Continuous Generation of Quantum Light from a Single Ground-State Atom in an Optical Cavity.

We show an optical wave-mixing scheme that generates quantum light by means of a single three-level atom. The atom couples to an optical cavity and two laser fields that together drive a cycling current within the atom. Weak driving in combination with strong atom-cavity coupling induces transitions in a harmonic ladder of dark states, accompanied by single-photon emission via a quantum Zeno effect and suppression of atomic excitation via quantum interference. For strong driving, the system can generate coherent or Schrödinger cat-like fields with frequencies distinct from those of the applied lasers.

Two-Photon Blockade in an Atom-Driven Cavity QED System.

Photon blockade is a dynamical quantum-nonlinear effect in driven systems with an anharmonic energy ladder. For a single atom strongly coupled to an optical cavity, we show that atom driving gives a decisively larger optical nonlinearity than cavity driving. This enhances single-photon blockade and allows for the implementation of two-photon blockade where the absorption of two photons suppresses the absorption of further photons. As a signature, we report on three-photon antibunching with simultaneous two-photon bunching observed in the light emitted from the cavity. Our experiment constitutes a significant step towards multiphoton quantum-nonlinear optics.