Generation of femtosecond radiation at 211 nm by femtosecond pulse upconversion in the field of a picosecond pulse.

We show that, in the case of sum-frequency mixing, one can alleviate group-velocity mismatch between IR and UV pulses by choosing different pulse widths, thus extending the interaction length of ultrashort pulses within nonlinear crystals. By fifth-harmonic generation with a Nd:glass laser, we demonstrate efficient frequency upconversion of 195-fs 264-nm pulses under the envelope of 0.9-ps 1055-nm pulses in beta-barium borate crystal, yielding <270-fs pulses with energy of up to 110muJ at 211 nm.

Two-Photon Absorbing Properties of Ultraviolet Phase-Matchable Crystals at 264 and 211 nm.

We investigated the intensity-dependent loss properties of nonlinear crystals by using subpicosecond laser pulses at 264 and 211 nm. Two-photon absorption coefficients for potassium dihydrogen phosphate, beta-barium borate, and lithium triborate crystals were obtained from the intensity-dependent transmission measurements.

Near-degenerate cascaded four-wave mixing in an optical parametric amplifier.

Efficient generation of new spectral components owing to second-order cascading in a seeded broadband beta -barium borate typeI phase-matching parametric amplifier is demonstrated. One can vary the number and magnitude of these components by changing amplification bandwidth (wavelength) and phase-matching conditions. The phenomenon is treated theoretically by use of a formalism developed previously for the case of cascaded self-diffraction.