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1.
Nat Commun ; 2: 394, 2011 Jul 12.
Artigo em Inglês | MEDLINE | ID: mdl-21750547

RESUMO

High-temperature superconductivity in iron-arsenic materials (pnictides) near an antiferromagnetic phase raises the possibility of spin-fluctuation-mediated pairing. However, the interplay between antiferromagnetic fluctuations and superconductivity remains unclear in the underdoped regime, which is closer to the antiferromagnetic phase. Here we report that the superconducting gap of underdoped pnictides scales linearly with the transition temperature, and that a distinct pseudogap coexisting with the superconducting gap develops on underdoping. This pseudogap occurs on Fermi surface sheets connected by the antiferromagnetic wavevector, where the superconducting pairing is stronger as well, suggesting that antiferromagnetic fluctuations drive both the pseudogap and superconductivity. Interestingly, we found that the pseudogap and the spectral lineshape vary with the Fermi surface quasi-nesting conditions in a fashion that shares similarities with the nodal-antinodal dichotomous behaviour observed in underdoped copper oxide superconductors.


Assuntos
Arsenicais/química , Condutividade Elétrica , Temperatura Alta , Ferro/química , Magnetismo , Espectroscopia Fotoeletrônica
2.
Phys Rev Lett ; 105(19): 197001, 2010 Nov 05.
Artigo em Inglês | MEDLINE | ID: mdl-21231191

RESUMO

We have performed angle-resolved photoemission spectroscopy of the iron-chalcogenide superconductor Fe1.03Te0.7Se0.3 to investigate the electronic structure relevant to superconductivity. We observed a holelike Fermi surface (FS) and an electronlike FS at the Brillouin zone center and corner, respectively, which are nearly nested by the Q∼(π,π) wave vector. We do not find evidence for the nesting instability with Q∼(π+δ,0) reminiscent of the antiferromagnetic order in the parent compound Fe1+yTe. We have observed an isotropic superconducting (SC) gap along the holelike FS with the gap size Δ of ∼4 meV (2Δ/kBTc ∼ 7), demonstrating the strong-coupling superconductivity. The observed similarity of low-energy electronic excitations between iron-chalcogenides and iron-arsenides strongly suggests that common interactions which involve Q∼(π,π) scattering are responsible for the SC pairing.

3.
Phys Rev Lett ; 102(22): 227006, 2009 Jun 05.
Artigo em Inglês | MEDLINE | ID: mdl-19658895

RESUMO

We have performed an ultrahigh-resolution angle-resolved photoemission spectroscopy study of slightly overdoped (Bi,Pb)2Sr2CuO6 to elucidate the origin of the pseudogap. By using a newly developed xenon-plasma light source, we determined the comprehensive momentum and temperature dependencies of the superconducting gap and the pseudogap. We found that the antinodal pseudogap persists far above the superconducting transition temperature and is smoothly connected to the nodal gap. The characteristic temperature of the pseudogap scales well with the superconducting gap size irrespective of the momentum location. The present experimental results point to the pairing origin of the pseudogap.

4.
Phys Rev Lett ; 103(4): 047002, 2009 Jul 24.
Artigo em Inglês | MEDLINE | ID: mdl-19659391

RESUMO

We have performed high-resolution angle-resolved photoemission spectroscopy on heavily overdoped KFe_{2}As_{2} (transition temperature T_{c} = 3 K). We observed several renormalized bands near the Fermi level with a renormalization factor of 2-4. While the Fermi surface around the Brillouin-zone center is qualitatively similar to that of optimally doped Ba_{1-x}K_{x}Fe_{2}As_{2} (x = 0.4; T_{c} = 37 K), the Fermi surface topology around the zone corner (M point) is markedly different: the two electron Fermi surface pockets are completely absent due to an excess of hole doping. This result indicates that the electronic states around the M point play an important role in the high-T_{c} superconductivity of Ba_{1-x}K_{x}Fe_{2}As_{2} and suggests that the interband scattering via the antiferromagnetic wave vector essentially controls the T_{c} value in the overdoped region.

5.
Proc Natl Acad Sci U S A ; 106(18): 7330-3, 2009 May 05.
Artigo em Inglês | MEDLINE | ID: mdl-19359490

RESUMO

The discovery of high-temperature superconductivity in iron pnictides raised the possibility of an unconventional superconducting mechanism in multiband materials. The observation of Fermi-surface (FS)-dependent nodeless superconducting gaps suggested that inter-FS interactions may play a crucial role in superconducting pairing. In the optimally hole-doped Ba(0.6)K(0.4)Fe(2)As(2), the pairing strength is enhanced simultaneously (2Delta/T(c) approximately 7) on the nearly nested FS pockets, i.e., the inner hole-like (alpha) FS and the 2 hybridized electron-like FSs, whereas the pairing remains weak (2Delta/T(c) approximately 3.6) in the poorly nested outer hole-like (beta) FS. Here, we report that in the electron-doped BaFe(1.85)Co(0.15)As(2), the FS nesting condition switches from the alpha to the beta FS due to the opposite size changes for hole- and electron-like FSs upon electron doping. The strong pairing strength (2Delta/T(c) approximately 6) is also found to switch to the nested beta FS, indicating an intimate connection between FS nesting and superconducting pairing, and strongly supporting the inter-FS pairing mechanism in the iron-based superconductors.

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