From localized to delocalized plasmonic modes, first observation of superradiant scattering in disordered semi-continuous metal films.

Our study proposes a new way to observe and explain the presence of extended plasmonic modes in disordered semi-continuous metal films before the percolation threshold. Attenuated total reflection spectroscopy allows us to follow the transition of plasmon modes from localized to delocalized resonances, but also reveals unobserved collective plasmon modes. These bright modes with out-of-plane polarization are transverse collective plasmonic resonances. By increasing the density of metallic nanoparticles in a wavelength scale, we observe an angular squeezing and spectral broadening of these modes. This behavior can be explained considering that transverse localized surface plasmon resonances of each nanoparticle, all resonant, interact in a collective and coherent way via a common confined light mode: the evanescent wave. These many-body resonances, which have never been clearly identified in such disordered semi-continuous metal films, can be described by analogy with atomic physics as superradiant modes. Our first simulations, using dyadic Green's formalism, demonstrate the existence of this mode for a dense array of plasmonic systems. In this regime, the radiation rate of the superradiant mode increases with the number of tied dipoles. This explains the spectral broadening observed in our work and constitutes the first manifestation of superradiance mode in plasmonic random structure.

Electromigrated electrical optical antennas for transducing electrons and photons at the nanoscale.

Background: Electrically controlled optical metal antennas are an emerging class of nanodevices enabling a bilateral transduction between electrons and photons. At the heart of the device is a tunnel junction that may either emit light upon injection of electrons or generate an electrical current when excited by a light wave. The current study explores a technological route for producing these functional units based upon the electromigration of metal constrictions. Results: We combine multiple nanofabrication steps to realize in-plane tunneling junctions made of two gold electrodes, separated by a sub-nanometer gap acting as the feedgap of an optical antenna. We electrically characterize the transport properties of the junctions in the light of the Fowler-Nordheim representation and the Simmons model for electron tunneling. We demonstrate light emission from the feedgap upon electron injection and show examples of how this nanoscale light source can be coupled to waveguiding structures. Conclusion: Electromigrated in-plane tunneling optical antennas feature interesting properties with their unique functionality enabling interfacing electrons and photons at the atomic scale and with the same device. This technology may open new routes for device-to-device communication and for interconnecting an electronic control layer to a photonic architecture.

Launching propagating surface plasmon polaritons by a single carbon nanotube dipolar emitter.

We report on the excitation of propagating surface plasmon polaritons in thin metal films by a single emitter. Upon excitation in the visible regime, individual semiconducting single-walled carbon nanotubes are shown to act as directional near-infrared point dipole sources launching propagating surface plasmons mainly along the direction of the nanotube axis. Plasmon excitation and propagation is monitored in Fourier and real space by leakage radiation microscopy and is modeled by rigorous theoretical calculations. Coupling to plasmons almost completely reshapes the emission of nanotubes both spatially and with respect to polarization as compared to photoluminescence on a dielectric substrate.

Excitation of a one-dimensional evanescent wave by conical edge diffraction of surface plasmon.

The experimental observation of a one-dimensional evanescent wave supported by a 90◦ metal edge is reported. Through a measurement of in-plane momenta, we clearly demonstrate the dimensional character of this surface wave and show that it is non-radiative in the superstrate. Excitation conditions, lateral extension and polarization properties of this wave are discussed. Finally, we explore the effect of the surrounding dielectric medium and demonstrate that a single edge can sustain distinct excitations.

Molecule non-radiative coupling to a metallic nanosphere: an optical theorem treatment.

The non-radiative coupling of a molecule to a metallic spherical particle is approximated by a sum involving particle quasistatic polarizabilities. We demonstrate that energy transfer from molecule to particle satisfies the optical theorem if size effects corrections are properly introduced into the quasistatic polarizabilities. We hope that this simplified model gives valuable information on the coupling mechanism between molecule and metallic nanostructures available for, e.g., surface enhanced spectroscopy signal analysis.

Gain-assisted propagation in a plasmonic waveguide at telecom wavelength.

The spatial confinement of surface plasmon polaritons is a promising route for realizing optical on-board interconnects. However, mode losses increase with the confinement factor. To overcome this road block, we investigate propagation assisted by stimulated emission in a polymer strip-loaded plasmonic waveguide doped with nanocrystals. We achieve 27% increase of the propagation length at telecom wavelength corresponding to a 160 cm(-1) optical gain coefficient. Such a configuration is a step toward integrated plasmonic amplifiers.

Polarization state of the optical near field.

The polarization state of the optical electromagnetic field lying several nanometers above complex dielectric-air interfaces reveals the intricate light-matter interaction that occurs in the near-field zone. From the experimental point of view, access to this information is not direct and can only be extracted from an analysis of the polarization state of the detected light. These polarization states can be calculated by different numerical methods, well suited to near-field optics. In this paper, we apply two different techniques (localized Green's function method and differential theory of gratings) to separate each polarization component associated with both electric and magnetic optical near fields produced by nanometer sized objects. A simple dipolar model is used to get an insight into the physical origin of the near-field polarization state. In a second stage, accurate numerical simulations of field maps complete data produced by analytical models. We conclude this study by demonstrating the role played by the near-field polarization in the formation of the local density of states.