavior of the magnetic defects. The stretched exponential function is described as arising from a distribution of 7Li nuclear spin-lattice relaxation rates and we present a model for the distribution in terms of the dynamics of the magnetic defects. Our results explain the origin of recent puzzling 7Li NMR literature data on LiV2O4 and our model is likely applicable to other glassy systems.

"Devil's staircase" in Pb/Si(111) ordered phases.

With scanning tunneling microscopy we have found that ordered phases in Pb/Si(111) are one of the best examples of the "devil's staircase" phase diagram. Phases within a narrow coverage range (1.2

Neutron resonance in the cuprates and its effect on fermionic excitations.

We argue that the exciton scenario for the magnetic resonance in the cuprate superconductors yields a small spectral weight of the resonance, in agreement with experiment. We show that the small weight is related to its concentration in a small region of momentum and energy. Despite this, we find that a large fermionic self-energy can indeed be generated by a resonance with such properties, i.e., the scattering from the resonance substantially affects the electronic properties of the cuprates below T(c).