Enhanced coherence between condensates formed resonantly at different times.

We demonstrate coherence between exciton-polariton condensates created resonantly at different times. The coherence persists much longer than the individual particle dephasing time, and this persistence increases as the particle density increases. The observed coherence time exceeds that of the injecting laser pulse by more than an order of magnitude. We show that this significant coherence enhancement relies critically on the many-body particle interactions, as verified by its dependence on particle density, interaction strength, and bath temperature, whereas the mass of the particles plays no role in the condensation of resonantly injected polaritons. Furthermore, we observe a large nonlinear phase shift resulting from intra-condensate interaction energy. Our results provide a new approach for probing ultrafast dynamics of resonantly-created condensates and open new directions in the study of coherence in matter.

Domain dynamics in thin solid films following ultrashort pulse excitation.

MnAs epilayers grown on GaAs are used as a model system to study the effects of strain and epitaxial constraints on the dynamics of structural domains following 150 fs pulse pumping. Optical diffraction over 7 orders of magnitude of time is used to probe the evolution of the domains that are spatially periodic between 10 and 42 °C because of misfit strain and substrate mediated periodic elastic strain. Following excitation of 150 and 190 nm thick films, the domain fractions and the elastic strain oscillate with an ~400 ps period while the average low temperature phase fraction decreases monotonically for ~2 ns reflecting MnAs heat diffusion. Equilibrium structures are restored in 100 ns-2 µs via substrate heat diffusion. Excitation of transient periodic domains from the homogeneous low temperature phase can occur for temperatures as low as 4 °C but only after ~20 ns during film cooling.

Dynamic Stark effect in strongly coupled microcavity exciton polaritons.

We present experimental observations of a nonresonant dynamic Stark shift in strongly coupled microcavity quantum well exciton polaritons--a system which provides a rich variety of solid-state collective phenomena. The Stark effect is demonstrated in a GaAs/AlGaAs system at 10 K by femtosecond pump-probe measurements, with the blueshift approaching the meV scale for a pump fluence of 2 mJ cm(-2) and 50 meV red detuning, in good agreement with theory. The energy level structure of the strongly coupled polariton Rabi doublet remains unaffected by the blueshift. The demonstrated effect should allow generation of ultrafast density-independent potentials and imprinting well-defined phase profiles on polariton condensates, providing a powerful tool for manipulation of these condensates, similar to dipole potentials in cold-atom systems.

All-optical ultrafast control of beaming through a single sub-wavelength aperture in a metal film.

We propose an ultrafast all-optical technique to control and beam the light emerging from a sub-wavelength slit in a planar gold film by exciting a transient grating in the area around the slit. A FDTD model is used to show how excitation of surface plasmon polaritons by the grating governs the beaming process. Both the grating and the beaming effect are shown to decay on a picosecond time-scale. An on-off contrast of 5 dB is obtained for the beaming, with a divergence angle of only 2.4 degrees.

Ultrafast silicon-based active plasmonics at telecom wavelengths.

Using a gold/silicon grating coupler and modulating the silicon dielectric constant with 775 nm, 800 fs pump pulses we demonstrate an ultrafast spectral shift to a surface plasmon polariton coupling resonance for 1300-1700 nm probe pulses. With a modest pump fluence of 2.2 mJ cm(-2) the pump-induced free carriers shift the resonance by more than its width, with recovery occurring in 103 ps due to surface recombination.

Ultrafast all-optical coupling of light to surface plasmon polaritons on plain metal surfaces.

We propose and demonstrate an ultrafast all-optical method to couple light to surface plasmon polaritons on planar gold films. By interfering two 150 fs, 810 nm pulses we excite a transient grating in the temperature of the free electrons of the metal, resulting in a grating in the dielectric function, and leading to a 1 ps launch window for plasmonic excitation. We use pump-probe experiments to identify these ultrashort plasmonic excitations between 520 and 570 nm.

Imaging the spin Hall effect of light inside semiconductors via absorption.

The opposite transverse shifts for the right and left circular polarization components of a 100 fs 820 nm linearly polarized pulse focused onto GaAs are observed in situ via absorption. A time-delayed normally incident probe pulse scanned across the excitation spot detects the differential circular dichroism associated with the pump-induced transfer of spin angular momentum from light to electrons. More generally, we show that for a nonnormally incident probe, one can observe the spin Hall effect for probe light through a variety of pump-induced changes to a material's optical properties.

Ultrafast carrier kinetics in exfoliated graphene and thin graphite films.

Time-resolved transmissivity and reflectivity of exfoliated graphene and thin graphite films on a 295 K SiO(2)/Si substrate are measured at 1300 nm following excitation by 150 fs, 800 nm pump pulses. From the extracted transient optical conductivity we identify a fast recovery time constant which increases from approximately 200 to 300 fs and a longer one which increases from 2.5 to 5 ps as the number of atomic layers increases from 1 to approximately 260. We attribute the temporal recovery to carrier cooling and recombination with the layer dependence related to substrate coupling. Results are compared with related measurements for epitaxial, multilayer graphene.

Ultrafast control of grating-assisted light coupling to surface plasmons.

We demonstrate subpicosecond control over the coupling of free-space radiation to surface-plasmon polaritons using 830 and 500 nm period gold gratings. Thermal changes to the electron distribution following irradiation by 100 fs, 810 nm pulses produce a shift of the 570 nm plasmon resonance by approximately 0.75 nm with reflectivity change up to 6% and decay time of approximately 1 ps.

Coherently controlled ballistic charge currents injected in single-walled carbon nanotubes and graphite.

Ballistic electrical currents are optically injected into aligned single-walled carbon nanotubes and bulk graphite at 300 K via quantum interference between single and two photon absorption of phase-related 700 and 1400 nm, 150 fs pulses. The transient currents are detected via the emitted terahertz radiation. Optical phase and power dependence are consistent with the quantum interference optical process. Under similar excitation conditions, the peak current for a forest of nanotubes, with a diameter distribution of approximately 2.5 +/- 1.5 nm, is 9 +/- 1 times larger than that in graphite. At peak focused intensities of 10 GW cm(-2) (1400 nm) and 0.15 GW cm(-2) (700 nm), the peak current is approximately 1 nA per nanotube. The peak current for pump light polarized along the tubes is approximately 3.5 times higher than that for light polarized perpendicular to the tubes.

Enhanced second-harmonic generation in AlGaAs microring resonators.

Highly efficient second-harmonic generation can be achieved by harnessing resonance effects in microring resonator structures. We propose an angular quasi-phase-matching scheme based on the position dependence of polarization inside the ring resonator.

Single-beam differential z-scan technique.

We report a single-beam, differential z-scan technique with improved sensitivity for the determination of nonlinear absorption and refraction of materials. A sample is scanned in the direction of beam propagation as usual, but, in addition, its longitudinal position is dithered, producing a detector signal proportional to the spatial derivative of only the nonlinear transmission and therefore giving a background-free signal; the nonlinear transmission for any spatial position of the sample can be recovered by simple integration. For both open and closed aperture scans in GaP, we find an improvement in the signal-to-noise ratio of >5 x compared with a balanced z-scan setup, but this can be improved with apparatus optimization. Nonlinear phase distortions