Exciting space-time surface plasmon polaritons by irradiating a nanoslit structure.

Space-time (ST) wave packets are propagation-invariant pulsed optical beams that travel freely in dielectrics at a tunable group velocity without diffraction or dispersion. Because ST wave packets maintain these characteristics even when only one transverse dimension is considered, they can realize surface-bound waves (e.g., surface plasmon polaritons at a metal-dielectric interface, which we call ST-SPPs) that have the same unique characteristics as their freely propagating counterparts. However, because the spatiotemporal spectral structure of ST-SPPs is key to their propagation invariance on the metal surface, their excitation methodology must be considered carefully. Using finite-difference time-domain simulations, we show that an appropriately synthesized ST wave packet in free space can be coupled to an ST-SPP via a single nanoscale slit inscribed in the metal surface. Our calculations confirm that this excitation methodology yields surface-bound ST-SPPs that are localized in all dimensions (and can thus be considered as plasmonic "bullets"), which travel rigidly at the metal-dielectric interface without diffraction or dispersion at a tunable group velocity.

Compact dual-band spectral analysis via multiplexed rotated chirped volume Bragg gratings.

Chirped Bragg volume gratings (CBGs) offer a useful alternative for spectral analysis, but increasing the bandwidth necessitates increasing the device area. In contrast, recently developed rotated CBGs (r-CBGs), in which the Bragg structure is rotated by 45° with respect to the device facets, require increasing only the device length to extend the bandwidth, in addition to the convenience of resolving the spectrum at normal incidence. Here, we multiplex r-CBGs in the same device to enable spectral analysis in two independent spectral windows without increasing the system volume. This new, to the best of our knowledge, device, which we term an X-CBG, allows for compact multi-band spectroscopy in contiguous or separated spectral windows for the visible and near-infrared applications in nonlinear microscopy and material identification and sensing.

The propagation speed of optical speckle.

That the speed of light in vacuum is constant is a cornerstone of modern physics. However, recent experiments have shown that when the light field is confined in the transverse plane, the observed propagation speed of the light is reduced. This effect is a consequence of the transverse structure which reduces the component of wavevector of the light in the direction of propagation, thereby modifying both the phase and group velocity. Here, we consider the case of optical speckle, which has a random transverse distribution and is ubiquitous with scales ranging from the microscopic to the astronomical. We numerically investigate the plane-to-plane propagation speed of the optical speckle by using the method of angular spectrum analysis. For a general diffuser with Gaussian scattering over an angular range of 5°, we calculate the slowing of the propagation speed of the optical speckle to be on the order of 1% of the free-space speed, resulting in a significantly higher temporal delay compared to the Bessel and Laguerre-Gaussian beams considered previously. Our results have implications for studying optical speckle in both laboratory and astronomical settings.

Ultra-compact synthesis of space-time wave packets.

Space-time wave packets (STWPs) are pulsed fields in which a strictly prescribed association between the spatial and temporal frequencies yields surprising and useful behavior. However, STWPs to date have been synthesized using bulky free-space optical systems that require precise alignment. We describe a compact system that makes use of a novel optical component: a chirped volume Bragg grating that is rotated by 45° with respect to the plane-parallel device facets. By virtue of this grating's unique structure, cascaded gratings resolve and recombine the spectrum without free-space propagation or collimation. We produce STWPs by placing a phase plate that spatially modulates the resolved spectrum between such cascaded gratings, with a device volume of 25 × 25 × 8 mm3, which is orders-of-magnitude smaller than previous arrangements.

Rotated chirped volume Bragg gratings for compact spectral analysis.

We introduce a new, to the best of our knowledge, optical component-a rotated chirped volume Bragg grating (r-CBG)-that spatially resolves the spectrum of a normally incident light beam in a compact footprint and without the need for subsequent free-space propagation or collimation. Unlike conventional chirped volume Bragg gratings in which both the length and width of the device must be increased to increase the bandwidth, by rotating the Bragg structure we sever the link between the length and width of a r-CBG, leading to a significantly reduced device footprint for the same bandwidth. We fabricate and characterize such a device in multiple spectral windows, we study its spectral resolution, and confirm that a pair of cascaded r-CBGs can resolve and then recombine the spectrum. Such a device can lead to ultracompact spectrometers and pulse modulators.

Generation of OAM-carrying space-time wave packets with time-dependent beam radii using a coherent combination of multiple LG modes on multiple frequencies.

Space-time (ST) wave packets, in which spatial and temporal characteristics are coupled, have gained attention due to their unique propagation characteristics, such as propagation invariance and tunable group velocity in addition to their potential ability to carry orbital angular momentum (OAM). Through experiment and simulation, we explore the generation of OAM-carrying ST wave packets, with the unique property of a time-dependent beam radius at various ranges of propagation distances. To achieve this, we synthesize multiple frequency comb lines, each assigned to a coherent combination of multiple Laguerre-Gaussian (LGℓ,p) modes with the same azimuthal index but different radial indices. The time-dependent interference among the spatial modes at the different frequencies leads to the generation of the desired OAM-carrying ST wave packet with dynamically varying radii. The simulation results indicate that the dynamic range of beam radius oscillations increases with the number of modes and frequency lines. The simulated ST wave packet for OAM of orders +1 or +3 has an OAM purity of >95%. In addition, we experimentally generate and measure the OAM-carrying ST wave packets with time-dependent beam radii. In the experiment, several lines of a Kerr frequency comb are spatially modulated with the superposition of multiple LG modes and combined to generate such an ST wave packet. In the experiment, ST wave packets for OAM of orders +1 or +3 have an OAM purity of >64%. In simulation and experiment, OAM purity decreases and beam radius becomes larger over the propagation.

Synthesis of near-diffraction-free orbital-angular-momentum space-time wave packets having a controllable group velocity using a frequency comb.

Novel forms of light beams carrying orbital angular momentum (OAM) have recently gained interest, especially due to some of their intriguing propagation features. Here, we experimentally demonstrate the generation of near-diffraction-free two-dimensional (2D) space-time (ST) OAM wave packets (ℓ = +1, +2, or +3) with variable group velocities in free space by coherently combining multiple frequency comb lines, each carrying a unique Bessel mode. Introducing a controllable specific correlation between temporal frequencies and spatial frequencies of these Bessel modes, we experimentally generate and detect near-diffraction-free OAM wave packets with high mode purities (>86%). Moreover, the group velocity can be controlled from 0.9933c to 1.0069c (c is the speed of light in vacuum). These ST OAM wave packets might find applications in imaging, nonlinear optics, and optical communications. In addition, our approach might also provide some insights for generating other interesting ST beams.

Space-time wave packets localized in all dimensions.

Optical wave packets that are localized in space and time, but nevertheless overcome diffraction and travel rigidly in free space, are a long sought-after field structure with applications ranging from microscopy and remote sensing, to nonlinear and quantum optics. However, synthesizing such wave packets requires introducing non-differentiable angular dispersion with high spectral precision in two transverse dimensions, a capability that has eluded optics to date. Here, we describe an experimental strategy capable of sculpting the spatio-temporal spectrum of a generic pulsed beam by introducing arbitrary radial chirp via two-dimensional conformal coordinate transformations of the spectrally resolved field. This procedure yields propagation-invariant 'space-time' wave packets localized in all dimensions, with tunable group velocity in the range from 0.7c to 1.8c in free space, and endowed with prescribed orbital angular momentum. By providing unprecedented flexibility in sculpting the three-dimensional structure of pulsed optical fields, our experimental strategy promises to be a versatile platform for the emerging enterprise of space-time optics.

Refraction of space-time wave packets in a dispersive medium.

Space-time (ST) wave packets are a class of pulsed optical beams whose spatiotemporal spectral structure results in propagation invariance, tunable group velocity, and anomalous refractive phenomena. Here, we investigate the refraction of ST wave packets normally incident onto a planar interface between two dispersive, homogeneous, isotropic media. We formulate a new, to the best of our knowledge, refractive invariant for ST wave packets in this configuration, from which we obtain a law of refraction that determines the change in their group velocity across the interface. We verify this new refraction law in ZnSe and CdSe, both of which manifest large chromatic dispersion at near-infrared frequencies in the vicinity of their band edges. ST wave packets can thus be utilized in nonlinear optics for bridging large group-velocity mismatches in highly dispersive scenarios.

Arbitrarily accelerating space-time wave packets.

All known realizations of optical wave packets that accelerate along their propagation axis, such as Airy wave packets in dispersive media or wave-front-modulated X-waves, exhibit a constant acceleration; that is, the group velocity varies linearly with propagation. Here we synthesize space-time wave packets that travel in free space with arbitrary axial acceleration profiles, including group velocities that change with integer or fractional exponents of the distance. Furthermore, we realize a composite acceleration profile: the wave packet accelerates from an initial to a terminal group velocity, before decelerating back to the initial value. These never-before-seen optical-acceleration phenomena are produced using the same experimental arrangement that precisely sculpts the wave packet's spatio-temporal spectral structure.

Tunability of space-time wave packet carrying tunable and dynamically changing OAM value.

Space-time (ST) wave packets have gained much interest due to their dynamic optical properties. Such wave packets can be generated by synthesizing frequency comb lines, each having multiple complex-weighted spatial modes, to carry dynamically changing orbital angular momentum (OAM) values. Here, we investigate the tunability of such ST wave packets by varying the number of frequency comb lines and the combinations of spatial modes on each frequency. We experimentally generate and measure the wave packets with tunable OAM values from +1 to +6 or from +1 to +4 during a ∼5.2-ps period. We also investigate, in simulation, the temporal pulse width of the ST wave packet and the nonlinear variation of the OAM values. The simulation results show that: (i) a pulse width can be narrower for the ST wave packet carrying dynamically changing OAM values using more frequency lines; and (ii) the nonlinearly varying OAM value can result in different frequency chirps along the azimuthal direction at different time instants.

Space-time vector light sheets.

We introduce the space-time (ST) vector light sheet. This unique one-dimensional ST wave packet is characterized by classical entanglement (CE), a correlation between at least two non-separable intrinsic degrees-of-freedom (DoFs), which in this case are the spatiotemporal DoFs in parallel with the spatial-polarization DoFs. We experimentally confirm that the ST vector light sheet maintains the intrinsic features of the uniformly polarized ST light sheet, such as near-diffraction-free propagation and self-healing, while also maintaining the intrinsic polarization structure of common vector beams, such as those that are radially polarized and azimuthally polarized. We also show that the vector beam structure of the ST vector light sheet is maintained in the subluminal and superluminal regimes.

Refraction of space-time wave packets: I. theoretical principles.

Space-time (ST) wave packets are pulsed optical beams endowed with precise spatio-temporal structure by virtue of which they exhibit unique and useful characteristics such as propagation invariance and tunable group velocity. We study in detail here, and in two accompanying papers, the refraction of ST wave packets at planar interfaces between non-dispersive, homogeneous, and isotropic dielectrics. We formulate a law of refraction that determines the change in the ST wave-packet group velocity across such an interface as a consequence of a newly identified optical refractive invariant that we call the "spectral curvature". Because the spectral curvature vanishes in conventional optical fields where the spatial and temporal degrees of freedom are separable, these phenomena have not been observed to date. We derive the laws of refraction for baseband, X wave, and sideband ST wave packets that reveal fascinating refractive phenomena, especially for the former class of wave packets. We predict theoretically, and confirm experimentally in the accompanying papers, refractive phenomena such as group-velocity invariance (ST wave packets whose group velocity does not change across the interface), anomalous refraction (group-velocity increase in higher-index media), group-velocity inversion (change in the sign of the group velocity upon refraction but not its magnitude), and the dependence of the group velocity of the refracted ST wave packet on the angle of incidence.

Refraction of space-time wave packets: II. experiments at normal incidence.

The refraction of space-time (ST) wave packets offers many fascinating surprises with respect to conventional pulsed beams. In the first paper in this sequence [J. Opt. Soc. Am. A38, 1409 (2021)10.1364/JOSAA.430105], we theoretically described the refraction of all families of ST wave packets at normal and oblique incidence at a planar interface between two nondispersive, homogeneous, isotropic dielectrics. Here, in this second paper in the sequence, we present experimental verification of the refractive phenomena predicted for baseband ST wave packets upon normal incidence on a planar interface. Specifically, we observe group velocity invariance, normal and anomalous refraction, and group velocity inversion leading to group delay cancellation. These phenomena are verified in a set of optical materials with refractive indices ranging from 1.38 to 1.76, including MgF2, fused silica, BK7 glass, and sapphire. We also provide a geometrical representation of the physics associated with anomalous refraction in terms of the dynamics of the spectral support domain for ST wave packets on the surface of the light cone.

Refraction of space-time wave packets: III. experiments at oblique incidence.

The refraction of space-time (ST) wave packets at planar interfaces between non-dispersive, homogeneous, isotropic dielectrics exhibits fascinating phenomena, even at normal incidence. Examples of such refractive phenomena include group-velocity invariance across the interface, anomalous refraction, and group-velocity inversion. Crucial differences emerge at oblique incidence with respect to the results established at normal incidence. For example, the group velocity of the refracted ST wave packet can be tuned simply by changing the angle of incidence. In the third paper, we present experimental verification of the refractive phenomena exhibited by ST wave packets at oblique incidence that were in the first paper of this sequence [J. Opt. Soc. Am. A38, 1409 (2021)10.1364/JOSAA.430105]. We also examine a proposal for "blind synchronization," whereby identical ST wave packets arrive simultaneously at different receivers without a priori knowledge of their locations except that they are all located at the same depth beyond an interface between two media. A first proof-of-principle experimental demonstration of this effect is provided.

Isochronous space-time wave packets.

The group delay incurred by an optical wave packet depends on its path length. Therefore, when a wave packet is obliquely incident on a planar homogeneous slab, the group delay upon traversing it inevitably increases with the angle of incidence. Here, we confirm the existence of isochronous "space-time" (ST) wave packets: pulsed beams whose spatiotemporal structure enables them to traverse the layer with a fixed group delay over a wide span of incident angles. This unique behavior stems from the dependence of the group velocity of a refracted ST wave packet on its angle of incidence. Isochronous ST wave packets are observed in slabs of optical materials with indices ranging from 1.38 to 2.5 for angles up to 50° away from normal incidence.

Space-time wave packets violate the universal relationship between angular dispersion and pulse-front tilt.

Introducing angular dispersion into a pulsed field tilts the pulse front with respect to the phase front. There exists between the angular dispersion and pulse-front tilt a universal relationship that is device-independent, and also independent of the pulse shape and bandwidth. We show here that this relationship is violated by propagation-invariant space-time (ST) wave packets, which are pulsed beams endowed with precise spatiotemporal structure corresponding to a particular form of angular dispersion. We demonstrate theoretically and experimentally that ST wave packets represent, to the best of our knowledge, the first example in optics of non-differentiable angular dispersion, resulting in pulse-front tilt that depends on the square-root of the pulse bandwidth.

Hybrid guided space-time optical modes in unpatterned films.

Light is confined transversely and delivered axially in a waveguide. However, waveguides are lossy static structures whose modal characteristics are fundamentally determined by their boundary conditions. Here we show that unpatterned planar waveguides can provide low-loss two-dimensional waveguiding by using space-time wave packets, which are unique one-dimensional propagation-invariant pulsed optical beams. We observe hybrid guided space-time modes that are index-guided in one transverse dimension and localized along the unbounded dimension. We confirm that these fields enable overriding the boundary conditions by varying post-fabrication the group index of the fundamental mode in a 2-µm-thick, 25-mm-long silica film, achieved by modifying the field's spatio-temporal structure. Tunability of the group index over an unprecedented range from 1.26 to 1.77 is verified while maintaining a spectrally flat zero-dispersion profile. Our work paves the way to utilizing space-time wave packets in on-chip platforms, and enable phase-matching strategies that circumvent restrictions due to intrinsic material properties.

Accelerating and Decelerating Space-Time Optical Wave Packets in Free Space.

Although a plethora of techniques are now available for controlling the group velocity of an optical wave packet, there are very few options for creating accelerating or decelerating wave packets whose group velocity varies controllably along the propagation axis. Here we show that "space-time" wave packets in which each wavelength is associated with a prescribed spatial bandwidth enable the realization of optical acceleration and deceleration in free space. Endowing the field with precise spatiotemporal structure leads to group-velocity changes as high as ∼c observed over a distance of ∼20 mm in free space, which represents a boost of at least ∼4 orders of magnitude over X waves and Airy pulses. The acceleration implemented is, in principle, independent of the initial group velocity, and we have verified this effect in both the subluminal and superluminal regimes.

Free-space optical delay line using space-time wave packets.

An optical buffer featuring a large delay-bandwidth-product-a critical component for future all-optical communications networks-remains elusive. Central to its realization is a controllable inline optical delay line, previously accomplished via engineered dispersion in optical materials or photonic structures constrained by a low delay-bandwidth product. Here we show that space-time wave packets whose group velocity is continuously tunable in free space provide a versatile platform for constructing inline optical delay lines. By spatio-temporal spectral-phase-modulation, wave packets in the same or in different spectral windows that initially overlap in space and time subsequently separate by multiple pulse widths upon free propagation by virtue of their different group velocities. Delay-bandwidth products of  ~100 for pulses of width  ~1 ps are observed, with no fundamental limit on the system bandwidth.