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1.
Nature ; 626(7999): 505-511, 2024 Feb.
Artigo em Inglês | MEDLINE | ID: mdl-38356069

RESUMO

Non-Abelian topological order is a coveted state of matter with remarkable properties, including quasiparticles that can remember the sequence in which they are exchanged1-4. These anyonic excitations are promising building blocks of fault-tolerant quantum computers5,6. However, despite extensive efforts, non-Abelian topological order and its excitations have remained elusive, unlike the simpler quasiparticles or defects in Abelian topological order. Here we present the realization of non-Abelian topological order in the wavefunction prepared in a quantum processor and demonstrate control of its anyons. Using an adaptive circuit on Quantinuum's H2 trapped-ion quantum processor, we create the ground-state wavefunction of D4 topological order on a kagome lattice of 27 qubits, with fidelity per site exceeding 98.4 per cent. By creating and moving anyons along Borromean rings in spacetime, anyon interferometry detects an intrinsically non-Abelian braiding process. Furthermore, tunnelling non-Abelions around a torus creates all 22 ground states, as well as an excited state with a single anyon-a peculiar feature of non-Abelian topological order. This work illustrates the counterintuitive nature of non-Abelions and enables their study in quantum devices.

2.
Phys Rev Lett ; 131(20): 200201, 2023 Nov 17.
Artigo em Inglês | MEDLINE | ID: mdl-38039472

RESUMO

In the field of monitored quantum circuits, it has remained an open question whether finite-time protocols for preparing long-range entangled states lead to phases of matter that are stable to gate imperfections, that can convert projective into weak measurements. Here, we show that in certain cases, long-range entanglement persists in the presence of weak measurements, and gives rise to novel forms of quantum criticality. We demonstrate this explicitly for preparing the two-dimensional Greenberger-Horne-Zeilinger cat state and the three-dimensional toric code as minimal instances. In contrast to random monitored circuits, our circuit of gates and measurements is deterministic; the only randomness is in the measurement outcomes. We show how the randomness in these weak measurements allows us to track the solvable Nishimori line of the random-bond Ising model, rigorously establishing the stability of the glassy long-range entangled states in two and three spatial dimensions. Away from this exactly solvable construction, we use hybrid tensor network and Monte Carlo simulations to obtain a nonzero Edwards-Anderson order parameter as an indicator of long-range entanglement in the two-dimensional scenario. We argue that our protocol admits a natural implementation in existing quantum computing architectures, requiring only a depth-3 circuit on IBM's heavy-hexagon transmon chips.

3.
Phys Rev Lett ; 131(18): 186301, 2023 Nov 03.
Artigo em Inglês | MEDLINE | ID: mdl-37977617

RESUMO

We propose a new formula that extracts the quantum Hall conductance from a single (2+1)D gapped wave function. The formula applies to general many-body systems that conserve particle number, and is based on the concept of modular flow, i.e., unitary dynamics generated from the entanglement structure of the wave function. The formula is shown to satisfy all formal properties of the Hall conductance: it is odd under time reversal and reflection, even under charge conjugation, universal and topologically rigid in the thermodynamic limit. Further evidence for relating the formula to the Hall conductance is obtained from conformal field theory arguments. Finally, we numerically check the formula by applying it to a noninteracting Chern band where excellent agreement is obtained.

4.
Phys Rev Lett ; 131(13): 136502, 2023 Sep 29.
Artigo em Inglês | MEDLINE | ID: mdl-37832017

RESUMO

The pursuit of exotic phases of matter outside of the extreme conditions of a quantizing magnetic field is a long-standing quest of solid state physics. Recent experiments have observed spontaneous valley polarization and fractional Chern insulators in zero magnetic field in twisted bilayers of MoTe_{2}, at partial filling of the topological valence band (ν=-2/3 and -3/5). We study the topological valence band at half filling, using exact diagonalization and density matrix renormalization group calculations. We discover a composite Fermi liquid (CFL) phase even at zero magnetic field that covers a large portion of the phase diagram near twist angle ∼3.6°. The CFL is a non-Fermi liquid phase with metallic behavior despite the absence of Landau quasiparticles. We discuss experimental implications including the competition between the CFL and a Fermi liquid, which can be tuned with a displacement field. The topological valence band has excellent quantum geometry over a wide range of twist angles and a small bandwidth that is, remarkably, reduced by interactions. These key properties stabilize the exotic zero field quantum Hall phases. Finally, we present an optical signature involving "extinguished" optical responses that detects Chern bands with ideal quantum geometry.

5.
Phys Rev Lett ; 131(6): 060405, 2023 Aug 11.
Artigo em Inglês | MEDLINE | ID: mdl-37625044

RESUMO

A highly coveted goal is to realize emergent non-Abelian gauge theories and their anyonic excitations, which encode decoherence-free quantum information. While measurements in quantum devices provide new hope for scalably preparing such long-range entangled states, existing protocols using the experimentally established ingredients of a finite-depth circuit and a single round of measurement produce only Abelian states. Surprisingly, we show there exists a broad family of non-Abelian states-namely those with a Lagrangian subgroup-which can be created using these same minimal ingredients, bypassing the need for new resources such as feed forward. To illustrate that this provides realistic protocols, we show how D_{4} non-Abelian topological order can be realized, e.g., on Google's quantum processors using a depth-11 circuit and a single layer of measurements. Our work opens the way toward the realization and manipulation of non-Abelian topological orders, and highlights counterintuitive features of the complexity of non-Abelian phases.

6.
Nat Mater ; 22(5): 583-590, 2023 May.
Artigo em Inglês | MEDLINE | ID: mdl-36894774

RESUMO

Using circularly polarized light to control quantum matter is a highly intriguing topic in physics, chemistry and biology. Previous studies have demonstrated helicity-dependent optical control of chirality and magnetization, with important implications in asymmetric synthesis in chemistry; homochirality in biomolecules; and ferromagnetic spintronics. We report the surprising observation of helicity-dependent optical control of fully compensated antiferromagnetic order in two-dimensional even-layered MnBi2Te4, a topological axion insulator with neither chirality nor magnetization. To understand this control, we study an antiferromagnetic circular dichroism, which appears only in reflection but is absent in transmission. We show that the optical control and circular dichroism both arise from the optical axion electrodynamics. Our axion induction provides the possibility to optically control a family of [Formula: see text]-symmetric antiferromagnets ([Formula: see text], inversion; [Formula: see text], time-reversal) such as Cr2O3, even-layered CrI3 and possibly the pseudo-gap state in cuprates. In MnBi2Te4, this further opens the door for optical writing of a dissipationless circuit formed by topological edge states.

7.
Nat Mater ; 22(3): 316-321, 2023 Mar.
Artigo em Inglês | MEDLINE | ID: mdl-36550373

RESUMO

Magic-angle twisted trilayer graphene (MATTG) hosts flat electronic bands, and exhibits correlated quantum phases with electrical tunability. In this work, we demonstrate a spectroscopy technique that allows for dissociation of intertwined bands and quantification of the energy gaps and Chern numbers C of the correlated states in MATTG by driving band crossings between Dirac cone Landau levels and energy gaps in the flat bands. We uncover hard correlated gaps with C = 0 at integer moiré unit cell fillings of ν = 2 and 3 and reveal charge density wave states originating from van Hove singularities at fractional fillings ν = 5/3 and 11/3. In addition, we demonstrate displacement-field-driven first-order phase transitions at charge neutrality and ν = 2, which are consistent with a theoretical strong-coupling analysis, implying C2T symmetry breaking. Overall, these properties establish a diverse electrically tunable phase diagram of MATTG and provide an avenue for investigating other related systems hosting both steep and flat bands.

8.
Nat Commun ; 13(1): 7615, 2022 Dec 09.
Artigo em Inglês | MEDLINE | ID: mdl-36494356

RESUMO

Emergent axion electrodynamics in magneto-electric media is expected to provide novel ways to detect and control material properties with electromagnetic fields. However, despite being studied intensively for over a decade, its theoretical understanding remains mostly confined to the static limit. Here, we introduce a theory of axion electrodynamics at general frequencies. We define a proper optical axion magneto-electric coupling through its relation to optical surface Hall conductivity and provide ways to calculate it in lattice systems. By employing our formulas, we show that axion electrodynamics can lead to a significant Kerr effect in thin-film antiferromagnets at wavelengths that are seemingly too long to resolve the spatial modulation of magnetism. We identify the wavelength scale above which the Kerr effect is suppressed. Our theory is particularly relevant to materials like MnBi2Te4, a topological antiferromagnet whose magneto-electric response is shown here to be dominated by the axion contribution even at optical frequencies.


Assuntos
Imagem de Difusão por Ressonância Magnética , Eletricidade , Condutividade Elétrica , Campos Eletromagnéticos
9.
Nat Commun ; 13(1): 6245, 2022 Oct 21.
Artigo em Inglês | MEDLINE | ID: mdl-36271002

RESUMO

The advent of moiré materials has galvanized interest in the nature of charge carriers in topological bands. In contrast to conventional materials with electron-like charge carriers, topological bands allow for more exotic possibilities where charge is carried by nontrivial topological textures, such as skyrmions. However, the real-space description of skyrmions is ill-suited to address the limit of small skyrmions and to account for momentum-space band features. Here, we develop a momentum-space approach to study the formation of the smallest skyrmions - spin polarons, formed as bound states of an electron and a spin flip - in topological ferromagnets. We show that, quite generally, there is an attraction between an electron and a spin flip that is purely topological in origin, promoting the formation of spin polarons. Applying our results to twisted bilayer graphene, we identify a range of parameters where spin polarons are formed and discuss their possible experimental signatures.

10.
Phys Rev Lett ; 129(9): 090501, 2022 Aug 26.
Artigo em Inglês | MEDLINE | ID: mdl-36083646

RESUMO

It has recently been established that clusterlike states-states that are in the same symmetry-protected topological phase as the cluster state-provide a family of resource states that can be utilized for measurement-based quantum computation. In this Letter, we ask whether it is possible to prepare clusterlike states in finite time without breaking the symmetry protecting the resource state. Such a symmetry-preserving protocol would benefit from topological protection to errors in the preparation. We answer this question in the positive by providing a Hamiltonian in one higher dimension whose finite-time evolution is a unitary that acts trivially in the bulk, but pumps the desired cluster state to the boundary. Examples are given for both the 1D cluster state protected by a global symmetry, and various 2D cluster states protected by subsystem symmetries. We show that even if unwanted symmetric perturbations are present in the driving Hamiltonian, projective measurements in the bulk along with feed-forward correction is sufficient to recover a clusterlike state.

11.
Phys Rev Lett ; 128(17): 176404, 2022 Apr 29.
Artigo em Inglês | MEDLINE | ID: mdl-35570445

RESUMO

We consider a family of twisted graphene multilayers consisting of n-untwisted chirally stacked layers, e.g., AB, ABC, etc, with a single twist on top of m-untwisted chirally stacked layers. Upon neglecting both trigonal warping terms for the untwisted layers and the same sublattice hopping between all layers, the resulting models generalize several remarkable features of the chiral model of twisted bilayer graphene (CTBG). In particular, they exhibit a set of magic angles which are identical to those of CTBG at which a pair of bands (i) are perfectly flat, (ii) have Chern numbers in the sublattice basis given by ±(n,-m) or ±(n+m-1,-1) depending on the stacking chirality, and (iii) satisfy the trace condition, saturating an inequality between the quantum metric and the Berry curvature, and thus realizing ideal quantum geometry. These are the first higher Chern bands that satisfy (iii) beyond fine-tuned models or combinations of Landau levels. We show that ideal quantum geometry is directly related to the construction of fractional quantum Hall model wave functions. We provide explicit analytic expressions for the flatband wave functions at the magic angle in terms of the CTBG wave functions. We also show that the Berry curvature distribution in these models can be continuously tuned while maintaining perfect quantum geometry. Similar to the study of fractional Chern insulators in ideal C=1 bands, these models pave the way for investigating exotic topological phases in higher Chern bands for which no Landau level analog is available.

12.
Proc Natl Acad Sci U S A ; 119(16): e2118482119, 2022 Apr 19.
Artigo em Inglês | MEDLINE | ID: mdl-35412918

RESUMO

SignificanceWhen two sheets of graphene are twisted to the magic angle of 1.1∘, the resulting flat moiré bands can host exotic correlated electronic states such as superconductivity and ferromagnetism. Here, we show transport properties of a twisted bilayer graphene device at 1.38∘, far enough above the magic angle that we do not expect exotic correlated states. Instead, we see several unusual behaviors in the device's resistivity upon tuning both charge carrier density and perpendicular magnetic field. We can reproduce these behaviors with a surprisingly simple model based on Hofstadter's butterfly. These results shed light on the underlying properties of twisted bilayer graphene.

13.
Nature ; 600(7889): 439-443, 2021 12.
Artigo em Inglês | MEDLINE | ID: mdl-34912084

RESUMO

Fractional Chern insulators (FCIs) are lattice analogues of fractional quantum Hall states that may provide a new avenue towards manipulating non-Abelian excitations. Early theoretical studies1-7 have predicted their existence in systems with flat Chern bands and highlighted the critical role of a particular quantum geometry. However, FCI states have been observed only in Bernal-stacked bilayer graphene (BLG) aligned with hexagonal boron nitride (hBN)8, in which a very large magnetic field is responsible for the existence of the Chern bands, precluding the realization of FCIs at zero field. By contrast, magic-angle twisted BLG9-12 supports flat Chern bands at zero magnetic field13-17, and therefore offers a promising route towards stabilizing zero-field FCIs. Here we report the observation of eight FCI states at low magnetic field in magic-angle twisted BLG enabled by high-resolution local compressibility measurements. The first of these states emerge at 5 T, and their appearance is accompanied by the simultaneous disappearance of nearby topologically trivial charge density wave states. We demonstrate that, unlike the case of the BLG/hBN platform, the principal role of the weak magnetic field is merely to redistribute the Berry curvature of the native Chern bands and thereby realize a quantum geometry favourable for the emergence of FCIs. Our findings strongly suggest that FCIs may be realized at zero magnetic field and pave the way for the exploration and manipulation of anyonic excitations in flat moiré Chern bands.

14.
Phys Rev Lett ; 127(24): 247701, 2021 Dec 10.
Artigo em Inglês | MEDLINE | ID: mdl-34951785

RESUMO

We propose a moiré bilayer as a platform where exotic quantum phases can be stabilized and electrically detected. Moiré bilayers consist of two separate moiré superlattice layers coupled through the interlayer Coulomb repulsion. In the small distance limit, an SU(4) spin can be formed by combining layer pseudospin and the real spin. As a concrete example, we study an SU(4) spin model on triangular lattice in the fundamental representation. By tuning a three-site ring exchange term K∼(t^{3}/U^{2}), we find the SU(4) symmetric crystallized phase and an SU(4)_{1} chiral spin liquid at the balanced filling. We also predict two different exciton supersolid phases with interlayer coherence at imbalanced filling under displacement field. Especially, the system can simulate an SU(2) Bose-Einstein condensation by injecting interlayer excitons into the magnetically ordered Mott insulator at the layer polarized limit. Smoking gun evidences of these phases can be obtained by measuring the pseudospin transport in the counterflow channel.

15.
Sci Adv ; 7(19)2021 May.
Artigo em Inglês | MEDLINE | ID: mdl-33952523

RESUMO

Topological solitons, a class of stable nonlinear excitations, appear in diverse domains as in the Skyrme model of nuclear forces. Here, we argue that similar excitations play an important role in a remarkable material obtained on stacking and twisting two sheets of graphene. Close to a magic twist angle, insulating behavior is observed, which gives way to superconductivity on doping. Here, we propose a unifying description of both observations. A symmetry breaking condensate leads to the ordered insulator, while topological solitons in the condensate-skyrmions-are shown to be charge 2e bosons. Condensation of skyrmions leads to a superconductor, whose physical properties we calculate. More generally, we show how topological textures can mitigate Coulomb repulsion and provide a previously unexplored route to superconductivity. Our mechanism not only clarifies why several other moiré materials do not show superconductivity but also points to unexplored platforms where robust superconductivity is anticipated.

16.
Nat Commun ; 12(1): 2732, 2021 May 12.
Artigo em Inglês | MEDLINE | ID: mdl-33980832

RESUMO

Moiré superlattices created by the twisted stacking of two-dimensional crystals can host electronic bands with flat energy dispersion in which enhanced interactions promote correlated electron states. The twisted double bilayer graphene (TDBG), where two Bernal bilayer graphene are stacked with a twist angle, is such a moiré system with tunable flat bands. Here, we use gate-tuned scanning tunneling spectroscopy to directly demonstrate the tunability of the band structure of TDBG with an electric field and to show spectroscopic signatures of electronic correlations and topology for its flat band. Our spectroscopic experiments are in agreement with a continuum model of TDBG band structure and reveal signatures of a correlated insulator gap at partial filling of its isolated flat band. The topological properties of this flat band are probed with the application of a magnetic field, which leads to valley polarization and the splitting of Chern bands with a large effective g-factor.

17.
Science ; 371(6534): 1133-1138, 2021 03 12.
Artigo em Inglês | MEDLINE | ID: mdl-33542148

RESUMO

Engineering moiré superlattices by twisting layers in van der Waals (vdW) heterostructures has uncovered a wide array of quantum phenomena. We constructed a vdW heterostructure that consists of three graphene layers stacked with alternating twist angles ±Î¸. At the average twist angle θ ~ 1.56°, a theoretically predicted "magic angle" for the formation of flat electron bands, we observed displacement field-tunable superconductivity with a maximum critical temperature of 2.1 kelvin. By tuning the doping level and displacement field, we found that superconducting regimes occur in conjunction with flavor polarization of moiré bands and are bounded by a van Hove singularity (vHS) at high displacement fields. Our findings display inconsistencies with a weak coupling description, suggesting that the observed moiré superconductivity has an unconventional nature.

18.
Nature ; 583(7815): 221-225, 2020 07.
Artigo em Inglês | MEDLINE | ID: mdl-32641816

RESUMO

Reducing the energy bandwidth of electrons in a lattice below the long-range Coulomb interaction energy promotes correlation effects. Moiré superlattices-which are created by stacking van der Waals heterostructures with a controlled twist angle1-3-enable the engineering of electron band structure. Exotic quantum phases can emerge in an engineered moiré flat band. The recent discovery of correlated insulator states, superconductivity and the quantum anomalous Hall effect in the flat band of magic-angle twisted bilayer graphene4-8 has sparked the exploration of correlated electron states in other moiré systems9-11. The electronic properties of van der Waals moiré superlattices can further be tuned by adjusting the interlayer coupling6 or the band structure of constituent layers9. Here, using van der Waals heterostructures of twisted double bilayer graphene (TDBG), we demonstrate a flat electron band that is tunable by perpendicular electric fields in a range of twist angles. Similarly to magic-angle twisted bilayer graphene, TDBG shows energy gaps at the half- and quarter-filled flat bands, indicating the emergence of correlated insulator states. We find that the gaps of these insulator states increase with in-plane magnetic field, suggesting a ferromagnetic order. On doping the half-filled insulator, a sudden drop in resistivity is observed with decreasing temperature. This critical behaviour is confined to a small area in the density-electric-field plane, and is attributed to a phase transition from a normal metal to a spin-polarized correlated state. The discovery of spin-polarized correlated states in electric-field-tunable TDBG provides a new route to engineering interaction-driven quantum phases.

19.
Phys Rev Lett ; 123(20): 206404, 2019 Nov 15.
Artigo em Inglês | MEDLINE | ID: mdl-31809078

RESUMO

The hallmark of symmetry-protected topological phases is the existence of anomalous boundary states, which can only be realized with the corresponding bulk system. In this work, we show that for every Hermitian anomalous boundary mode of the ten Altland-Zirnbauer classes, a non-Hermitian counterpart can be constructed, whose long-time dynamics provides a realization of the anomalous boundary state. We prove that the non-Hermitian counterpart is characterized by a point-gap topological invariant, and furthermore, that the invariant exactly matches that of the corresponding Hermitian anomalous boundary mode. We thus establish a correspondence between the topological classifications of (d+1)-dimensional gapped Hermitian systems and d-dimensional point-gapped non-Hermitian systems. We illustrate this general result with a number of examples in different dimensions. This work provides a new perspective on point-gap topological invariants in non-Hermitian systems.

20.
Nat Commun ; 10(1): 5333, 2019 11 25.
Artigo em Inglês | MEDLINE | ID: mdl-31767862

RESUMO

Two graphene monolayers twisted by a small magic angle exhibit nearly flat bands, leading to correlated electronic states. Here we study a related but different system with reduced symmetry - twisted double bilayer graphene (TDBG), consisting of two Bernal stacked bilayer graphenes, twisted with respect to one another. Unlike the monolayer case, we show that isolated flat bands only appear on application of a vertical displacement field. We construct a phase diagram as a function of twist angle and displacement field, incorporating interactions via a Hartree-Fock approximation. At half-filling, ferromagnetic insulators are stabilized with valley Chern number [Formula: see text]. Upon doping, ferromagnetic fluctuations are argued to lead to spin-triplet superconductivity from pairing between opposite valleys. We highlight a novel orbital effect arising from in-plane fields plays an important role in interpreting experiments. Combined with recent experimental findings, our results establish TDBG as a tunable platform to realize rare phases in conventional solids.

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