RESUMO
We report on investigations concerning the shot-to-shot spectral stability properties of a supercontinuum source based on nonlinear processes such as self-phase modulation and optical wave-breaking in a highly concentrated K2ZnCl4 double salt solution. The use of a liquid medium offers both damage resistance and high third-order optical nonlinearity. Approximately 40 µJ pulses spanning a spectral range between 390 and 960 nm were produced with 3.8% RMS energy stability, using infrared input pulses of 500±50 fs FWHM durations and 2.42±0.04 mJ energies with an RMS stability of 2%. The spectral stability was quantified via acquiring single-shot spectra and studying shot-to-shot variation across a spectral range of 200-1100 nm, as well as by considering spectral correlations. The regional spectral correlation variations were indicative of nonlinear processes leading to sideband generation. Spectral stability and efficiency of energy transfer into the supercontinuum were found to weakly improve with increasing driver pulse energy, suggesting that the nonlinear broadening processes are more stable when driven more strongly, or that self-guiding effects in a filament help to stabilize the supercontinuum generation.
RESUMO
Thin liquid sheet jet flows in vacuum provide a new platform for performing experiments in the liquid phase, for example X-ray spectroscopy. Micrometer thickness, high stability, and optical flatness are the key characteristics required for successful exploitation of these targets. A novel strategy for generating sheet jets in vacuum is presented in this article. Precision nozzles were designed and fabricated using high resolution (0.2 µm) 2-photon 3D printing and generated 1.49 ± 0.04 µm thickness, stable, and <λ/20-flat jets in isopropanol under normal atmosphere and under vacuum at 5 × 10-1 mbar. The thin sheet technology also holds great promise for advancing the fields of high harmonic generation in liquids, laser acceleration of ions as well as other fields requiring precision and high repetition rate targets.
RESUMO
We have investigated the temporal intensity contrast characteristics from a broad range of mode-locked short-pulse oscillators used for seeding high-power terawatt and petawatt-class laser systems. Saturable absorber (SESAM), Kerr lens (KLM), nonlinear polarization evolution (NPE) in optical fibers and synchronously pumped optical parametric oscillator (OPO) mode-locked sources have been measured using a third-order autocorrelator with up to 1010 dynamic range. We restricted the temporal characterization to features <30 ps about the laser pulse that reflect fundamental mode-locking processes. We find additional nonlinear terms and residual higher-order dispersion limits the performance of KLM and NPE sources up to the 105 contrast level, while >108 contrast was observed from the SESAM and OPO laser pulse trains.
RESUMO
In this paper we present an optically synchronized Nd:YLF regenerative amplifier optimized for use as a preamplifier in a few-cycle optical parametric chirped pulse amplification pump laser. In the pump amplification process we employ a combination of spectral modulation and chirping in order to control and optimize the temporal shape of the pulses. We report on a comparative study of two methods for generating near-flat-top or custom real-time variable-shaped pump pulses using either controlled chirp and shaping of the spectrum of the pulses seeding a regenerative amplifier or intracavity spectral filtering to broaden the gain bandwidth of the system. We show that in addition to minimizing gain narrowing and B-integral, the efficiency of the cascaded nonlinear processes of the parametric amplifiers can be increased.
