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1.
Environ Sci Technol ; 52(20): 11941-11951, 2018 10 16.
Artigo em Inglês | MEDLINE | ID: mdl-30207717

RESUMO

We present a statistically enhanced version of the GreenHouse gas emissions of current Oil Sands Technologies model that facilitates characterization of variability of greenhouse gas (GHG) emissions associated with mining and upgrading of bitumen from Canadian oil sands. Over 30 years of publicly available project-specific operating data are employed as inputs, enabling Monte Carlo simulation of individual projects and the entire industry, for individual years and project life cycles. We estimate that median lifetime GHG intensities range from 89 to 137 kg CO2eq/bbl synthetic crude oil (SCO) for projects that employ upgrading. The only project producing dilbit that goes directly to a refinery has a median lifetime GHG intensity of 51 kg CO2eq/bbl dilbit. As SCO and dilbit are distinct products with different downstream processing energy requirements, a life cycle assessment ("well to wheel") is needed to properly compare them. Projects do not reach steady-state in terms of median GHG intensity. Projects with broader distributions of annual GHG intensities and higher median values are linked to specific events (e.g., project expansions). An implication for policymakers is that no specific technology or operating factor can be directly linked to GHG intensity and no particular project or year of operation can be seen as representative of the industry or production technology.


Assuntos
Poluentes Atmosféricos , Gases de Efeito Estufa , Canadá , Efeito Estufa , Campos de Petróleo e Gás , Óleo de Brassica napus
2.
Environ Sci Technol ; 46(14): 7865-74, 2012 Jul 17.
Artigo em Inglês | MEDLINE | ID: mdl-22667690

RESUMO

Life cycle greenhouse gas (GHG) emissions associated with two major recovery and extraction processes currently utilized in Alberta's oil sands, surface mining and in situ, are quantified. Process modules are developed and integrated into a life cycle model-GHOST (GreenHouse gas emissions of current Oil Sands Technologies) developed in prior work. Recovery and extraction of bitumen through surface mining and in situ processes result in 3-9 and 9-16 g CO(2)eq/MJ bitumen, respectively; upgrading emissions are an additional 6-17 g CO(2)eq/MJ synthetic crude oil (SCO) (all results are on a HHV basis). Although a high degree of variability exists in well-to-wheel emissions due to differences in technologies employed, operating conditions, and product characteristics, the surface mining dilbit and the in situ SCO pathways have the lowest and highest emissions, 88 and 120 g CO(2)eq/MJ reformulated gasoline. Through the use of improved data obtained from operating oil sands projects, we present ranges of emissions that overlap with emissions in literature for conventional crude oil. An increased focus is recommended in policy discussions on understanding interproject variability of emissions of both oil sands and conventional crudes, as this has not been adequately represented in previous studies.


Assuntos
Poluentes Atmosféricos/análise , Efeito Estufa , Mineração/métodos , Modelos Teóricos , Óleos/química , Dióxido de Silício/química , Alberta , Hidrocarbonetos/química , Propriedades de Superfície , Meios de Transporte
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