Sub-cycle strong-field tunneling dynamics in solids.

Tunneling ionization is a crucial process in the interaction between strong laser fields and matter which initiates numerous nonlinear phenomena including high-order harmonic generation, photoelectron holography, etc. Both adiabatic and nonadiabatic tunneling ionization are well understood in atomic systems. However, the tunneling dynamics in solids, especially nonadiabatic tunneling, has not yet been fully understood. Here, we study the sub-cycle resolved strong-field tunneling dynamics in solids via a complex saddle-point method. We compare the instantaneous momentum at the moment of tunneling and the tunneling distances over a range of Keldysh parameters. Our results demonstrate that for nonadiabatic tunneling, tunneling ionization away from Γ point is possible. When this happens the electron has a nonzero initial velocity when it emerges in the conduction band. Moreover, consistent with atomic tunneling, a reduced tunneling distance as compared to the quasi-static case is found. Our results provide remarkable insight into the basic physics governing the sub-cycle electron tunneling dynamics with significant implications for understanding subsequent strong-field nonlinear phenomena in solids.

Attosecond temporal confinement of interband excitation by intraband motion.

High order harmonic generation (HHG) in semiconductors opens a new frontier in strong field physics and attosecond science. However, the underlying physical mechanisms are not yet fully understood and lively debated. Here, we identify and discuss carrier-wave population transfer as a novel and important dynamical effect. We find that the interband excitation occurs in an extremely short time window due to the intraband motion. Our analysis based on this finding allows for a physically intuitive interpretation of the anomalous carrier-envelope phase dependence observed in HHG from MgO and to understand the dominant role of the interband polarization as reported in a series of recent semiconductor HHG experiments. Motivated by the discovered coupling mechanism, we demonstrate that the interband excitation can be controlled by an appropriately tailored two-color field. An ultrabroad supercontinuum spectrum covering the entire plateau region can be generated which directly creates an isolated-attosecond pulse even without phase compensation. Our results provide remarkable insight into the basic physics governing the sub-cycle electron motion with significant implications for the generation of isolated-attosecond light pulses in semiconductor materials.