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1.
Adv Mater ; 34(38): e2205677, 2022 Sep.
Artigo em Inglês | MEDLINE | ID: mdl-35924314

RESUMO

The lithium (Li)-metal anode offers a promising solution for high-energy-density lithium-metal batteries (LMBs). However, the significant volume expansion of the Li metal during charging results in poor cycling stability as a result of the dendritic deposition and broken solid electrolyte interphase. Herein, a facile one-step roll-to-roll fabrication of a zero-volume-expansion Li-metal-composite anode (zeroVE-Li) is proposed to realize high-energy-density LMBs with outstanding electrochemical and mechanical stability. The zeroVE-Li possesses a sandwich-like trilayer structure, which consists of an upper electron-insulating layer and a bottom lithiophilic layer that synergistically guides the Li deposition from the bottom up, and a middle porous layer that eliminates volume expansion. This sandwich structure eliminates dendrite formation, prevents volume change during cycling, and provides outstanding flexibility to the Li-metal anode even at a practical areal capacity over 3.0 mAh cm-2 . Pairing zeroVE-Li with a commercial NMC811 or LCO cathode, flexible LMBs that offer a record-breaking figure of merit (FOM, 45.6), large whole-cell energy density (375 Wh L-1 , based on the volume of the anode, separator, cathode, and package), high-capacity retention (> 99.8% per cycle), and remarkable mechanical robustness under practical conditions are demonstrated.

3.
Cad Saude Publica ; 36(11): e00123719, 2020.
Artigo em Inglês | MEDLINE | ID: mdl-33237201

RESUMO

This study aimed to illustrate the impact of injury-related deaths on life expectancy in China in 2016 and to identify the high-risk population. Standard life tables were used to calculate life expectancy and cause-eliminated life expectancy by utilizing mortality data from the national mortality surveillance system. In 2016, the life expectancy of Chinese residents was 78.91 years. After eliminating injury-related mortality, the life expectancy of the residents increased by 1.13 years, which was higher in male and rural residents compared with female and urban residents. The life expectancy on the Eastern and Central regions increased slowly compared with the Western region. The greatest influencing factor on life expectancy was road traffic injuries, followed by falls. Falls had a greater impact on life expectancy for children under 5 years old and those aged over 65 years. This study indicates that deaths caused by injury had a noteworthy impact on life expectancy in China. More attention should be paid to road traffic injuries, and effective preventive measures should be taken to reduce deaths related to injury to increase the life expectancy of residents, especially in children under 5 years and adults over 65 years. By reducing the deaths caused by injury, the life expectancy level is likely to further improve.


Assuntos
Expectativa de Vida , População Rural , Adulto , Idoso , Brasil , Causas de Morte , Criança , Pré-Escolar , China/epidemiologia , Feminino , Humanos , Tábuas de Vida , Masculino
4.
Front Chem ; 8: 241, 2020.
Artigo em Inglês | MEDLINE | ID: mdl-32300584

RESUMO

Hard carbon derived from fossil products is widely used as anode material for lithium-ion batteries. However, there are still several main shortcomings such as high cost, and poor rate performance, which restrict its wide application. Then tremendous efforts have been devoted to developing biomaterials in the battery applications. Recently, especially agricultural and industrial by-products have attracted much attention due to the electric double-layer capacitors. Herein, we report the sulfur-doped hard carbon (SHC) materials from the tannin-furanic resins (TF-Resin) of the derived agricultural by-products, followed by enveloping rGO on its surface through the hexadecyl trimethyl ammonium bromide. SHC provides sites for the storage of lithium, while the rGO layers can offer a highly conductive matrix to achieve good contact between particles and promote the diffusion and transport of ions and electrons. As a result, the SHC@rGO shows excellent lithium storage performance with initial discharge capacity around 746 mAh g-1 at a current density of 50 mA g-1, and shows superb stability keeping capacity retention of 91.9% after 200 cycles. Moreover, even at a high current density of 2,000 mAg-1, SHC@rGO still delivers a specific capacity of 188 mAg-1. These desired promising properties are active to the implement in the possible practical application.

5.
Cad. Saúde Pública (Online) ; 36(11): e00123719, 2020. tab, graf
Artigo em Inglês | LILACS, Sec. Est. Saúde SP | ID: biblio-1132843

RESUMO

Abstract: This study aimed to illustrate the impact of injury-related deaths on life expectancy in China in 2016 and to identify the high-risk population. Standard life tables were used to calculate life expectancy and cause-eliminated life expectancy by utilizing mortality data from the national mortality surveillance system. In 2016, the life expectancy of Chinese residents was 78.91 years. After eliminating injury-related mortality, the life expectancy of the residents increased by 1.13 years, which was higher in male and rural residents compared with female and urban residents. The life expectancy on the Eastern and Central regions increased slowly compared with the Western region. The greatest influencing factor on life expectancy was road traffic injuries, followed by falls. Falls had a greater impact on life expectancy for children under 5 years old and those aged over 65 years. This study indicates that deaths caused by injury had a noteworthy impact on life expectancy in China. More attention should be paid to road traffic injuries, and effective preventive measures should be taken to reduce deaths related to injury to increase the life expectancy of residents, especially in children under 5 years and adults over 65 years. By reducing the deaths caused by injury, the life expectancy level is likely to further improve.


Resumo: O estudo teve como objetivos analisar o impacto dos óbitos por causas externas na expectativa de vida na China em 2016 e identificar a população de risco. Foram utilizadas tábuas de mortalidade padronizadas para calcular a expectativa de vida e a expectativa de vida depois de eliminar as causas externas, com base nos dados de mortalidade do Sistema Nacional de Vigilância da Mortalidade. Em 2016, a expectativa de vida dos chineses era 78,91 anos. Depois de eliminar a mortalidade por causas externas, a expectativa de vida dos chineses aumentou em 1,13 anos, e o aumento foi maior nos homens e nos moradores da área rural, comparados às mulheres e aos moradores da área urbana. A expectativa de vida das regiões Leste e Central aumentou mais lentamente do que na região Oeste do país. Os acidentes de trânsito foram o fator de maior impacto sobre a expectativa de vida, seguidos de quedas. As quedas tiveram um impacto maior sobre a expectativa de vida nas crianças abaixo de 5 anos e nos idosos acima de 65 anos de idade. O estudo indica que os óbitos por causas externas tiveram um impacto relevante na expectativa de vida na China. As lesões por acidentes de trânsito merecem mais atenção, e medidas efetivas devem ser tomadas para reduzir os óbitos por causas externas para aumentar a expectativa de vida na população chinesa, principalmente nas crianças abaixo de 5 anos e nos idosos acima de 65 anos. A redução dos óbitos por causas externas deverá melhorar mais ainda o nível de expectativa de vida.


Resumen: El objetivo de este estudio fue ilustrar el impacto de los fallecimientos relacionados con lesiones y la esperanza de vida en China en 2016, así como identificar a la población de alto riesgo. Las tablas de estándar de vida se utilizaron para calcular la esperanza de vida y la causa de la supresión de esperanza de vida se calculó utilizando datos de mortalidad del sistema de vigilancia de la mortalidad. En 2016, la esperanza de vida de los chinos residentes era 78,91 años. Tras eliminar la mortalidad relacionada con lesiones, la esperanza de vida de los residentes se incrementó en 1,13 años, que fue mayor en hombres, residentes en áreas rurales, comparada con las mujeres, residentes en áreas urbanas. La esperanza de vida en las regiones orientales y centrales se incrementó lentamente, comparada con la región occidental. El factor de mayor influencia en la esperanza de vida fue las lesiones en accidentes de tráfico, seguidas de las caídas. Las caídas tuvieron un impacto mayor en la esperanza de vida para los niños menores de 5 años, así como los ancianos con una edad por encima de los 65 años. Este estudio indica que las muertes causadas por lesiones tuvieron un impacto notorio en la esperanza de vida en China. Se debe prestar más atención a las lesiones por accidente de tráfico, y se deberían tomar medidas preventivas efectivas para reducir las muertes relacionadas con las lesiones para incrementar la esperanza de vida de los residentes, especialmente en niños menores de 5 años y personas mayores con más de 65 años. Si se reducen las muertes causadas por lesiones, cabe esperar que mejore el nivel de esperanza de vida.


Assuntos
Humanos , Masculino , Feminino , Pré-Escolar , Criança , Adulto , Idoso , População Rural , Expectativa de Vida , Brasil , China/epidemiologia , Causas de Morte , Tábuas de Vida
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