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1.
Adv Sci (Weinh) ; 10(22): e2207617, 2023 Aug.
Artigo em Inglês | MEDLINE | ID: mdl-37327250

RESUMO

2D ferromagnet is a good platform to investigate topological effects and spintronic devices owing to its rich spin structures and excellent external-field tunability. The appearance of the topological Hall Effect (THE) is often regarded as an important sign of the generation of chiral spin textures, like magnetic vortexes or skyrmions. Here, interface engineering and an in-plane current are used to modulate the magnetic properties of the nearly room-temperature 2D ferromagnet Fe5 GeTe2 . An artificial topology phenomenon is observed in the Fe5 GeTe2 /MnPS3 heterostructure by using both anomalous Hall Effect and reflective magnetic circular dichroism (RMCD) measurements. Through tuning the applied current and the RMCD laser wavelength, the amplitude of the humps and dips observed in the hysteresis loops can be modulated accordingly. Magnetic field-dependent hysteresis loops demonstrate that the observed artificial topological phenomena are induced by the generation and annihilation of the magnetic domains. This work provides an optical method for investigating the topological-like effects in magnetic structures and proposes an effective way to modulate the magnetic properties of magnetic materials, which is important for developing magnetic and spintronic devices in van der Waals magnetic materials.

2.
ACS Nano ; 16(8): 12437-12444, 2022 Aug 23.
Artigo em Inglês | MEDLINE | ID: mdl-35900014

RESUMO

Two-dimensional (2D) magnets are crucial in the construction of 2D magnetic and spintronic devices. Many devices, including spin valves and multiple tunneling junctions, have been developed by vertically stacking 2D magnets with other functional blocks. However, owing to limited local interactions at the interfaces, the device structures are typically extremely complex. To solve this problem, the nonlocal manipulation of magnetism may be a good solution. In this study, we use the magneto-optical Kerr effect technique to demonstrate the nonlocal manipulation of magnetism in an itinerant 2D ferromagnet, Fe3GeTe2 (FGT), whose magnetism can be manipulated via an antiferromagnet/ferromagnet interface or a current-induced spin-orbital torque placed distant from the local site. It is discovered that the coupling of a small piece of MnPS3 (∼40 µm2) with FGT can significantly enhance the coercive field and emergence of exchange bias in the entire FGT flake (∼2000 µm2). Moreover, FGT flakes with different thicknesses have the same coercive field at low temperatures if they are coupled together. Our study provides an understanding of the basic magnetism of 2D itinerant ferromagnets as well as opportunities for engineering magnetism with an additional degree of freedom.

3.
ACS Appl Mater Interfaces ; 13(20): 24314-24320, 2021 May 26.
Artigo em Inglês | MEDLINE | ID: mdl-33977712

RESUMO

Fe3GeTe2/MnPS3 and Fe3GeTe2/MnPSe3 van der Waals heterostructures were fabricated by mechanical exfoliation. Via the magneto-optical Kerr effect and reflected magnetic circular dichroism measurements, we have observed nearly three times enhancement of the coercive field, improvement of Curie temperature, and exchange bias effect in both heterostructures. These observations may provide new insights into the emergent heterostructure devices between itinerant ferromagnets and metal thio- and selenophosphates for both applied and fundamental research studies in magnetic correlations.

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