Highly intense monocycle terahertz vortex generation by utilizing a Tsurupica spiral phase plate.

Optical vortex, possessing an annular intensity profile and an orbital angular momentum (characterized by an integer termed a topological charge) associated with a helical wavefront, has attracted great attention for diverse applications due to its unique properties. In particular for terahertz (THz) frequency range, several approaches for THz vortex generation, including molded phase plates consisting of metal slit antennas, achromatic polarization elements and binary-diffractive optical elements, have been recently proposed, however, they are typically designed for a specific frequency. Here, we demonstrate highly intense broadband monocycle vortex generation near 0.6 THz by utilizing a polymeric Tsurupica spiral phase plate in combination with tilted-pulse-front optical rectification in a prism-cut LiNbO3 crystal. A maximum peak power of 2.3 MW was obtained for THz vortex output with an expected topological charge of 1.15. Furthermore, we applied the highly intense THz vortex beam for studying unique nonlinear behaviors in bilayer graphene towards the development of nonlinear super-resolution THz microscopy and imaging system.

Evaluation of polarized terahertz waves generated by Cherenkov phase matching.

We report terahertz (THz) wave generation by satisfying Cherenkov phase-matching condition in both s and p polarizations. A dual-wavelength optical parametric oscillator is constructed from two potassium titanium oxide phosphate crystals pumped by a frequency-doubled Nd:YAG laser. By rotating the orientation of both a lithium niobate crystal (LiNbO3) and the polarization of the pump waves, the polarization of the THz wave changes. Due to the difference in the refractive index and absorption, the output power for p polarization is one tenth that for s polarization. A tuning range from 0.2 to 6.5 THz is obtained for s polarization, and from 0.2 to 4.2 and 5.4 to 6.9 THz for p polarization. The extraction efficiency is improved by changing the angle of prism for p polarization, and a large phase change occurs at total internal reflection. Consequently, p-polarized THz waves are optimal for spectroscopic applications.

THz-wave sensing via pump and signal wave detection interacted with evanescent THz waves.

We report a novel sensing technique that uses an evanescent terahertz (THz) wave, without detecting the THz wave directly. When a THz wave generated by Cherenkov phase matching via difference frequency generation undergoes total internal reflection, the evanescent THz wave is subject to a phase change and an amplitude decrease. The reflected THz wave, under the influence of the sample, interferes with the propagating THz wave and the changing electric field of the THz wave interacts with the electric field of the pump waves. We demonstrate a sensing technique for detecting changes in the electric field of near-infrared light, transcribed from changes in the electric field of a THz wave.

Broadband THz-wave generation by satisfying the noncollinear phase-matching condition with a reflected signal beam.

We demonstrated broadband terahertz (THz) wave generation by satisfying the noncollinear phase-matching condition with a reflected signal beam. We constructed a dual-wavelength optical parametric oscillator with two potassium titanium oxide phosphate crystals pumped by a frequency-doubled Nd:YAG laser. The collinear pump and signal waves were irradiated into a lithium niobate crystal. The pump and the signal waves were reflected at the crystal surface. Because the pump and the signal waves have a finite beam diameter, when the reflected signal wave and unreflected pump wave were irradiated at the correct angle, the noncollinear phase-matching condition was satisfied. By changing the incident angle to the crystal, broadband THz-wave generation with a range of over 0.2-7.2 THz was achieved.

Entangled photon generation in two-period quasi-phase-matched parametric down-conversion.

We proposed and demonstrated a simple but deterministic scheme for generating polarization-entangled photon pairs at telecommunication wavelengths with type-II quasi-phase-matched spontaneous parametric down-conversion (QPM-SPDC) having two poling periods. We fabricated a LiNbO3 crystal having two poling periods so as to generate entangled photons at two wavelengths, i.e., 1506 nm and 1594 nm. We characterized the two-photon polarization state with state tomography and confirmed that the state was highly entangled.

Prism-coupled Cherenkov phase-matched terahertz wave generation using a DAST crystal.

Terahertz (THz) wave generation based on nonlinear frequency conversion is a promising method for realizing a tunable monochromatic high-power THz-wave source. Unfortunately, many nonlinear crystals have strong absorption in the THz frequency region. This limits efficient and widely tunable THz-wave generation. The Cherenkov phase-matching method is one of the most promising techniques for overcoming these problems. Here, we propose a prism-coupled Cherenkov phase-matching (PCC-PM) method, in which a prism with a suitable refractive index at THz frequencies is coupled to a nonlinear crystal. This has the following advantages. Many crystals can be used as THz-wave emitters; the phase-matching condition inside the crystal does not have to be observed; the absorption of the crystal does not prevent efficient generation of radiation; and pump sources with arbitrary wavelengths can be employed. Here we demonstrate PCC-PM THz-wave generation using the organic crystal 4-dimethylamino-N-metyl-4-stilbazolium tosylate (DAST) and a Si prism coupler. We obtain THz-wave radiation with tunability of approximately 0.1 to 10 THz and with no deep absorption features resulting from the absorption spectrum of the crystal. The obtained spectra did not depend on the pump wavelength in the range 1300 to 1450 nm. This simple technique shows promise for generating THz radiation using a wide variety of nonlinear crystals.

Cherenkov phase matched THz-wave generation with surfing configuration for bulk lithium nobate crystal.

We demonstrated a Cherenkov phase matched THz-wave generation with surfing configuration for bulk lithium niobate crystal. THz-wave output was enhanced about 50 times by suppressing phase mismatching for THz-wave propagation direction. The suppression was achieved by combining two pumping waves with dual wavelength with finite angle, and THz-frequency was controllable by changing the angle within 2.5 degrees range. Higher frequency THz-wave generation at around 4.0 THz was successfully obtained by the method.

High-resolution time-of-flight terahertz tomography using a femtosecond fiber laser.

High-resolution tomographic imaging is demonstrated using a reflection-type terahertz time-domain spectroscopy. To realize a practical system for general use, a robust all-fiber laser was used as the pump light source. Broadband terahertz waves were generated with the combination of optical pulses compressed to 17 fs using optical fibers and a DAST crystal. Using deconvolution signal processing, the wideband spectrum of the generated terahertz waves provided high-axial resolution leading to successful imaging of a multilayered structure containing a 2-microm-thin GaAs layer. To our knowledge, this is the first demonstration of terahertz tomographic imaging of such a thin layer.

Extremely frequency-widened terahertz wave generation using Cherenkov-type radiation.

Terahertz (THz) wave generation based on nonlinear frequency conversion is promising way for realizing a tunable monochromatic bright THz-wave source. Such a development of efficient and wide tunable THz-wave source depends on discovery of novel brilliant nonlinear crystal. Important factors of a nonlinear crystal for THz-wave generation are, 1. High nonlinearity and 2. Good transparency at THz frequency region. Unfortunately, many nonlinear crystals have strong absorption at THz frequency region. The fact limits efficient and wide tunable THz-wave generation. Here, we show that Cherenkov radiation with waveguide structure is an effective strategy for achieving efficient and extremely wide tunable THz-wave source. We fabricated MgO-doped lithium niobate slab waveguide with 3.8 microm of thickness and demonstrated difference frequency generation of THz-wave generation with Cherenkov phase matching. Extremely frequency-widened THz-wave generation, from 0.1 to 7.2 THz, without no structural dips successfully obtained. The tuning frequency range of waveguided Cherenkov radiation source was extremely widened compare to that of injection seeded-Terahertz Parametric Generator. The tuning range obtained in this work for THz-wave generation using lithium niobate crystal was the widest value in our knowledge. The highest THz-wave energy obtained was about 3.2 pJ, and the energy conversion efficiency was about 10(-5) %. The method can be easily applied for many conventional nonlinear crystals, results in realizing simple, reasonable, compact, high efficient and ultra broad band THz-wave sources.

Generation and detection of broadband coherent terahertz radiation using 17-fs ultrashort pulse fiber laser.

We describe the generation and detection of broadband terahertz radiation using an all-fiber laser. Optical pulses from a mode-locked fiber laser oscillator are compressed using nonlinear and dispersion effects induced in optical fibers, and 17-fs optical pulses with 170-kW peak power are generated at the wavelength region around 1.5 microm. By injecting these pulses into an organic crystal DAST (4-N, N-dimethylamino-4'-N"-methyl-stilbazolium tosylate), broadband terahertz field is radiated at 0.1-25 THz. The frequency region exceeding 20 THz is achieved with a fiber laser for the first time.

Cherenkov phase-matched monochromatic THzwave generation using difference frequency generation with a lithium niobate crystal.

We demonstrated a Cherenkov phase-matching method for monochromatic THz-wave generation using the difference frequency generation process with a lithium niobate crystal, which resulted in high conversion efficiency and wide tunability. We successfully generated monochromatic THz waves across the range 0.2-3.0 THz. We obtained efficient energy conversion in the low frequency region below 0.5 THz, and achieved a flat tuning spectrum by varying the pumping wavelength during THz-wave tuning.

Terahertz-wave generation in a conventional optical fiber.

We theoretically propose surface-emitted and collinear phase-matched terahertz (THz)-wave generation in a conventional optical fiber. The third-order nonlinear effect, four-wave mixing (FWM), is used to generate THz waves in an optical fiber. Surface-emitted THz-wave generation via FWM is realized using a single-mode fiber. Perfect phase matching is obtained at ~800 nm and 1.5 microm pumping, and it follows that third-order polarization in an optical fiber has the same phase at any point. In this situation, the optical fiber acts like a phased array antenna of the THz wave. Collinear phase-matching THz waves are obtained under the same conditions as for surface-emitted THz waves, and the THz wave is propagated in the silica cladding of the optical fiber. This is a promising method for realizing a reasonable THz-wave source.

High-power terahertz-wave generation using DAST crystal and detection using mid-infrared powermeter.

The exact power output of a table-top-sized terahertz (THz)-wave source using a nonlinear optical process has not been clarified because detectors for these experiments [Si bolometer, deuterated triglycine sulfate (DTGS), etc.] are not calibrated well. On the other hand, powermeters for the mid-infrared (mid-IR) region are well established and calibrated. We constructed a high-power dual-wavelength optical parametric oscillator with two KTP crystals as a light source for difference frequency generation. The obtained powers of dual waves were 21 mJ at ~1300 nm, ten times higher than that of the previous measurement. The device provides high-power THz-wave generation with ~100 times greater output power than that reported in previous works. A well-calibrated mid-IR powermeter at ~27 THz detected the generated THz wave; its measured energy was 2.4 microJ. Although the powermeter had no sensitivity in the lower-frequency range (below 20 THz), the pulse energy at such a low-frequency region was estimated in reference to the output spectrum obtained using a DTGS detector: the energy would be from about the submicrojoule level to a few microjoules in the THz-wave region.