RESUMO
Cuprate superconductors have the highest critical temperatures (Tc) at ambient pressure, yet a consensus on the superconducting mechanism remains to be established. Finding an empirical parameter that limits the highest reachable Tc can provide crucial insight into this outstanding problem. Here, in the first two Ruddlesden-Popper members of the model Hg-family of cuprates, which are chemically nearly identical and have the highest Tc among all cuprate families, we use inelastic photon scattering to reveal that the energy of magnetic fluctuations may play such a role. In particular, we observe the single-paramagnon spectra to be nearly identical between the two compounds, apart from an energy scale difference of ~30% which matches their difference in Tc. The empirical correlation between paramagnon energy and maximal Tc is further found to extend to other cuprate families with relatively high Tc's, hinting at a fundamental connection between them.
RESUMO
The 5d iridium-based transition metal oxides have gained broad interest because of their strong spin-orbit coupling, which favors new or exotic quantum electronic states. On the other hand, they rarely exhibit more mainstream orders like ferromagnetism due to generally weak electron-electron correlation strength. Here, a proximity-induced ferromagnetic (FM) state with TC ≈ 100 K and strong magnetocrystalline anisotropy is shown in a SrIrO3 (SIO) heterostructure via interfacial charge transfer by using a ferromagnetic insulator in contact with SIO. Electrical transport allows to selectively probe the FM state of the SIO layer and the direct observation of a strong, intrinsic, and positive anomalous Hall effect (AHE). For T ≤ 20 K, the AHE displays unusually large coercive and saturation field, a fingerprint of a strong pseudospin-lattice coupling. A Hall angle, σxy AHE /σxx , larger by an order of magnitude than in typical 3d metals and an FM net moment of about 0.1 µB /Ir, is reported. This emphasizes how efficiently the nontrivial topological band properties of SIO can be manipulated by structural modifications and the exchange interaction with 3d TMOs.