RESUMO
We report on theoretical and experimental results concerning the low-temperature specific heat of the frustrated spin-tube material [(CuCl(2)tachH(3)Cl]Cl(2) (tach denotes 1,3,5-triaminocyclohexane). This substance turns out to be an unusually perfect spin-tube system which allows to study the physics of quasi-one-dimensional antiferromagnetic structures in rather general terms. An analysis of the specific-heat data demonstrates that at low enough temperatures the system exhibits a Tomonaga-Luttinger liquid behavior corresponding to an effective spin-3/2 antiferromagnetic Heisenberg chain with short-range exchange interactions. On the other hand, around 2 K the composite spin structure of the chain is revealed through a Schottky-type peak in the specific heat. We argue that the dominating contribution to the peak originates from gapped magnon-type excitations related to the internal degrees of freedom of the rung spins.
RESUMO
Spin transport in the anisotropic Heisenberg chain is typically investigated theoretically with respect to the finiteness of transport coefficients only. Assuming their finiteness at high temperatures, we develop a concrete quantitative picture of the diffusion constant/(dc-)conductivity as a function of both the anisotropy parameter Δ and the spin quantum number s, going beyond the most commonly considered case s=1/2. Using this picture, we enable the comparison of finite transport coefficients from complementary theoretical methods on a quantitative level, having more significance than the finiteness alone. Our method is essentially based on an application of the time-convolutionless projection operator technique to current autocorrelations. This technique, although being a perturbation theory in Δ, is found to be applicable, even if Δ is not small. This finding supports the applicability to a wider class of strongly interacting many-particle quantum systems.
