Spatially resolved amplitude and phase characterization of femtosecond optical pulses.

Ultrabroadband pulses exhibit a frequency-dependent mode size owing to the wavelength dependence of free-space diffraction. Additionally, rather complex lateral dependence of the temporal pulse shape has been reported for Kerr-lens mode-locked lasers and broadband amplifier chains and in frequency-domain pulse shapers, for example. We demonstrate an ultrashort-pulse characterization technique that reveals lateral pulse-shape variations by spatially resolved amplitude and phase measurements by use of spectral phase interferometry for direct electric-field reconstruction (SPIDER). Unlike with autocorrelation techniques, with SPIDER we can obtain spatially resolved pulse characterization even after the nonlinear process. Thus, with this method the spectral phase of the pulse can be resolved very rapidly along one lateral beam axis in a single measurement.

Collinear type II second-harmonic-generation frequency-resolved optical gating for the characterization of sub-10-fs optical pulses.

For the first time to our knowledge, we demonstrate a collinear frequency-resolved optical gating (FROG) technique that is suitable for the characterization of sub-10-fs pulses. This FROG variant does not suffer from geometrical blurring effects, and a temporal resolution of 1 fs can be achieved without the need for additional aperturing. The apparatus is suitable for subnanojoule pulse energies. We apply this technique for the full characterization of pulses from a Kerr-lens mode-locked Ti:sapphire laser.

Semiconductor saturable-absorber mirror assisted Kerr-lens mode-locked Ti:sapphire laser producing pulses in the two-cycle regime.

Pulses of sub-6-fs duration have been obtained from a Kerr-lens mode-locked Ti:sapphire laser at a repetition rate of 100 MHz and an average power of 300 mW. Fitting an ideal sech(2) to the autocorrelation data yields a 4.8-fs pulse duration, whereas reconstruction of the pulse amplitude profile gives 5.8 fs. The pulse spectrum covers wavelengths from above 950 nm to below 630 nm, extending into the yellow beyond the gain bandwidth of Ti:sapphire. This improvement in bandwidth has been made possible by three key ingredients: carefully designed spectral shaping of the output coupling, better suppression of the dispersion oscillation of the double-chirped mirrors, and a novel broadband semiconductor saturable-absorber mirror.

Characterization of sub-6-fs optical pulses with spectral phase interferometry for direct electric-field reconstruction.

We demonstrate spectral phase interferometry for direct electric-field reconstruction (SPIDER) as a novel method to characterize sub-6-fs pulses with nanojoule pulse energy. SPIDER reconstructs pulse phase and amplitude from a measurement of only two optical spectra by use of a fast noniterative algorithm. SPIDER is well suited to the measurement of ultrabroadband pulses because it is quite insensitive to crystal phase-matching bandwidth and to unknown detector spectral responsivity. Moreover, it combines highly accurate pulse-shape measurement with the potential for online laser system diagnostics at video refresh rates.

Self-starting 6.5-fs pulses from a Ti:sapphire laser.

We demonstrate self-starting 6.5-fs pulses from a Kerr-lens mode-locked Ti:sapphire laser with 200-mW average output power at a pulse repetition rate of ~86 M Hz. This is to our knowledge the shortest pulse ever generated directly from a laser. For dispersion compensation we used a prism pair in combination with double-chirped mirrors, which balances the higher-order dispersion of the prism pair and therefore flattens the average total group-delay dispersion in the laser cavity. For self-starting mode locking we used a broadband semiconductor saturable-absorber mirror.