Characterization of sub-20-attosecond timing jitter in erbium-doped fiber laser system.

The significance of timing jitter stems from its pivotal role in enhancing the precision of applications like spectroscopy and frequency metrology. In this study, we introduce a comprehensive procedure for achieving low timing jitter values in mode-locked fiber laser systems, highlighting dispersion, intracavity pulse energy, pulse length, and spectral bandwidth as key parameters. Notably, we unveil the influence of fiber amplifier pump power on jitter, a factor neglected in established theories and recent experiments. Applying this procedure to a 200-MHz all-polarization-maintaining (PM) erbium-doped (Er:) nonlinear amplifying loop mirror (NALM) fiber laser system, we demonstrate an exceptionally low timing jitter of 14.25 attoseconds, measured using the balanced optical cross-correlation (BOC) technique and integrated from 10 kHz to 4 MHz. The implementation of our novel method offers the opportunity to improve jitter results in various fiber laser systems and increase the accuracy of fiber laser applications.

End-to-end topology for fiber comb based optical frequency transfer at the 10-21 level: erratum.

In this erratum we correct errors in the scaling and caption of Fig. 4 in the original manuscript [1].

Comb-locked frequency-swept synthesizer for high precision broadband spectroscopy.

Frequency combs have made optical metrology accessible to hundreds of laboratories worldwide and they have set new benchmarks in multi-species trace gas sensing for environmental, industrial and medical applications. However, current comb spectrometers privilege either frequency precision and sensitivity through interposition of a cw probe laser with limited tuning range, or spectral coverage and measurement time using the comb itself as an ultra-broadband probe. We overcome this restriction by introducing a comb-locked frequency-swept optical synthesizer that allows a continuous-wave laser to be swept in seconds over spectral ranges of several terahertz while remaining phase locked to an underlying frequency comb. This offers a unique degree of versatility, as the synthesizer can be either repeatedly scanned over a single absorption line to achieve ultimate precision and sensitivity, or swept in seconds over an entire rovibrational band to capture multiple species. The spectrometer enables us to determine line center frequencies with an absolute uncertainty of 30 kHz and at the same time to collect absorption spectra over more than 3 THz with state-of-the-art sensitivity of a few 10-10 cm-1. Beyond precision broadband spectroscopy, the proposed synthesizer is an extremely promising tool to force a breakthrough in terahertz metrology and coherent laser ranging.

End-to-end topology for fiber comb based optical frequency transfer at the 10-21 level.

We introduce a simple and robust scheme for optical frequency transfer of an ultra-stable source light field via an optical frequency comb to a field at a target optical frequency, where highest stability is required, e.g., for the interrogation of an optical clock. The scheme relies on a topology for end-to-end suppression of the influence of optical path-length fluctuations, which is attained by actively phase-stabilized delivery, combined with common-path propagation. This approach provides a robust stability improvement without the need for additional isolation against environmental disturbances such as temperature, pressure or humidity changes. We measure residual frequency transfer instabilities by comparing the frequency transfers carried out with two independent combs simultaneously. Residual fractional frequency instabilities between two systems of 8 × 10-18 at 1 s and 3 × 10-21 at 105 s averaging time are observed. We discuss the individual noise contributions to the residual instability. The presented scheme is technically simple, robust against environmental parameter fluctuations and enables an ultra-stable frequency transfer, e.g., to optical clock lasers or to lasers in gravitational wave detectors.

Molecular properties of liquid crystals in the terahertz frequency range.

We report on a first experimental study of the molecular properties of nematic liquid crystals in the terahertz range. In the beginning, we extract the frequency and temperature dependent refractive index and absorption coefficient of the cyanobiphenyls 5CB, 6CB and 7CB from terahertz time domain spectroscopy measurements and investigate the impact of the alkyl chain length on the macroscopic liquid crystal characteristics, focusing especially on the pronounced odd and even effect. Next, we deduce the principle polarizabilities and the order parameter S by applying Vuks' approximation and Haller's approach. On this basis, we calculate the main polarizabilities along the longitudinal and transverse axis and link the observed terahertz properties to the molecular structure of the liquid crystals.

Optical sampling by laser cavity tuning.

Most time-resolved optical experiments rely either on external mechanical delay lines or on two synchronized femtosecond lasers to achieve a defined temporal delay between two optical pulses. Here, we present a new method which does not require any external delay lines and uses only a single femtosecond laser. It is based on the cross-correlation of an optical pulse with a subsequent pulse from the same laser. Temporal delay between these two pulses is achieved by varying the repetition rate of the laser. We validate the new scheme by a comparison with a cross-correlation measurement carried out with a conventional mechanical delay line.

Liquid crystal based electrically switchable Bragg structure for THz waves.

We demonstrate the first electronically switchable Bragg structure for THz frequencies. The structure works as stop-band filter and as mirror. It exhibits the 60 GHz broad stop-band around 300 GHz which can be removed by reorienting liquid crystal molecules in an external electric field. Our first proof-of-principle experiments agree very well with transfer matrix calculations.

Continuous wave terahertz spectrometer as a noncontact thickness measuring device.

We present a low cost terahertz (THz) spectrometer with coherent detection based on two simple and robust dipole antennas driven by two laser diodes. The spectrometer covers frequencies up to 1 THz, with a peak signal-to-noise ratio exceeding 40 dB for a lock-in integration time of 30 ms. We demonstrate that the thickness profile of a sample can be reconstructed from an acquired THz image.

Highly accurate optical material parameter determination with THz time-domain spectroscopy.

We improve the existing data extraction algorithms for THz time-domain spectroscopy (THz TDS) in two aspects. On the one hand, we merge the up-to-date knowledge of THz TDS signal processing into a single powerful optical material parameter extraction algorithm. On the other hand, we introduce a novel iterative algorithm that further enhances the accuracy of the parameter extraction. In contrast to most of the published experiments, we are able to reliably investigate samples with thicknesses as small as 100microm, samples with low indexes of refraction, i.e. close to 1, as well as samples with sharp peaks in the material parameter curves.

Terahertz time-domain spectroscopy and imaging of artificial RNA.

We use terahertz time-domain spectroscopy (THz-TDS) to measure the far-infrared dielectric function of two artificial RNA single strands, composed of polyadenylic acid (poly-A) and polycytidylic acid (poly-C). We find a significant difference in the absorption between the two types of RNA strands, and we show that we can use this difference to record images of spot arrays of the RNA strands. Under controlled conditions it is possible to use the THz image to distinguish between the two RNA strands. We discuss the requirements to sample preparation imposed by the lack of sharp spectral features in the absorption spectra.