Polarization control of quantum dot emission by chiral photonic crystal slabs.

We investigate theoretically the polarization properties of the quantum dot's (QDs) optical emission from chiral photonic crystal structures made of achiral materials in the absence of external magnetic field at room temperature. The mirror symmetry of the local electromagnetic field is broken in this system due to the decreased symmetry of the chiral modulated layer. As a result, the radiation of randomly polarized QDs normal to the structure becomes partially circularly polarized. The sign and degree of circular polarization are determined by the geometry of the chiral modulated structure and depend on the radiation frequency. A degree of circular polarization up to 99% can be achieved for randomly distributed QDs, and can be close to 100% for some single QDs.

Rotation of a single acetylene molecule on Cu(001) by tunneling electrons in STM.

We study the elementary processes behind one of the pioneering works on scanning tunneling microscope controlled reactions of single molecules [Stipe et al., Phys. Rev. Lett. 81, 1263 (1998)]. Using the Keldysh-Green function approach for the vibrational generation rate in combination with density functional theory calculations to obtain realistic parameters we reproduce the experimental rotation rate of an acetylene molecule on a Cu(100) surface as a function of bias voltage and tunneling current. This combined approach allows us to identify the reaction coordinate mode of the acetylene rotation and its anharmonic coupling with the C-H stretch mode. We show that three different elementary processes, the excitation of C-H stretch, the overtone ladder climbing of the hindered rotational mode, and the combination band excitation together explain the rotation of the acetylene molecule on Cu(100).

Derivation of plasmonic resonances in the Fourier modal method with adaptive spatial resolution and matched coordinates.

A very stable approach for finding optical resonances is to solve an eigenvalue equation that evolves from the linearization of the inverse scattering matrix. In this paper, we show how to use this approach in the Fourier modal method so that advanced coordinate transformation methods such as adaptive spatial resolution and matched coordinates can be included. Furthermore, we present a way that accelerates the computation of the inverse scattering matrix tremendously and allows the derivation of the resonant field distribution inside the structure efficiently.

Resonant mode coupling of optical resonances in stacked nanostructures.

We propose a method to obtain the resonance frequencies of coupled optical modes for a stack of two periodically corrugated slabs. The method is based on the modes in each slab, which are derived by the Fourier modal method in combination with the optical scattering matrix theory. We then use the resonant mode approximation of the scattering matrices to develop a linear eigenvalue problem with dimensions equal to the number of resonant modes. Its solutions are the resonance frequencies of the coupled system and exhibit a good agreement with exact solutions. We demonstrate the capabilities of this method for pairs of planar waveguides and gratings of one-dimensional wires.

Transverse photovoltage induced by circularly polarized light.

We discovered that when circularly polarized light is obliquely incident on a two-dimensional metallic photonic crystal slab, electrical voltage is induced perpendicular to the incident plane. The sign of the signal is reversed by changing the sense of polarization or incident angle. The origin of this transverse photoinduced voltage is explained in terms of the force proportional to the light intensity induced by the asymmetry, which is brought about by the angular momentum of the incident light, along with the modification of local near-surface electromagnetic fields in the slab and field enhancement due to surface plasmon resonance.

Matched coordinates and adaptive spatial resolution in the Fourier modal method.

Several improvements have been introduced for the Fourier modal method in the last fifteen years. Among those, the formulation of the correct factorization rules and adaptive spatial resolution have been crucial steps towards a fast converging scheme, but an application to arbitrary two-dimensional shapes is quite complicated.We present a generalization of the scheme for non-trivial planar geometries using a covariant formulation of Maxwell's equations and a matched coordinate system aligned along the interfaces of the structure that can be easily combined with adaptive spatial resolution. In addition, a symmetric application of Fourier factorization is discussed.

Symmetry breaking in a plasmonic metamaterial at optical wavelength.

We numerically study the effect of structural asymmetry in a plasmonic metamaterial made from gold nanowires. It is reported that optically inactive (i.e., optically dark) particle plasmon modes of the symmetric wire lattice are immediately coupled to the radiation field, when a broken structural symmetry is introduced. Such higher order plasmon resonances are characterized by their subradiant nature. They generally reveal long lifetimes and distinct absorption losses. It is shown that the near-field interaction strongly determines these modes.